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Method for extracting bromine from brine

A brine and hydrophobic technology, applied in the field of bromine extraction, can solve the problems of temperature influence and high energy consumption, and achieve the effect of improving efficiency and reducing energy consumption

Active Publication Date: 2012-06-27
TIANJIN SEA WATER DESALINATION & COMPLEX UTILIZATION INST STATE OCEANOGRAPHI
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

[0004] Aiming at the disadvantages of high energy consumption and serious temperature influence in the prior art bromine extraction method, the present invention provides a new bromine extraction method, which utilizes the affinity of non-polar organic solvents and hydrophobic microporous membranes to form The organic solvent liquid membrane supported by the hydrophobic microporous membrane, with the help of the dissolving ability of the organic solvent for bromine and the diffusion of bromine in the organic solvent, through the non-dispersive contact of the bromine-containing brine and the absorption liquid flowing independently on both sides of the liquid membrane And the same level of transfer, the bromine in the brine is absorbed by the alkaline absorption liquid, the efficiency of the bromine extraction process is improved, and the energy consumption is reduced

Method used

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Examples

Experimental program
Comparison scheme
Effect test

Embodiment 1

[0015] Take the hollow fiber membrane module with polypropylene microporous membrane inside, the membrane area is 1m 2 (Inner diameter meter), inner diameter 0.36mm, membrane pore diameter 0.05μm, adding kerosene to soak for 24 hours, polypropylene hollow fiber microporous membrane becomes transparent. 1m 3 The brine with a bromide ion concentration of 201.23 mg / L was passed into 100 g of chlorine gas to oxidize bromine ions as free bromine, and the free bromine concentration in the brine was measured to be 183.11 mg / L. Add hydrochloric acid to adjust the pH to 3.5, and then take a sodium formate solution with a concentration of 28g / L. Both 2L of sodium formate solution and 3L of acidified and oxidized brine will circulate through the outside and inside of the hollow fiber membrane at a speed of 20L / h. The solution absorbed the bromine in the brine. After 25 minutes, the bromine concentration in the brine was measured to be 17.42 mg / L, and the debromination rate reached 90.48%. ...

Embodiment 2

[0017] Take the hollow fiber membrane module with polypropylene microporous membrane inside, the membrane area is 1m 2 (Inner diameter meter), inner diameter 0.36mm, membrane pore diameter 0.05μm, adding kerosene to soak for 24 hours, polypropylene hollow fiber microporous membrane becomes transparent. 1m 3 Brine with a bromide ion concentration of 344.43mg / L was passed into 170g of chlorine to oxidize bromine ions as free bromine, and hydrochloric acid was added to adjust the pH to 3.5. The free bromine concentration in the brine was measured to be 311.41mg / L. Take 2L of sodium hydroxide solution with a concentration of 40g / L and 3L of brine after acidification and oxidation, and circulate them through the outer and inner sides of the hollow fiber membranes respectively. The flow rate of sodium hydroxide solution is 20L / h, the flow rate of brine is 60L / h, 25 Minutes later, the bromine concentration in the brine was 11.09mg / L, and the debromination rate reached 96.44%.

Embodiment 3

[0019] Take the hollow fiber membrane module with the polyvinylidene fluoride microporous membrane inside, the membrane area is 0.25m 2 (Inner diameter meter), the inner diameter is 1.1mm, the membrane pore diameter is 0.05μm, and kerosene is added to soak for 24 hours, the polyvinylidene fluoride hollow fiber microporous membrane becomes transparent. 1m 3 Brine with a bromide ion concentration of 223.51 mg / L was passed into chlorine gas and 110 g of oxidized bromine ions were free bromine. Hydrochloric acid was added to adjust the pH to 3.0. The free bromine concentration in the brine was measured to be 198.63 mg / L. Then take 2L of sodium hydroxide solution with a concentration of 40g / L and 2L of acidified and oxidized brine, and circulate them through the outer and inner sides of the hollow fiber membranes respectively. The sodium hydroxide solution flow rate is 10L / h, and the brine flow rate is 20L / h. After 30 minutes, the free bromine concentration in the brine was measured ...

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PUM

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Abstract

The invention discloses a method for extracting bromine from brine. In the method, the affinity of a non-polar solvent and a hydrophobic microporous membrane is utilized and a microporous membrane supported organic solvent liquid membrane is formed; and the brine-containing free bromide and absorption solution flow on two sides of the liquid membrane respectively, and the free bromide is absorbedby the alkaline absorption solution through the liquid membrane by means of the solubility and diffusivity of the free bromide in the organic solvent so as to separate the bromine enriched in the brine. The method comprises the technical steps of organic liquid membrane preparation, brine acidification, and bromine separation and extraction, wherein the hydrophobic microporous membrane is immersed in the non-polar solvent to prepare the organic liquid membrane; the acidified brine which is filled with chloride and the alkaline absorption solution flow on the two sides of the organic liquid membrane respectively; in the organic liquid membrane preparation step, the organic solvent is kerosene, carbon tetrachloride and dichloroethane, and the hydrophobic microporous membrane is a microporous membrane of polypropylene, polyvinylidene fluoride and polyethylene; and in the bromine separation and extraction step, the alkaline absorption solution is 28g / L sodium formate or 40g / L sodium hydroxide solution.

Description

Technical field [0001] The invention relates to bromine extraction technology, in particular to a method for extracting bromine from brine by using a liquid film formed by an organic solvent and a hydrophobic microporous membrane. Background technique [0002] Bromine is the only liquid non-metallic element at room temperature. It has strong oxidizing properties and is one of the basic chemical raw materials. It is widely used in the synthesis of detergents, flame retardants, refrigerants, water treatment agents and pharmaceutical intermediates. . Bromine extraction technology is a technological process that separates bromine in the form of elemental substances. Currently, it is mainly extracted from brine. Industrial bromine extraction technology is mainly based on steam distillation and air blowing. The steam distillation method uses steam to distill the elemental bromine, which consumes a large amount of steam, and is generally suitable for high-grade bromine-containing raw ...

Claims

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Application Information

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Patent Type & Authority Patents(China)
IPC IPC(8): C01B7/09
Inventor 张慧峰刘伟姚颖高书宝王颖张雨山王国强
Owner TIANJIN SEA WATER DESALINATION & COMPLEX UTILIZATION INST STATE OCEANOGRAPHI