Photosensitive composition, photosensitive film, photosensitive laminate, method for forming permanent pattern, and printed board
A photosensitive composition and photosensitivity technology, which is applied in the fields of printed circuit, printed circuit, printed circuit manufacturing, etc., can solve the compromise of flame retardancy and folding resistance, and has not developed a combination of flame retardancy and folding resistance photosensitivity and other problems, to achieve the effect of excellent folding resistance and flame retardancy
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Embodiment 1
[0345] -Synthesis of photosensitive polyurethane resin U1-
[0346] In a 500 mL three-neck round bottom flask equipped with a condenser and a stirrer, 10.22g (0.069mol) 2,2-bis(hydroxymethyl)butyric acid (DMBA), 12.97g (0.081mol) monomethacrylic acid Glycerides (GLM) and 4.80 g (0.004 mol) polypropylene glycol (molecular weight: 1,200) (PPG 1,200) were dissolved in 79 mL of propylene glycol monomethyl ether monoacetate. To this solution, 37.54g (0.15mol) 4,4-diphenylmethane diisocyanate (MDI), 0.1g 2,6-di-tert-butylhydroxytoluene and 0.2g NEOSTAN U-600 (from Nitto Kasei Co. Ltd.), and the mixture was stirred at 75°C for 5 hours. Thereafter, the solution was diluted with 9.61 mL of methanol and the resulting diluted solution was stirred for 30 minutes to obtain 145 g of a photosensitive polyurethane resin U1 solution (solid content: 45% by mass).
[0347] The obtained photosensitive polyurethane resin U1 had an acid value of 65 mgKOH / g, as measured by gel permeation chromatography...
Embodiment 2
[0352] -Synthesis of photosensitive polyurethane resin U2 (when the diisocyanate compound does not contain aromatic compounds)-
[0353] A photosensitive polyurethane resin U2 solution (solid content: 45% by mass) was prepared in the same manner as in Synthesis Example 1, except that 37.54 g (0.15 mol) of 4,4-diphenylmethane diisocyanate (MDI) Change to 30.03g (0.12mol) isophorone diisocyanate (IPDI).
Embodiment 3
[0355] -Synthesis of photosensitive polyurethane resin U3 (when the polymer polyol compound has a mass average molecular weight less than 400)-
[0356] A photosensitive polyurethane resin U3 solution (solid content: 45% by mass) was prepared in the same manner as in Synthesis Example 1, except that 4.80 g (0.004 mol) of polypropylene glycol (mass average molecular weight: 1,200) (PPG1200) was changed It is 1.20g (0.004mol) polypropylene glycol (mass average molecular weight: 300) (PPG300).
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