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Method for preparing two-dimensional magnetic nanometer photocatalysts

A magnetic nanometer and photocatalyst technology, applied in chemical instruments and methods, physical/chemical process catalysts, chemical/physical processes, etc., can solve the problems of cumbersome process and low yield, and achieve no precious metal doping, low cost, The effect of increasing the photocatalytic activity

Active Publication Date: 2016-12-07
UNIV OF JINAN
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

[0005] At present, most of the synthesis methods are synthesized separately, and then compound the catalyst and the carrier, the process is cumbersome and the yield is not high

Method used

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Examples

Experimental program
Comparison scheme
Effect test

Embodiment 1

[0023] Example 1 Fe-TiO 2 / MoS 2 preparation of

[0024] (1) Add 0.6 g of molybdenum disulfide powder and 0.2 mmol of iron salt to 3 mL of n-butyllithium solution, and stir for 12 hours under nitrogen protection at 60 °C to obtain the reacted solution;

[0025] (2) Wash the reacted solution in step (1) with a non-polar solvent, and then perform ultrasonic treatment in a water bath at 60 °C. After the treatment, wash the treated solution with a non-polar solvent, and dry it in vacuum to obtain iron Intercalated molybdenum disulfide nanomaterials;

[0026] (3) Add 500 mg of the iron-intercalated molybdenum disulfide nanomaterials prepared in step (2) into 5 mL of tetrabutyl titanate, and after stirring for 1 hour, slowly add 0.5 mL of hydrofluoric acid while stirring, and then Reaction in the reactor at 160°C for 18 hours;

[0027] (4) The reaction product obtained in step (3) was centrifuged and washed three times with ultrapure water and absolute ethanol, and then vacuum-d...

Embodiment 2

[0032] Example 2 Fe-TiO 2 / MoS 2 preparation of

[0033] (1) Add 0.6 g of molybdenum disulfide powder and 1.0 mmol of iron salt to 5 mL of n-butyllithium solution, and stir for 24 hours under nitrogen protection at 30 °C to obtain the reacted solution;

[0034] (2) Wash the reacted solution in step (1) with a non-polar solvent, and then perform ultrasonic treatment in a water bath at 30 °C. After the treatment, wash the treated solution with a non-polar solvent, and dry it in vacuum to obtain iron Intercalated molybdenum disulfide nanomaterials;

[0035](3) Add 200 mg of the iron-intercalated molybdenum disulfide nanomaterials prepared in step (2) into 5 mL of tetrabutyl titanate, stir for 1 hour, slowly add 0.6 mL of hydrofluoric acid while stirring, and then Reaction in the reactor at 180°C for 20 hours;

[0036] (4) The reaction product obtained in step (3) was centrifuged and washed three times with ultrapure water and absolute ethanol, and then vacuum-dried at 50 °C t...

Embodiment 3

[0041] Example 3 Fe-TiO 2 / MoS 2 preparation of

[0042] (1) Add 0.6 g of molybdenum disulfide powder and 2.0 mmol of iron salt into 10 mL of n-butyllithium solution, and stir for 48 hours under nitrogen protection at 50 °C to obtain the reacted solution;

[0043] (2) Wash the reacted solution in step (1) with a non-polar solvent, and then perform ultrasonic treatment in a water bath at 50 °C. After the treatment, wash the treated solution with a non-polar solvent, and dry it in vacuum to obtain iron Intercalated molybdenum disulfide nanomaterials;

[0044] (3) Add 10 mg of the iron-intercalated molybdenum disulfide nanomaterials prepared in step (2) into 5 mL of tetrabutyl titanate, stir for 1 hour, then slowly add 0.8 mL of hydrofluoric acid while stirring, and then Reaction in the reactor at 200°C for 24 hours;

[0045] (4) The reaction product obtained in step (3) was centrifuged and washed three times with ultrapure water and absolute ethanol, and then vacuum-dried at...

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Abstract

The invention discloses a method for preparing two-dimensional magnetic nanometer photocatalysts, and belongs to the technical field of novel nanometer functional materials and green energy sources. The method includes compounding iron-doped titanium dioxide nanometer sheet materials on molybdenum disulfide nanometer sheets of iron intercalation layers in an in-situ manner; preparing two-dimensional nanometer composite materials Fe-TiO2 / MoS2 by the aid of one-pot processes. Iron-doped titanium dioxide nanometer squares are compounded with molybdenum disulfide in the two-dimensional nanometer composite materials in an in-situ manner. The method has the advantages that the two-dimensional magnetic nanometer photocatalysts are free of precious metal doping, low in cost, easy to prepare and high in photocatalytic activity; the two-dimensional composite materials Fe-TiO2 / MoS2 prepared by the aid of the method can be applied to the fields of photocatalytic water decomposition for hydrogen production, photocatalytic degradation of organic pollutants, preparation of solar photovoltaic cells and the like.

Description

technical field [0001] The invention relates to a method for preparing a magnetic nanometer photocatalyst. The prepared photocatalyst can be applied to the fields of photocatalytic water splitting to produce hydrogen, photocatalytic degradation of organic pollutants, preparation of solar photovoltaic cells and the like. The invention belongs to the technical field of novel nano functional materials and green energy. Background technique [0002] Photocatalyst is a substance that does not change itself under the irradiation of light, but can promote chemical reactions. For example, common chlorophyll is a typical photocatalyst, which can promote carbon dioxide and hydration in the air in the photosynthesis of plants. become oxygen and carbohydrates. The catalysis of photocatalysts is to convert light energy into energy required for chemical reactions under the irradiation of light that exists in nature. Photocatalysts can excite surrounding oxygen and water molecules into f...

Claims

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Application Information

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IPC IPC(8): B01J27/051
CPCB01J27/0515B01J35/396B01J35/33B01J35/39
Inventor 张勇郭继涛马洪敏吴丹杜斌
Owner UNIV OF JINAN