Alumina microsphere air purifying agent, preparation method and application of air purifying agent
An air purifier, alumina technology, applied in the field of air purification, can solve the problems of cumbersome and delicate operation and modification process, inability to realize industrialization, marketization, poor stability, etc., and achieve stable photocatalytic activity and excellent photocatalysis performance, the effect of good performance stability
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[0048] Preparation of alumina microspheres
[0049] The cleaned aluminum balls were annealed in a vacuum furnace at 600°C for 2h to eliminate the mechanical stress therein. Then, adopt the mixed acid solution of 5wt% phosphoric acid and 0.4mol / L oxalic acid (volume ratio 1: 1) to form as electrolytic solution, with aluminum ball as anode, stainless steel plate as cathode, 90V DC voltage anodic primary oxidation 5h under 5 ℃, then Take it out, put it into a solution of phosphochromic acid (a mixed solution containing 10wt% of phosphoric acid and 3wt% of chromic acid) to wash away the irregular holes generated by the primary oxidation. Then, under the same conditions, it was anodized twice for 20 hours to obtain porous alumina microspheres with regular pores, the diameter of which was 80nm.
[0050] By changing the oxidation conditions, alumina microspheres with a wide range of pore diameters such as 40-250nm can be obtained.
Embodiment 1
[0052] (1). Add 0.3mol analytically pure TiCl 4 Add dropwise deionized water to prepare a transparent aqueous solution with a mass concentration of 35%, and then add an aqueous sodium carbonate solution with a mass concentration of 40% to obtain TiO 2 Precipitate, this precipitate carries out high-speed shear (5000rpm / min) in dehydrated alcohol, and shearing time is 50 minutes, obtains stable suspension, TiO 2 The particle size is 20nm;
[0053] (2). Add 0.1mol silver sulfate to the solution of step (1), and use ultrasonic vibration to make it completely mixed until a uniform and transparent sol is formed;
[0054] (3). Immerse 0.3mol alumina microspheres with a channel diameter of 80nm in the sol of step (2), and perform ultrasonic oscillation for 30 minutes, and then dry naturally;
[0055] (4). Calcining the dried alumina microspheres in step (3) in a muffle furnace, first calcining at 250°C for 1.5 hours, and then increasing the temperature at a heating rate of 150°C / h t...
Embodiment 2
[0058] Except that the aperture of alumina microspheres is 100nm, this embodiment is implemented in the same manner as in Example 1, and the nano-TiO of final alumina microsphere air purifier material 2 The ratio of particle diameter to alumina microsphere diameter is 1:5.
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