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Method for extracting natural proanthocyanidins with different degrees of polymerization from cranberries

A technology of proanthocyanidins and degree of polymerization, applied in the direction of organic chemistry, which can solve the problems of increasing the risk of degradation of active substances and extremely high requirements for processes and equipment, and achieves soft extraction and purification conditions, strong operability and high yield Effect

Active Publication Date: 2021-04-30
HUNAN HUACHENG BIOTECH
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

This method involves repeated vacuum concentration, which will increase the risk of degradation of active substances. At the same time, it uses ozone as a depolymerization accelerator, which has extremely high requirements on process and equipment, and the forced depolymerization has a great risk to the activity of proanthocyanidins.

Method used

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Examples

Experimental program
Comparison scheme
Effect test

reference example 1

[0051] The polyamide resin used in the embodiment of the present invention is activated before use. The specific method is: after immersing the fresh resin in an ethanol solution with a volume fraction of 95% for 24 hours, rinse it with distilled water until it has no alcohol smell, and then use 2.5BV , Soak in 3.5% NaOH solution for 5.5 hours, rinse with distilled water until neutral, then soak in 2.5BV, 2.5% acetic acid solution for 5.5 hours, rinse with distilled water until neutral, and serve.

Embodiment 1

[0053] (1) Water extraction: Add 2000g of frozen cranberries with water in 3 times (the amount of water added is 20kg, 10kg, 10kg in turn), and heat extraction at 70°C respectively, and the time of each heating extraction is 3h , the time of heating, extracting and stirring each time is 5min, and then the clear liquid is obtained after passing through a decanter centrifuge;

[0054] (2) Ultrafiltration: pass the clear liquid obtained in step (1) through an ultrafiltration membrane with a molecular weight cut-off of 50,000 Da, and collect the permeate;

[0055] (3) Adsorption: Put the permeate obtained in step (2) directly on the 40-mesh polyamide resin column I for adsorption. When the leakage point is reached, start to string the column II with the same model and specification, and continue to add the permeate that is 0.8 times the weight of the loaded column;

[0056] (4) Water washing: use 1.5BV of water at a flow rate of 1.5BV / h, under the condition of series connection, ...

Embodiment 2

[0061] (1) Water extraction: dilute 400g cranberry extract concentrate with water to a dilution of 4brix;

[0062] (2) Ultrafiltration: pass the diluted solution obtained in step (1) through an ultrafiltration membrane with a molecular weight cut-off of 100,000 Da, and collect the permeate;

[0063] (3) Adsorption: Put the permeate obtained in step (2) directly on the 80-mesh polyamide resin column I for adsorption. The resin volume of column I is 200ml, the ratio of height to diameter is 5:1, and the flow rate on the column is 1.5BV / h. When the leakage point is reached, start to string the column II with the same type and specification, and continue to add permeate of 0.6 times the weight of the loaded column;

[0064] (4) Washing: use 2.5BV of water, at a flow rate of 1.0BV / h, under the condition of series connection, wash the column Ⅰ after step (3) adsorption with water, then untie the series connection, use 0.8BV of water alone, Use water at a flow rate of 1BV / h to catch...

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Abstract

The method for extracting natural proanthocyanidins with different degrees of polymerization from cranberries comprises the following steps: (1) after crushing the cranberries, adding water, heating and extracting, centrifuging, and suction filtering to obtain the supernatant; (2) dissolving the supernatant Pass the ultrafiltration membrane to collect the effluent; (3) Put the effluent on column I, when the effluent reaches the leakage point, start to connect the column II, and continue to put on the column and then stop the column; Then wash column II with water alone; (5) Desorb column I with gradient alcohol, desorb column II with alcohol aqueous solution at one time and collect the desorption solution; (6) Concentrate each desorption solution and dry it. The present invention can simultaneously obtain natural proanthocyanidin products with high content and high degree of polymerization and proanthocyanidin products with high content and low content of oligopolymerization, and the yield is high; the process of the present invention is simple, the requirements for process conditions are low, the extraction and purification conditions are soft, and no harmful Reagent, green and environment-friendly, suitable for industrial production.

Description

technical field [0001] The invention relates to a method for extracting proanthocyanidins, in particular to a method for simultaneously extracting natural proanthocyanidins with different degrees of polymerization from cranberries. Background technique [0002] Cranberry is one of the three traditional fruits in North America. It is very popular in the United States and is known as the "Ruby of North America". At the same time, it is being introduced into the Chinese market. Cranberries are rich in proanthocyanidins, which have many special functions such as anti-oxidation, anti-aging, prevention and treatment of digestive system diseases, prevention and treatment of urinary tract infections, anti-cancer, and protection of oral cavity and teeth. The proanthocyanidins contained in cranberries are a kind of phenolic compound, which is mainly a polymer formed by catechin and epicatechin. It is internationally recognized as the most effective natural antioxidant for clearing fre...

Claims

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Application Information

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Patent Type & Authority Patents(China)
IPC IPC(8): C07D311/62
CPCC07D311/62
Inventor 何安乐李伟黄华学
Owner HUNAN HUACHENG BIOTECH