Method for determining waster water COD by simulating sunlight photoelectrocatalysis
A photoelectric catalysis and sunlight technology, which is applied in the fields of electrochemical variables of materials, measurement devices, and material analysis by electromagnetic means, to achieve the effects of rapid measurement, simple preparation, and large free space.
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Embodiment 1
[0021] An electrode for measuring wastewater COD by simulating sunlight photoelectric catalysis, the electrode is based on a titanium plate, and an upright and orderly TiO is constructed by anodization 2 -NTs, in TiO 2 -There is a urea solution with a mass fraction of 5% in the pores of NTs, and the titanium plate is carbonized at a high temperature to obtain C-N / TiO 2 -NTs.
[0022] The preparation method of an electrode for measuring wastewater COD by simulating sunlight photoelectric catalysis comprises the following steps:
[0023] (1) Upright ordered TiO on Ti-based surface 2 -Growth and reduction of NTs
[0024] Construction of upright and ordered TiO on the surface of titanium plate by anodic oxidation method 2 -NTs, then 1mol L -1 NH 4 The Cl solution is the electrolyte, the temperature is controlled at 25°C, and the TiO 2 -NTs restore 3s;
[0025] (2) C-N / TiO 2 - Preparation of NTs electrode
[0026] Loading of urea solution into TiO by vacuum load impregnat...
Embodiment 2
[0032] The practicability of this method was investigated with actual water samples obtained from food factories, urban domestic sewage, river water and hospital sewage. In order to minimize the influence of the matrix (such as pH value), the experiment adopts the standard addition method to simulate the solar photocatalytic oxidation to detect the COD value of the actual sample. The procedure is as follows: (a) use C-N / TiO2-NTs electrode in 90ml 0.1mol L -1 Na 2 SO 4 Measured in electrolyte solution i blank ; (b) at 0.1M Na 2 SO 4 Add 10ml of the actual sample solution to the electrolyte solution, mix well and measure i total , and calculate i net , if i net If it exceeds the linear range, first use 0.1M Na 2 SO 4 The electrolyte solution is diluted to within the detection range; (c) 500 μl of a mixed organic solution with a theoretical COD value of 2000 ppm is added to the diluted actual sample solution after the (b) step, and a COD value increased by 10 ppm is mea...
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