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Quantum dot composite microsphere with two-component shell and preparation method thereof

A technology of composite microspheres and quantum dots, applied in the field of quantum dots, can solve the problems of inability to prepare temperature-sensitive quantum dots, and achieve high luminous efficiency

Inactive Publication Date: 2017-11-24
谢永芳
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

Therefore, the existing technology cannot prepare quantum dots with very high temperature sensitivity

Method used

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Examples

Experimental program
Comparison scheme
Effect test

Embodiment 1

[0031] (1) mixing myristic acid, styrene and ethyl orthosilicate with a phase transition temperature of 52 to 54° C. in a mass ratio of 6:9:1 to obtain a mixture;

[0032] Add the above mixture into a 500mL round-bottomed flask, stir with sheet stainless steel, heat in a water bath to 60°C at a stirring speed of 1500 rpm, add 1g of sodium dodecylbenzenesulfonate into 100mL of water, and disperse homogeneous, and added to a round-bottomed flask for emulsification for 20 minutes, then heated up to 80°C, and continued to emulsify for 10 minutes at a stirring speed of 1500 rpm to obtain a uniform microemulsion, wherein the sodium dodecylbenzenesulfonate The ratio of mass to the mass sum of myristic acid, styrene and ethyl orthosilicate is 1:13;

[0033] After the emulsification was completed, the temperature of the water bath was adjusted to 85°C. Dissolve 1 g of ammonium persulfate in 7.5 mL of deionized water, and slowly add it dropwise to the round bottom flask until complete....

Embodiment 2

[0044] (1) mixing palmitic acid, styrene and ethyl orthosilicate with a phase transition temperature of 62 to 63° C. in a mass ratio of 10:15:4 to obtain a mixture;

[0045] Add the above mixture into a 500mL round-bottomed flask, stir with sheet stainless steel, heat in a water bath to 70°C at a stirring speed of 1500 rpm, add 1g of sodium dodecylbenzenesulfonate to 100mL of deionized Disperse evenly in water, add it to a round bottom flask for emulsification for 10 minutes, then raise the temperature to 80°C, and continue to emulsify for 20 minutes at a stirring speed of 1500 rpm to obtain a uniform milky white microemulsion. Among them, sodium tetradecyl sulfate The ratio of the quality of palmitic acid, styrene and ethyl orthosilicate to the sum of the quality is 1:25;

[0046] After the emulsification was completed, the temperature of the water bath was adjusted to 85°C. Dissolve 1 g of ammonium persulfate in 7.5 mL of deionized water, and slowly add it dropwise to the r...

Embodiment 3

[0056] (1) Mixing lauric acid, styrene and ethyl orthosilicate with a phase transition temperature of 43 to 45° C. in a mass ratio of 8:12:2 to obtain a mixture;

[0057] Add the above mixture into a 500mL round-bottomed flask, stir with sheet stainless steel, heat to 60°C in a water bath at a stirring speed of 1500 rpm, add 1g of sodium lauryl sulfate to 42.5mL of deionized water Disperse evenly, add it to a round bottom flask for emulsification for 15 minutes, then raise the temperature to 80°C, and continue to emulsify for 15 minutes at a stirring speed of 1500 rpm to obtain a uniform milky white microemulsion, in which dodecylbenzenesulfonic acid The ratio of the quality of sodium to the sum of the quality of lauric acid, styrene and ethyl orthosilicate is 1:20;

[0058] After the emulsification was completed, the temperature of the water bath was adjusted to 85°C. Dissolve 1 g of initiator and catalyst ammonium persulfate in 7.5 mL of deionized water, and slowly add it d...

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Abstract

The invention discloses a quantum dot composite microsphere with a bi-component shell layer and a preparation method of the quantum dot composite microsphere. The quantum dot composite microsphere comprises a quantum dot and a microcapsule, wherein the quantum dot is self-assembled at the surface of the microcapsule, the microcapsule comprises a shell layer and a core, the shell layer contains polystyrene and silicon dioxide, and the core is higher aliphatic acid. According to the quantum dot composite microsphere provided by the invention, the quantum dot can keep the excellent characteristics of high light emitting efficiency and photochemical stability of a common quantum dot, and the light intensity has a specific temperature sensitive value, which can be used for associating with specific temperature. The quantum dot provided by the invention also has excellent reusability and cannot fall off.

Description

technical field [0001] The invention relates to a quantum dot, more specifically, to a quantum dot composite microsphere with a two-component shell and a preparation method thereof. Background technique [0002] When the size of the material is reduced to the nanometer level, due to its nano effect, the material will produce many novel and unique functional properties superior to traditional materials, and has a wide range of application values ​​in the fields of microelectronics, bioengineering, chemical engineering, and medicine. . [0003] In recent years, nano-luminescent materials with transition metals as active ions have been widely used in light-emitting devices, fluorescence imaging, solar cells, Fields such as fluorescence detection and biomarkers show broad application prospects. However, when quantum dots are used in light-emitting devices or fluorescence detection, in the range of 25-100°C, the red shifts of the quantum dot absorption peak wavelength and photo...

Claims

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Application Information

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Patent Type & Authority Patents(China)
IPC IPC(8): C09K11/88C09K11/02B01J13/04B01J13/16B01J13/22G01N21/64
CPCB01J13/043B01J13/16B01J13/22C09K11/025C09K11/88G01N21/6402
Inventor 谢永芳
Owner 谢永芳