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Porous polyimide/electrospinning polyimide fibrous composite material and application thereof

A polyimide fiber, polyimide technology, applied in the direction of fiber type, fiber processing, textile and papermaking, etc., to achieve the effect of improving capture and good application prospects

Active Publication Date: 2015-09-23
CHINA UNIV OF GEOSCIENCES (WUHAN)
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

However, there is no relevant report on the combination of polyimide porous materials and electrospun fiber materials in this field

Method used

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Examples

Experimental program
Comparison scheme
Effect test

Embodiment 1

[0022] In an ice-water bath at 0°C, add 4,4′-diaminodiphenyl ether and N,N′-dimethylformamide into the three-necked flask. After dissolving, add pyromellitic dianhydride in three times, two The reaction was stopped within 1 hour, and the solid content of the polyamic acid obtained was 20 wt%. Then add in DMF, under the condition of 0 ℃, dilute the original solution to a solid content of 12wt%, and carry out electrospinning with the obtained solution. Aluminum foil collectors collect the nanofibers. The distance from the spinneret to the collector is 15cm, and the injection rate is 0.25mL / h. Put the spun fiber membrane in an oven for half an hour to dry at 60, 100, 150, 200, 250, and 300°C for imidization, and set aside; add melamine and dimethyl sulfoxide to a three-necked flask respectively, and then Add pyromellitic dianhydride, after dissolving, heat up to 180°C in a nitrogen atmosphere for high-temperature polycondensation, react for 24 hours, stop heating until cooling,...

Embodiment 2

[0024] In an ice-water bath at 0°C, add 4,4′-diaminodiphenyl ether and N,N′-dimethylformamide into the three-necked flask. After dissolving, add pyromellitic dianhydride in three times, two The reaction was stopped within 1 hour, and the solid content of the obtained polyamic acid was 20 wt%. Then add in DMF, under the condition of 0 ℃, dilute the original solution to a solid content of 12wt%, and carry out electrospinning with the obtained solution. Aluminum foil collectors collect the nanofibers. The distance from the spinneret to the collector is 15cm, and the injection rate is 0.25mL / h. Put the spun fiber membrane in an oven for half an hour to dry at 60, 100, 150, 200, 250, and 300°C for imidization, and set aside; add melamine and dimethyl sulfoxide to a three-necked flask respectively, and then Add pyromellitic dianhydride, after dissolving, heat up to 180°C in a nitrogen atmosphere for high-temperature polycondensation, react for 24 hours, stop heating until cooling,...

Embodiment 3

[0026] In an ice-water bath at 0°C, add 4,4′-diaminodiphenyl ether and N,N′-dimethylformamide into the three-necked flask. After dissolving, add pyromellitic dianhydride in three times, two The reaction was stopped within 1 hour, and the solid content of the obtained polyamic acid was 20 wt%. Then add in DMF, under the condition of 0 ℃, dilute the original solution to a solid content of 12wt%, and carry out electrospinning with the obtained solution. Aluminum foil collectors collect the nanofibers. The distance from the spinneret to the collector is 15cm, and the injection rate is 0.25mL / h. Put the spun fiber membrane in an oven for half an hour to dry at 60, 100, 150, 200, 250, and 300°C for imidization, and set aside; add melamine and dimethyl sulfoxide to a three-necked flask respectively, and then Add pyromellitic dianhydride, after dissolving, heat up to 180°C in a nitrogen atmosphere for high-temperature polycondensation, react for 24 hours, stop heating until cooling,...

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PUM

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Abstract

The invention provides a porous polyimide / electrospinning polyimide fibrous composite material. Firstly, under the condition of ice-water bath, 4,4'-diaminodiphenyl ether and N,N'-dimethylformamide are added into a container, after a monomer is dissolved, pyromellitic dianhydride is added, a polyimide solution is obtained after the reaction is completed, then electrostatic spinning is conducted, and a polyimide fiber is prepared; then imidization processing is conducted, and an electrospinning linear polyimide fiber is prepared; a melamine monomer, dimethyl sulfoxide and an anhydride monomer are added in another container and are heated for a polymerization reaction under the nitrogen atmosphere, and a porous polyimide solution is prepared; the electrospinning linear polyimide fiber is soaked in the porous polyimide solution, vacuum drying is conducted after ultrasonic oscillation processing, and the porous polyimide / electrospinning polyimide fibrous composite material is obtained. The prepared porous polyimide / electrospinning polyimide fibrous composite material can be used for absorbing organic pollutants in water.

Description

technical field [0001] The invention provides a novel composite material in which porous polyimide is loaded on the surface of linear polyimide electrospun fibers, is a material used for absorbing and removing organic pollutants in water bodies, and belongs to the technical field of polymer materials. Background technique [0002] Water quality problems have seriously threatened the survival and development of human beings. For example, organic pollutants from leather, paper, printing, plastics and other industries are directly or indirectly discharged into the environment, seriously affecting the quality of water bodies. Some organic dyes are toxic. Even cause cancer; antibiotics have played an important role in the development of animal husbandry, but as people gradually deepen their understanding of antibiotics, their use in animal and food production has been widely questioned. Tetracycline is a common antibiotic that enters the human body through the food chain. It has ...

Claims

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Application Information

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Patent Type & Authority Applications(China)
IPC IPC(8): D06M15/59C08G73/10B01J20/26B01J20/30C02F1/28C02F1/58D06M101/30
Inventor 廖桂英王燕夏华王东升
Owner CHINA UNIV OF GEOSCIENCES (WUHAN)