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Water-based acrylic acid pressure-sensitive adhesive and preparation method thereof

A technology of acrylic pressure-sensitive adhesives and acrylic monomers, applied in the field of pressure-sensitive adhesives, can solve the problems of poor high temperature resistance, high initial adhesion, poor water resistance and low temperature resistance, etc., and achieve improved peel strength and high temperature resistance. Effect

Inactive Publication Date: 2018-10-26
TAICANG YUNTONG BIOCHEM ENG
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

Acrylate pressure-sensitive adhesives have the characteristics of weather resistance, oil resistance and transparency. At present, acrylic pressure-sensitive adhesives are available in water-emulsion type and solvent type. Solvent-type acrylic pressure-sensitive adhesives have high initial adhesion and good water resistance. Advantages, the biggest disadvantage is poor water resistance and low temperature resistance. Compared with conventional emulsion pressure-sensitive adhesives, soap-free emulsion pressure-sensitive adhesives have good water resistance and pressure-sensitive adhesive properties
[0003] In the prior art, pressure-sensitive adhesives have poor peel strength and poor high temperature resistance

Method used

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Examples

Experimental program
Comparison scheme
Effect test

Embodiment 1

[0021] Step 1. Proportioning raw materials, namely acrylic acid monomer (0.84:1 methyl methacrylate and hydroxyethyl acrylate), 0.2wt% ammonium persulfate initiator, 1wt% emulsification based on the acrylic monomer mass as 100wt% (The mass ratio is 1.5:1 CO-459 emulsifier and NPES 45 emulsifier), 8wt% tetramethyltetravinylcyclotetrasiloxane.

[0022] Step 2: Put acrylic monomer, emulsifier, sodium bicarbonate and water into the flask, and mechanically stir on a high-speed shearing machine at 1000 rpm for 20 minutes to obtain a pre-emulsified water dispersion.

[0023] Step 3. Take 0.10 of the emulsified water dispersion of the total mass of the pre-emulsified water dispersion and 0.10 of the ammonium persulfate of the total mass of the ammonium persulfate initiator, and put them into a constant pressure drop device, agitator, and condenser. Into a 500ml four-necked flask with nitrogen and nitrogen, and pass nitrogen protection, adjust the temperature to 7℃, polymerize for 1 hour, a...

Embodiment 2

[0028] Step 1. Proportioning raw materials, namely acrylic acid monomer (0.62:1 methyl methacrylate and hydroxyethyl acrylate), 0.8wt% ammonium persulfate initiator, 5wt% emulsification based on the acrylic monomer mass as 100wt% (The mass ratio is 1.1:1 CO-459 emulsifier and NPES 45 emulsifier), 15wt% tetramethyltetravinylcyclotetrasiloxane.

[0029] Step 2: Put acrylic monomer, emulsifier, sodium bicarbonate and water in the flask, and mechanically stir at 3000 rpm on a high-speed shearing machine for 10 minutes to obtain a pre-emulsified water dispersion.

[0030] Step 3: Take 0.30 of the emulsified water dispersion of the total mass of the pre-emulsified water dispersion, and 0.30 of the ammonium persulfate of the total mass of the ammonium persulfate initiator, and put them into a constant pressure drop device, agitator, and condenser. Into a 500ml four-neck flask with nitrogen and nitrogen, and pass nitrogen protection, adjust the temperature to 85℃, polymerize for 0.5h, and ...

Embodiment 3

[0035] Step 1. Proportioning raw materials, namely acrylic acid monomer (0.75:1 methyl methacrylate and hydroxyethyl acrylate), 0.5wt% ammonium persulfate initiator and 3wt% emulsification based on the acrylic monomer mass as 100wt% (The mass ratio of CO-459 emulsifier and NPES 45 emulsifier is 1.3:1), 12wt% tetramethyltetravinylcyclotetrasiloxane.

[0036] Step 2: Put acrylic monomer, emulsifier, sodium bicarbonate and water into the flask, and mechanically stir at 2000 rpm on a high-speed shear for 15 minutes to obtain a pre-emulsified water dispersion.

[0037] Step 3. Take 0.2 of the emulsified water dispersion of the total mass of the pre-emulsified water dispersion, and 0.2 of the ammonium persulfate of the total mass of the ammonium persulfate initiator, and put them into a constant pressure drop device, agitator, and condenser. Into a 500ml four-neck flask with nitrogen and nitrogen, and pass nitrogen protection, adjust the temperature to 80℃, polymerize for 0.75h, and obta...

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Abstract

The invention discloses a water-based acrylic acid pressure-sensitive adhesive and a preparation method thereof. According to the water-based acrylic acid pressure-sensitive adhesive, by adding tetravinyl tetramethylcyclotetrasiloxane into acrylic monomers, carbon-carbon double bonds of tetravinyl tetramethylcyclotetrasiloxane are grafted with macromolecular main chains formed through polymerization of the acrylic monomers to obtain a molecular structure containing grafted silicon-oxygen bonds, and the high temperature resistance of acrylic acid is improved; besides, a silicon-oxygen structureand an adhesive base material can form hydrogen-bond interaction, so that the peeling strength is improved.

Description

Technical field [0001] The invention relates to the technical field of pressure-sensitive adhesives, in particular to water-based acrylic pressure-sensitive adhesives and a preparation method thereof. Background technique [0002] Pressure-sensitive adhesive refers to a type of adhesive that can wet the surface to be adhered and stick the adherend firmly with a certain amount of pressure to produce practical bonding strength. Acrylic pressure sensitive adhesives have the characteristics of weather resistance, oil resistance and transparency. At present, acrylic pressure sensitive adhesives are available in water emulsion type and solvent type. Solvent type acrylic pressure sensitive adhesives have large initial adhesion and good water resistance. Advantages, the biggest disadvantage is poor water resistance and low temperature resistance. Compared with conventional emulsion pressure sensitive adhesives, soap-free emulsion pressure sensitive adhesives have good water resistance an...

Claims

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Application Information

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Patent Type & Authority Applications(China)
IPC IPC(8): C09J133/14C08F220/20C08F220/14C08F230/08
CPCC08F220/20C09J143/04C08F220/14C08F230/08
Inventor 张卫东
Owner TAICANG YUNTONG BIOCHEM ENG