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Lignosulfonate alkylation modified surfactant and preparation method and application thereof

A technology of sulfonate alkyl and lignosulfonate, which is applied in the direction of anionic surface active compounds, chemical instruments and methods, chemical/physical processes, etc., and can solve the problem of low surface activity of modified products and heterogeneous system reactions Poor effect and other problems, to achieve the effect of solving heterogeneous reaction, reducing process cost and equipment cost, and reducing cost

Active Publication Date: 2013-10-23
GUANGZHOU CHEM CO LTD CHINESE ACADEMY OF SCI +1
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

[0007] In order to overcome the shortcomings and deficiencies of the prior art, especially the Chinese patent CN 00130812.2 technology, the heterogeneous system reaction effect caused by the difference in lipophilic and hydrophilic properties of lignosulfonate and alkylating agent is not good, and the modified product The shortcoming of low surface activity, the primary purpose of the present invention is to provide a kind of preparation method of lignosulfonate alkylation modified surfactant

Method used

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Examples

Experimental program
Comparison scheme
Effect test

Embodiment 1

[0032] (1) 10g sodium lignosulfonate is dissolved in 100ml mixed solution (obtained by isopropanol and water by volume ratio 1: 4), then the pH value is adjusted to 10 with mass volume ratio 10% sodium hydroxide solution, stir Fully dissolve sodium lignosulfonate.

[0033] (2) Add 3 g of chlorinated paraffin containing 14-17 carbon atoms (chlorinated paraffin 52, the average number of carbon atoms is 14-17) and 1.0 ml of pyridine (concentration ≥ 99.5%) as a catalyst. Under the protection of nitrogen, the temperature was raised to 60° C., condensed and refluxed for 6 h, and then cooled naturally. The pH of the reaction solution was adjusted with hydrochloric acid until precipitation appeared. After the precipitation was complete, it was filtered, washed, and dried to obtain a dark brown solid. According to GB / T 22237-2008, the surface tension of the product aqueous solution with a mass concentration of 1% measured by the platinum plate method at room temperature is 29.229mN / m...

Embodiment 2

[0035] (1) 10g sodium lignosulfonate is dissolved in 100ml mixed solution (obtained by isopropanol and water by volume ratio 1: 1), then the pH value is adjusted to 12 with mass volume ratio 10% sodium hydroxide solution, stir Fully dissolve sodium lignosulfonate.

[0036] (2) Add 8g of chlorinated paraffin (chlorinated paraffin 52, the average number of carbon atoms is 14-17) and 2.7ml pyridine (concentration ≥ 99.5%) containing 14-17 carbon atoms as a catalyst, under the protection of nitrogen Then, the temperature was raised to 70°C to condense and reflux for 4 hours, and then cooled naturally. The pH of the reaction solution was adjusted with hydrochloric acid until precipitation appeared. After the precipitation was complete, it was filtered, washed, and dried to obtain a dark brown solid. According to GB / T 22237-2008, the surface tension of the product aqueous solution with a mass concentration of 1% measured by the platinum plate method at room temperature is 29.385mN / ...

Embodiment 3

[0038] (1) Dissolve 10g sodium lignosulfonate in 100ml mixed solution (obtained by isopropanol and water in a volume ratio of 3:7), then adjust the pH value to 11 with mass volume ratio 10% sodium hydroxide solution, stir Fully dissolve sodium lignosulfonate.

[0039] (2) Add 2g of chlorinated paraffin containing 14-17 carbon atoms (chlorinated paraffin 52, the average number of carbon atoms is 14-17) and 0.65ml (concentration ≥ 99.5%) pyridine as a catalyst, under the protection of nitrogen Then, the temperature was raised to 50°C to condense and reflux for 5 hours, and then cooled naturally. The pH of the reaction solution was adjusted with hydrochloric acid until precipitation appeared. After the precipitation was complete, it was filtered, washed, and dried to obtain a dark brown solid. The pH of the reaction solution was adjusted with hydrochloric acid until precipitation appeared. After the precipitation was complete, it was filtered, washed, and dried to obtain a dark ...

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Abstract

The invention discloses a lignosulfonate alkylation modified surfactant and a preparation method and application thereof. The method comprises the following steps of: dissolving lignosulfonate in a mixed solution of an organic solvent and water, regulating the pH value of the solution to 10 to 12, and stirring to ensure that the lignosulfonate is dissolved fully; and adding halogenated hydrocarbon and an alkaline organic amine catalyst, performing reflux reaction under the protection of inert gas, cooling, performing acid precipitation on a reaction solution, washing and drying to obtain the lignosulfonate alkylation modified surfactant. According to the lignosulfonate alkylation modified surfactant, the alkaline organic amine catalyst is used, and the mixed solution of the organic solvent and the water is used as a reaction solvent, so that the problems of a non-ideal effect of heterogeneous reaction and low activity of modified products, which are caused by difference of the oleophylic and hydrophilic performance of the lignosulfonate and an alkylation reagent, are solved, and the obtained lignosulfonate alkylation modified surfactant of which the surface tension is 29.299mN / m meets the activity requirement of daily washing. According to the method, one-step reaction is adopted, and the yield is 91 percent, so the method is good in industrial prospect.

Description

technical field [0001] The invention belongs to the field of surfactant preparation, in particular to a lignin sulfonate alkylation modified surfactant and its preparation method and application. Background technique [0002] Industrial lignosulfonate is a by-product of the acidic paper industry. Direct discharge not only wastes resources, but also causes great pollution to the environment. In recent years, due to the sharp fluctuations in oil prices and unsustainable oil resources, the production of traditional petroleum-based surfactants is facing enormous cost pressure. Lignosulfonate is a derivative of lignin, the second most abundant biomass resource in nature. Lignosulfonate has certain surface activity because it contains hydrophilic groups such as sulfonic acid groups and C3-C6 hydrophobic skeleton and aromatic ring. Through certain molecular design and structural modification, it is expected to prepare a new generation of new environmentally friendly Biodegradable...

Claims

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Application Information

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Patent Type & Authority Patents(China)
IPC IPC(8): B01F17/50C09K8/584C11D1/30C09K23/50
Inventor 沈敏敏周宝文哈成勇莫建强岑学杨胡志忠
Owner GUANGZHOU CHEM CO LTD CHINESE ACADEMY OF SCI