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Magnesium-loaded biological composite material as well as preparation method and application method thereof

A composite material and biological technology, applied in chemical instruments and methods, other chemical processes, adsorbed water/sewage treatment, etc., can solve the problem that slow-release fertilizers cannot be used, achieve good adsorption effect, low production cost, and avoid mass transfer. blocking effect

Active Publication Date: 2015-06-03
YANSHAN UNIV
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

Although the immobilized zirconia biocomposite has a good removal effect on phosphorus, it cannot be used for slow-release fertilizers

Method used

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Examples

Experimental program
Comparison scheme
Effect test

Embodiment 1

[0017] Weigh magnesium nitrate to prepare an aqueous solution with a mass fraction of 5%. Add artemia eggshells that have been ultrasonically cleaned and dried for 4 hours in advance to 100mL of the above aqueous solution. Ultrasonic at 15°C, ultrasonic frequency 60Hz, and ultrasonic power 50W Disperse for 4 hours, stir magnetically at room temperature for 10 hours, so that all Artemia egg shells sink to the bottom of the beaker, evaporate the solution to dryness in a water bath at 40°C, add it to 400 mL of 0.4% NaOH solution, and stir magnetically. Filter, wash with deionized water until neutral, and dry to obtain the magnesium-loaded biocomposite material.

[0018] 500mL of KH with a concentration of 5mg / L 2 PO 4 Put it into a Erlenmeyer flask, add 1 g of the above-mentioned magnesium-loaded biocomposite material, adjust the pH value of the solution to 7 with NaOH and HCl, shake at a constant temperature at room temperature (25° C.), and rotate at 120 rpm. After 24 hours, ...

Embodiment 2

[0021] Weigh magnesium nitrate to prepare an aqueous solution, the mass percentage of which is 20%. Add artemia eggshells that have been ultrasonicated for 4 hours and washed and dried in advance to 100mL of the above aqueous solution. Ultrasonic at 20°C, ultrasonic frequency 60Hz, and ultrasonic power Disperse for 6 hours, stir magnetically at room temperature for 16 hours, and make Artemia egg shells sink to the bottom of the beaker. The solution is evaporated to dryness in a water bath at 60°C, added to 400 mL of 1% NaOH solution, and stirred magnetically. Filter, wash with deionized water until neutral, and dry to obtain the magnesium-loaded biocomposite material.

[0022] 500mL of KH with a concentration of 10mg / L 2 PO 4 Put it into a Erlenmeyer flask, add 2g of the above-mentioned magnesium-loaded biocomposite material, adjust the pH value of the solution to 7 with NaOH and HCl, shake at a constant temperature at room temperature (25° C.), and rotate at a speed of 160 r...

Embodiment 3

[0025] Weigh magnesium nitrate to prepare an aqueous solution with a mass fraction of 40%. Add artemia eggshells that have been ultrasonicated for 4 hours and washed and dried in advance to 100mL of the above aqueous solution. Ultrasonic at 15°C, ultrasonic frequency 60Hz, and ultrasonic power 50W Disperse for 4 hours, and stir magnetically at room temperature for 12 hours to make Artemia eggshells sink to the bottom of the beaker. The solution is evaporated to dryness in a water bath at 40°C, and added to 400 mL of 4% NaOH solution, and stirred magnetically. Filter, wash with deionized water until neutral, and dry to obtain the magnesium-loaded biocomposite material.

[0026] 500mL of KH with a concentration of 30mg / L 2 PO 4 Put it into a Erlenmeyer flask, add 3g of the above-mentioned magnesium-loaded biocomposite material, adjust the pH value of the solution to 7 with NaOH and HCl, shake at a constant temperature at room temperature (25° C.), and rotate at a speed of 180 r...

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Abstract

The invention discloses a magnesium-loaded biological composite material. The magnesium-loaded biological composite material is prepared from magnesium nitrate, sodium hydroxide and eggshell of artemia cysts; a preparation method of the magnesium-loaded biological composite material comprises the following steps: preparing the magnesium nitrate into a water solution; adding 2g to 8g of the eggshell of artemia cysts into every 100ml of the water solution; ultrasonically dispersing for 2 to 8 hours; magnetically stirring for 10 to 20 hours; evaporating the solution to be dry in a water bath at the temperature of 40 to 80 DEG C; adding into a NaOH solution; magnetically stirring for 8 to 12 hours; filtering; washing by using deionized water until the solution is neutral; and drying to obtain the magnesium-loaded biological composite material. When the magnesium-loaded biological composite material is used for removing phosphorus wastewater of which the concentration is 5mg / L to 30mg / L, the removal rate is 45% to 80%, so that the magnesium-loaded biological composite material is a quite good adsorbent; after the phosphorus is adsorbed, the magnesium-loaded biological composite material is a bio-degradable phosphorus controlled release fertilizer. The magnesium-loaded biological composite material disclosed by the invention is easy to control in production process and relatively low in production cost; the prepared magnesium-loaded biological composite material has a good adsorption effect on the phosphorus, and the phosphorus-gathered magnesium-loaded biological composite material can be used as the degradable controlled release fertilizer.

Description

technical field [0001] The invention relates to a biocomposite material and methods for its preparation and use. Background technique [0002] Metal oxides are a kind of artificially synthesized high-efficiency adsorbents, which are widely used in the adsorption of phosphorus-containing wastewater. However, due to the influence of the structure, the traditional nanometer metal oxide phosphorus removal adsorbent has the technical shortcomings of particle agglomeration in the pores and poor adsorption and mass transfer rate, resulting in low utilization rate of the adsorbent. Therefore, there are more and more studies on the preparation of new adsorption materials by using adsorption resins to immobilize nanometer metal oxides. Although this new type of adsorption material has a good adsorption effect, the resin cannot be biodegraded, and the regeneration of the adsorbent requires the consumption of chemical reagents, the regeneration cost is high, and the phosphorus adsorbed...

Claims

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Application Information

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Patent Type & Authority Applications(China)
IPC IPC(8): B01J20/22B01J20/30C02F1/28
Inventor 王素凤马梦璇
Owner YANSHAN UNIV