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Preparation method of La-doped W-Cu composite powder

A composite powder, w-cu technology, applied in coating and other directions, can solve the problems of easy introduction of impurities, long processing time, and difficulty in mass production in the preparation method, and achieve low preparation cost, high degree of homogenization, and high degree of densification. Effect

Active Publication Date: 2013-02-13
HEFEI UNIV OF TECH
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

Some of the above methods have high costs, long processing time, and difficulty in mass production. Some preparation methods have the phenomenon of easy introduction of impurities, high oxygen content, and easy agglomeration of powders.

Method used

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Examples

Experimental program
Comparison scheme
Effect test

Embodiment 1

[0019] 1. Preparation of activated tungsten powder

[0020] The tungsten powder with a particle size of less than 1 micron is placed in the activation solution for ultrasonic activation for 30 minutes, the ultrasonic frequency is 40KHz, and the power is 300-400W. After the activation is completed, it is washed three times with deionized water and dried at 200 ° C for 1 hour to obtain activated tungsten powder. ;

[0021] The activation solution is an aqueous solution of hydrofluoric acid, ammonium fluoride and nitric acid, and the concentration of hydrofluoric acid in the activation solution is 60 ml / L, calculated as a hydrofluoric acid solution with a mass concentration of 40%; the concentration of ammonium fluoride is 9g / L; the concentration of nitric acid is 60ml / L, calculated as a nitric acid solution with a mass concentration of 65%;

[0022] 2. Preparation of composite powder

[0023] The activated tungsten powder was added to the chemical deposition solution, the amou...

Embodiment 2

[0029] 1. Preparation of activated tungsten powder

[0030] The tungsten powder with a particle size of less than 1 micron is placed in the activation solution for ultrasonic activation for 40 minutes, the ultrasonic frequency is 40KHz, and the power is 300-400W. After the activation is completed, it is washed three times with deionized water and dried at 180 ° C for 3 hours to obtain activated tungsten powder. ;

[0031] The activation solution is an aqueous solution of hydrofluoric acid, ammonium fluoride and nitric acid, and the concentration of hydrofluoric acid in the activation solution is 30 ml / L, calculated as a hydrofluoric acid solution with a mass concentration of 40%; the concentration of ammonium fluoride is 8g / L; the concentration of nitric acid is 80ml / L, calculated as a nitric acid solution with a mass concentration of 65%;

[0032] 2. Preparation of composite powder

[0033] The activated tungsten powder was added to the chemical deposition solution, the amo...

Embodiment 3

[0039] 1. Preparation of activated tungsten powder

[0040] The tungsten powder with a particle size of less than 1 micron is placed in the activation solution for ultrasonic activation for 35 minutes, the ultrasonic frequency is 40KHz, and the power is 300-400W. After the activation is completed, it is washed three times with deionized water and dried at 190 ° C for 2 hours to obtain activated tungsten powder. ;

[0041]The activation solution is an aqueous solution of hydrofluoric acid, ammonium fluoride and nitric acid, and the concentration of hydrofluoric acid in the activation solution is 50 ml / L, calculated as a hydrofluoric acid solution with a mass concentration of 40%; the concentration of ammonium fluoride is 10g / L; the concentration of nitric acid is 50ml / L, calculated as a nitric acid solution with a mass concentration of 65%;

[0042] 2. Preparation of composite powder

[0043] The activated tungsten powder was added to the chemical deposition solution, the amo...

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Abstract

The invention discloses a preparation method of La-doped W-Cu composite powder, which comprises the preparation of activated tungsten powder and the preparation of composite powder, wherein the preparation of the activated tungsten powder comprises the following steps: carrying out ultrasonic activation on tungsten powder in an activation liquid for 30-40 minutes, washing with de-ionized water after the activation is completed, and drying to obtain the activated tungsten powder. The preparation of the composite powder comprises the following steps: adding the activated tungsten powder into a chemical deposition solution, wherein the dosage of the tungsten powder is 30-50g / L; regulating with sodium hydroxide until the pH value is 12.0-13.0; carrying out ultrasonic deposition and coating at normal temperature for 40-80 minutes; and standing for 2-3 hours, filtering, washing, and drying to obtain the composite powder. The obtained powder has high component homogenizing degree, avoids the tungsten and copper oxide reduction process of the conventional preparation method, and has the advantages of simple treatment process and low preparation cost. Besides, the invention greatly improves the flowability of the composite powder in the sintering process, and carries out direct sintering at low temperature; and the relative density of sintering samples can be up to 98.7% or above.

Description

1. Technical field [0001] The invention relates to the field of powder material preparation, in particular to a preparation method of La-doped W-Cu composite powder. 2. Background technology [0002] Powder metallurgy W-Cu composite material has good physical and mechanical properties, strong ablation resistance, thermal shock resistance, and excellent thermal control and microwave absorption properties, etc. Machining and other fields have been widely used and occupy an important position in the national economy. Therefore, tungsten-based alloys have always been highly valued by countries around the world and have become one of the more active research fields in the material science community. In these applications, higher densification levels of W-Cu materials are often required to improve their performance levels. As far as the current main research directions are concerned, ultrafine / nanostructured and gradient-structured functional materials are the main research direc...

Claims

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Application Information

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Patent Type & Authority Patents(China)
IPC IPC(8): B22F1/02C23C18/48
Inventor 罗来马吴玉程程继贵
Owner HEFEI UNIV OF TECH