Unleaded epoxy resin composite for printed circuit copper clad laminate
A lead-free epoxy resin and epoxy resin technology, used in printed circuit components, circuit substrate materials, layered products, etc., can solve the problems of harsh resin Tg and heat resistance, large thermal expansion coefficient, and large performance drop. , to achieve the effect of good reactivity, easy impregnation and reduction of thermal expansion coefficient
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Embodiment 1
[0026] (1) Preparation of acetone solution containing modified epoxy resin:
[0027] 360 parts of bisphenol A type epoxy resin, 28 parts of tetrafunctional novolac epoxy resin, 120 parts of brominated bisphenol A type epoxy resin, 150 parts of tetrabromobisphenol A and 9 parts of tetraphenol Add 0.15 parts of catalyst butyltriphenylphosphine bromide when heating at 120°C, continue heating to 170°C for 2 hours; then cool down to 150°C, add 80 parts of norophenol formaldehyde ring Oxygen resin, after mixing evenly, add acetone solvent to dissolve into the acetone solution containing modified epoxy resin that the solid content is 75%. The above-mentioned consumptions are all parts by weight.
[0028] (2) Preparation of epoxy resin composition:
[0029] Take by weighing the acetone solution containing modified epoxy resin obtained in step (1) as shown in the table below, and add inorganic filler, phenolic curing agent, curing accelerator and solvent to the acetone solution conta...
Embodiment 2
[0034] (1) Preparation of acetone solution containing modified epoxy resin:
[0035] 380 parts of bisphenol F type epoxy resin, 40 parts of four-functional novolac epoxy resin, 120 parts of brominated bisphenol A type epoxy resin, 140 parts of tetrabromobisphenol A and 13 parts of tetraphenol Add 0.12 parts of catalyst butyltriphenylphosphine bromide when heating at 120°C, continue heating to 170°C for 1.8-2.5 hours; then cool down to 130°C, add 120-135 parts of thread Type phenol-formaldehyde epoxy resin, after mixing evenly, add acetone solvent and dissolve into the acetone solution that the solid content is 75% containing modified epoxy resin. The above-mentioned consumptions are all parts by weight.
[0036] (2) Preparation of epoxy resin composition:
[0037] Take by weighing the acetone solution containing modified epoxy resin obtained in step (1) as shown in the table below, and add inorganic filler, phenolic curing agent, curing accelerator and solvent to the acetone...
Embodiment 3
[0042] (1) Preparation of acetone solution containing modified epoxy resin:
[0043] 330 parts of bisphenol S type epoxy resin, 39 parts of four-functional novolac epoxy resin, 95 parts of brominated bisphenol A type epoxy resin, 170 parts of tetrabromobisphenol A and 14 parts of tetraphenol Mix and heat the base ethane together, add 0.10 parts of catalyst butyltriphenylphosphine bromide when heating at 120°C, continue heating to 170°C for 2 hours; then cool down to 150°C, add 80 parts of norophenol formaldehyde ring Oxygen resin, after mixing evenly, add acetone solvent to dissolve into the acetone solution containing modified epoxy resin that the solid content is 75%. The above-mentioned consumptions are all parts by weight.
[0044] (2) Preparation of epoxy resin composition:
[0045]Take by weighing the acetone solution containing modified epoxy resin obtained in step (1) as shown in the table below, and add inorganic filler, phenolic curing agent, curing accelerator and...
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