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A method for producing lubricating oil base oil

A technology for lubricating base oil and hydrocracking tail oil, which is applied in the directions of lubricating compositions, chemical instruments and methods, petroleum industry, etc. The effect of skeleton silicon-alumina structure uniformity, maintaining uniformity, high catalytic activity and isomerization ability

Active Publication Date: 2016-10-19
CHINA PETROLEUM & CHEM CORP +1
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

[0003] At present, the cracking components used in hydrocracking catalysts are mostly Y-type molecular sieves and β molecular sieves, and the hydrogenation tail oil produced by catalysts with Y-type molecular sieves as cracking components has disadvantages such as high pour point, such as the hydrocracking When the tail oil is used to prepare lubricating oil base oil, multiple steps such as noble metal isomerization dewaxing and supplementary refining are required for post-treatment, which greatly reduces the yield of base oil and increases the production cost

Method used

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Experimental program
Comparison scheme
Effect test

preparation example Construction

[0031] The preparation method of the used b molecular sieve of hydrocracking catalyst carrier of the present invention specifically comprises the steps:

[0032] (1) Treat the raw powder of β molecular sieve under normal pressure and dynamic steam conditions, the treatment temperature is 500~650℃, and the treatment time is 5~10 hours;

[0033] The present invention adopts the raw powder of beta molecular sieve synthesized by conventional hydrothermal method. The chemical SiO of the used molecular sieve powder 2 / Al 2 o 3 Molar ratio 22.5~28.5, Na 2 The O content is 1.0wt%~3.0wt%, and the relative crystallinity is above 95%;

[0034] The hydrothermal treatment condition adopted in the present invention is to use 100wt% water vapor, and the water vapor passes through the molecular sieve at 50-100L / h per kilogram of β molecular sieve. In order to make the molecular sieve treatment more uniform, it is best to place the molecular sieve in a rotating container, and the water va...

Embodiment 1

[0045] Take the original powder of β molecular sieve (provided by Sinopec Catalyst Fushun Branch), its chemical SiO 2 / Al 2 o 3 The molar ratio is 25.5, the relative crystallinity is 96%, Na 2 O content is 2.45wt%, in its skeleton structure, through 29Si MAS NMR spectrum, the distribution of silicon atoms in different coordination states is obtained as follows: Si (4Al) is 7.6%, Si (3Al) is 30.6%, Si (2Al) is 32.3%, Si (1Al) is 21.0% %, Si (0Al) is 8.5%. Take 1000g of the above-mentioned molecular sieve, put it into a tube furnace, adopt the method of temperature program (heating rate: 100°C / hour), and start to introduce 100wt% water vapor when the temperature of the tube furnace rises to 300°C, the flow rate of water vapor is 50L / hour, the tube furnace is heated to 550°C, and the constant temperature time is 6 hours. The obtained molecular sieve is coded as BS-1, and its properties are shown in Table 1.

Embodiment 2

[0047] Get the former powder of β molecular sieve with embodiment 1. Take 1000g of the above-mentioned molecular sieve, put it into a tube furnace, adopt the method of temperature program (heating rate: 100°C / hour), and start to introduce 100wt% water vapor when the temperature of the tube furnace rises to 300°C, the flow rate of water vapor is 70L / hour, the tube furnace is heated to 600°C, and the constant temperature time is 8 hours. The obtained molecular sieve is coded as BS-2, and its properties are shown in Table 1.

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Abstract

The invention discloses a method for producing lubricating oil base oil. The method is to combine the hydrocracking process and supplementary refining process to produce lubricating oil base oil. In the hydrocracking process, a hydrocracking catalyst containing β molecular sieve is used. The β molecular sieve has a uniform skeleton silicon-alumina structure, suitable acidity, Reasonable pore structure and other characteristics, so that the obtained hydrocracking tail oil can obtain lubricating oil base oil products with lower pour point and better stability through conventional supplementary refining process.

Description

technical field [0001] The invention relates to a method for producing lubricating oil base oil, in particular to a method for producing lubricating oil base oil by combining hydrocracking and hydrofining processes. Background technique [0002] Hydrocracking is one of the most important heavy oil processing methods in today's oil refining industry. The main products produced after hydrocracking of raw materials are gas, gasoline, diesel, jet fuel and high-quality hydrocracking tail oil and other products. The advantages of low content. [0003] At present, the cracking components used in hydrocracking catalysts are mostly Y-type molecular sieves and β molecular sieves, and the hydrogenation tail oil produced by catalysts with Y-type molecular sieves as cracking components has disadvantages such as high pour point, such as the hydrocracking When the tail oil is used to prepare lubricating oil base oil, multiple steps such as noble metal isomerization dewaxing and supplemen...

Claims

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Application Information

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Patent Type & Authority Patents(China)
IPC IPC(8): C10G65/12C10M177/00B01J29/78
Inventor 刘昶王凤来杜艳泽赵红王珂琦关明华
Owner CHINA PETROLEUM & CHEM CORP