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Nano photoelectric catalysis coupled microbial membrane electrode sleeve reactor and its application

A technology of photoelectric catalysis and microbial membrane, which is applied in the field of sewage treatment of new materials, pharmaceuticals and personal care products, and the field of microbial photoelectrochemistry. It can solve the problems of difficult to effectively degrade, low energy consumption, and low efficiency of electric energy utilization, and achieve the increase of hydroxyl free radicals. , Promote chemical degradation, low energy consumption

Active Publication Date: 2020-07-31
SOUTHEAST UNIV
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

[0004] Purpose of the invention: Aiming at the existing problems in the biofilm electrochemical system such as the small specific surface area of ​​the microbial film, low power utilization efficiency, complex composition and content of PPCPs, high removal cost, and difficulty in effective degradation, one of the purposes of the present invention It is to provide a sleeve-type reactor with nano-photoelectric catalysis coupled with microbial membrane electrodes, which integrates photoelectric catalysis technology and micro-current enhanced microbial biodegradation process, which has low energy consumption and good PPCPs treatment effect

Method used

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  • Nano photoelectric catalysis coupled microbial membrane electrode sleeve reactor and its application
  • Nano photoelectric catalysis coupled microbial membrane electrode sleeve reactor and its application
  • Nano photoelectric catalysis coupled microbial membrane electrode sleeve reactor and its application

Examples

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Embodiment 1

[0031] Such as Figure 1-Figure 3 , the present invention nano photoelectric catalysis coupled microbial membrane electrode sleeve reactor comprises a reaction chamber 1 with a water outlet, an anode module 2 and a cathode module 3 arranged in the reaction chamber, a power supply module 4 and a peristaltic pump 5 .

[0032] The reaction chamber 1 is made of plexiglass and has a cylindrical shape with an open top. The side of the reaction chamber 1 has a water outlet, and the water outlet is connected with an outlet pipe 6 through which the treated sewage is discharged.

[0033] The cathode module 3 includes a conductive inner cylinder 9 , a photoelectric catalytic activated carbon fiber 10 , a graphite rod 11 and a light source 12 arranged in the reaction chamber 1 . The conductive inner cylinder 9 is a stainless steel cylinder, and the bottom edge of the conductive inner cylinder 9 abuts against the bottom wall of the reaction chamber 1, so that the cathode module becomes an...

Embodiment 2

[0042] The nano-photoelectric catalysis coupled microbial membrane electrode sleeve reactor according to Example 1 of the present invention is used to treat sewage containing medicines and personal care products.

[0043] Specific parameter design of the reactor: the diameter of the reaction chamber 1 is 100 cm, the height is 120 cm, and the volume ratio of the cathode module 3 and the anode module 2 is 1:5. The water outlet height of the cathode module is 8-10cm higher than that of the anode module 2, and the water outlet height of the water outlet pipe is the same as that of the anode module 2.

[0044] Reactor startup: 1L of anaerobic activated sludge and 100L of nutrient solution (glucose 10g / L, NH 4 Cl0.12g / L, KH 2 PO 4 0.022g / L, NaCl 0.15g / L, trace elements 20mL) the mixed solution is introduced into the anode module 2 of the reactor, the external DC voltage is 1.2V-2.5V, the mixed solution is changed once a week, and the activated carbon fiber rope membrane is complet...

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Abstract

The invention discloses a nanometer photoelectrocatalysis coupling microorganism membrane electrode telescopic reactor and application. The reactor comprises: a reaction chamber provided with a water outlet, a positive electrode module, a negative electrode module, a power supply module and a peristaltic pump. The negative electrode module comprises: a conductive inner cylinder arranged in the reaction chamber and having an inner wall with photoelectrocatalytic active carbon fibers attached, a graphite rod and a light source disposed in the conductive inner cylinder, wherein the graphite rod is in electrical connection to the negative electrode of the power supply module which is powered up by the light source. The positive electrode module includes a conductive outer cylinder arranged in the reaction chamber and sleeving the conductive inner cylinder and connected to the positive electrode of the power supply module, active carbon fibers arranged between the conductive inner and other cylinders. The peristaltic pump is connected to a water inlet pipe, a water discharge end of which extends into the conductive inner cylinder. The invention further discloses an application of the reactor to treat PPCPs-containing sewage. The reactor couples photoelectrocatalysis and microcurrent-enhanced microorganism biodegradation into one body, and is low in energy consumption and good in PPCPs processing effect.

Description

technical field [0001] The invention relates to the technical field of microbial photoelectrochemistry, new materials, medicines and personal care products sewage treatment, in particular to a nano-photoelectric catalysis coupled microbial membrane electrode sleeve reactor and its application in the removal of medicines and personal care products. Background technique [0002] Pharmaceuticals and personal care products (PPCPs), as emerging environmental pollutants, have been detected in environmental media such as sewage, surface water, groundwater, and soil, and have been proven to have certain effects on the ecological environment and human health. Risks have aroused widespread concern from academia and the public. PPCPs mainly include estrogens, antibiotics, tranquilizers, contrast agents, antiepileptic drugs, blood lipid-regulating drugs, antipyretic, analgesic and anti-inflammatory drugs, and spices commonly used in cosmetics. Although the half-life of PPCPs is relativ...

Claims

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Application Information

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Patent Type & Authority Patents(China)
IPC IPC(8): C02F3/34
CPCC02F3/005C02F3/34C02F2203/006C02F2305/023C02F2305/10Y02W10/37
Inventor 张帅宋海亮杨小丽李骅张昱悦
Owner SOUTHEAST UNIV
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