A kind of cross-linkable quaternary ammonium salt water-soluble cationic monomer and its preparation method and application
A technology of water-soluble cationic and quaternary ammonium salts, applied in the field of cationic monomers, can solve the problems of low cationization degree and inability to achieve performance of polymers, and achieve the effects of high cationic degree, large molecular weight, and improved performance.
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Embodiment 1
[0034] 1. Preparation of cross-linkable water-soluble cationic monomer
[0035] Add 2.0mol of epichlorohydrin and 10ml of water to a four-neck flask equipped with a condensing reflux tube, a thermometer, a dropping funnel and a stirrer, raise the temperature to 30°C, and add 33% dimethylamine dropwise at 30°C 1.0 mol (calculated as the number of moles of dimethylamine), after dripping, keep warm at 30°C for 10 hours, then distill under reduced pressure to remove unreacted monomer and water. Cool down to below 20°C, add 42.9g of 33% glacial acetic acid aqueous solution to adjust the pH value of the material to 4-5, slowly add 2.0mol of dimethylallylamine dropwise and control the system temperature to 30°C, after the dripping is completed, set the temperature at 30°C Insulated reaction for 10 h, vacuum distillation to remove unreacted monomer and water to obtain the desired cross-linkable water-soluble cationic monomer.
[0036] 2. Polymerization reaction
[0037] Add 100 g of...
Embodiment 2
[0039] 1. Preparation of cross-linkable water-soluble cationic monomer
[0040] Add 2.8mol of epibromopropane and 10ml of water into a four-neck flask equipped with a condensing reflux tube, a thermometer, a dropping funnel and a stirrer, raise the temperature to 30°C, and add 50% methylpropane dropwise at 30°C 1.0 mol of methyl propyl amine (calculated as the number of moles of methyl propyl amine), after dropping, keep it warm at 30°C for 10 hours, then distill under reduced pressure to remove unreacted monomer and water. Cool down to below 20°C, add 26.9g of 36.5% hydrochloric acid aqueous solution to adjust the pH value of the material to 4~5, slowly add 3.0mol of methpropylallylamine and control the system temperature to 30°C Insulated reaction for 10 h, vacuum distillation to remove unreacted monomer and water to obtain the desired cross-linkable water-soluble cationic monomer.
[0041] 2. Polymerization reaction
[0042] Add 100 g of the synthesized cross-linkable wat...
Embodiment 3
[0044] 1. Preparation of cross-linkable water-soluble cationic monomer
[0045] Add 2.0mol of epibromopropane and 10ml of water to a four-neck flask equipped with a condensing reflux tube, a thermometer, a dropping funnel and a stirrer, raise the temperature to 30°C, and add 33% dimethylamine dropwise at 30°C 1.0 mol (calculated as the number of moles of dimethylamine), after dripping, keep warm at 30°C for 10 hours, then distill under reduced pressure to remove unreacted monomer and water. Cool down to below 20°C, add 38.8g of 33% glacial acetic acid aqueous solution to adjust the pH value of the material to 4-5, slowly add 2.0mol of dimethylallylamine dropwise and control the system temperature to 30°C, after the dripping is completed, set the temperature at 30°C Insulated reaction for 10 h, vacuum distillation to remove unreacted monomer and water to obtain the desired cross-linkable water-soluble cationic monomer.
[0046] 2. Polymerization reaction
[0047] Add 100 g of...
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