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Method for preparing high-temperature gas desulfurizer in iron oxide by microwave

A desulfurizer, medium-high temperature technology, applied in the direction of combustible gas purification, combustible gas purification/transformation, petroleum industry, etc., can solve the problems of reduced vulcanization activity, pulverization of the internal structure of the desulfurizer, etc., to achieve mass transfer rate increase, high mechanical The effect of strength and rich pore structure

Active Publication Date: 2017-03-15
西安润川环保科技有限公司
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

[0007] The purpose of the present invention is to provide a method for microwave preparation of high-temperature gas desulfurizer in iron oxide, so as to improve the utilization rate of sulfur capacity and mechanical strength of the desulfurizer, and to solve the problem of reducing the vulcanization activity of the iron oxide desulfurizer during the vulcanization-regeneration cycle and the pulverization of the internal structure of the desulfurizer

Method used

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Examples

Experimental program
Comparison scheme
Effect test

Embodiment 1

[0020] Weigh 3.98g of ferrous chloride tetrahydrate and 2.52g of oxalic acid dihydrate, mix them and grind them in a mortar for 1 hour, then put them into a ball mill, and ball mill them at a speed of 350r / min for 2 hours. After drying the ball-milled product at 105°C for 2 hours, add 3.42g of red clay, continue to mill in a ball mill for 2 hours, add water to extrude, and dry at 105°C to obtain a desulfurizer precursor. Put the desulfurizer precursor into a microwave tube furnace, set the microwave frequency to 2450MHz, microwave power to 1000W, and use three-stage heating to process the material. First raise the temperature to 250°C in the air atmosphere to decompose the material. After reaching the target temperature, switch to the simulated Texaco gas atmosphere, raise the temperature to 350°C, and take 1000h -1 Vulcanize the material at a certain vulcanization space velocity; after the vulcanization is complete, raise the temperature to 550°C, convert it into a nitrogen-a...

Embodiment 2

[0023] Weigh 3.98g of ferrous chloride tetrahydrate and 2.52g of oxalic acid dihydrate, mix them and grind them in a mortar for 1 hour, then put them into a ball mill, and ball mill them at a speed of 400r / min for 2 hours. After drying the ball-milled product at 100°C for 2 hours, add 3.19g of red clay, continue to mill in a ball mill for 2 hours, add water to extrude, and dry at 100°C to obtain a desulfurizer precursor. Put the desulfurizer precursor into a microwave tube furnace, set the microwave frequency to 2450MHz, microwave power to 1000W, and use three-stage heating to process the material. First raise the temperature to 300°C in the air atmosphere to decompose the material. After reaching the target temperature, switch to the simulated Texaco gas atmosphere, raise the temperature to 350°C, and take 1000h -1 The vulcanization space velocity will vulcanize the material; after the vulcanization is complete, the temperature will be raised to 600°C, and it will be converte...

Embodiment 3

[0026] Weigh 3.98g of ferrous chloride tetrahydrate and 2.52g of oxalic acid dihydrate, mix them and grind them in a mortar for 1 hour, then put them into a ball mill, and ball mill them at a speed of 450r / min for 2 hours. After drying the ball-milled product at 110°C for 2 hours, add 2.96g of red clay, continue to mill in a ball mill for 2 hours, add water to extrude, and dry at 110°C to obtain a desulfurizer precursor. Put the desulfurizer precursor into a microwave tube furnace, set the microwave frequency to 2450MHz, microwave power to 1000W, and use three-stage heating to process the material. First raise the temperature to 250°C in the air atmosphere to decompose the material. After reaching the target temperature, switch to the simulated Texaco gas atmosphere, raise the temperature to 400°C, and take 1000h -1 The vulcanization space velocity will vulcanize the material; after the vulcanization is complete, the temperature will be raised to 620°C, and converted into a ni...

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Abstract

The invention discloses a method for preparing a high-temperature gas desulfurizer in iron oxide by microwave. A microwave in-situ synthesis method is used, ferrous oxalate and a red soil carrier are prepared in a mixed manner to obtain a desulfurizer precursor, and in a microwave environment, the desulfurizer precursor is roasted at low temperature to be decomposed, and then vulcanized at low temperature and constant temperature in the atmosphere which simulates Texaco coal gas, and finally regenerated and cured in situ in the oxygen-containing atmosphere to obtain fresh medium-high temperature gas desulfurizer. The method for preparing the high-temperature gas desulfurizer in iron oxide by the microwave disclosed by the invention solves the problems of lowered vulcanization activity and powdered internal structure of the desulfurizer generated in a vulcanization-regeneration cycle process, enhances all the desulfurization efficiency, sulfur-capacity utilization rate and mechanical strength of the prepared desulfurizer, still keeps the desulfurization efficiency 98% or above after ten-time vulcanization / regeneration recycling use, and further reaches the mechanical strength by about 165cN / cm.

Description

technical field [0001] The invention belongs to the technical field of coal chemical desulfurizer preparation, and relates to a method for preparing a medium-high temperature gas desulfurizer, in particular to a microwave-based method for preparing an iron oxide desulfurizer. Background technique [0002] Clean transformation and efficient utilization of coal resources are important energy utilization technologies for sustainable economic and social development and environmental friendliness in my country. New power generation technologies such as integrated gasification combined cycle (IGCC) and molten carbonate fuel cells (CMFC) and The new coal-based polygeneration process of synthetic oil and alcohol ether fuel has become the main development direction of clean and efficient utilization of coal due to its advantages of high thermal efficiency and low pollution. However, the presence of sulfide in coal gasification products not only corrodes equipment and pipelines, but al...

Claims

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Application Information

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Patent Type & Authority Applications(China)
IPC IPC(8): C10K1/20C10K1/26
Inventor 冯宇米杰李阳武蒙蒙贾磊鲍卫仁
Owner 西安润川环保科技有限公司