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A kind of affinity adsorbent with yeast flocculin as ligand and its application

A flocculation protein and adsorbent technology, applied in the field of affinity adsorbent, can solve the problems of many side reactions, difficult separation and purification, etc., and achieve the effect of high efficiency

Active Publication Date: 2021-05-04
JIANGNAN UNIV
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

Mannan oligosaccharides are mainly obtained by hydrolyzing mannan with endomannanase, but there are many side reactions, and there are certain difficulties in separation and purification. Specific separation, which has broad application prospects for the preparation of single mannan oligosaccharides

Method used

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Examples

Experimental program
Comparison scheme
Effect test

Embodiment 1

[0025] Example 1 Expression of exogenous N-Lg-Flo1p in recombinant Escherichia coli

[0026] Based on the theory of yeast flocculation, the N-terminus of yeast cell wall flocculation protein was exogenously expressed in Escherichia coli, and used as a ligand to prepare an affinity adsorbent for separating functional sugars such as mannan oligosaccharides. Specific steps are as follows:

[0027] (1) Synthesize the gene encoding N-Lg-FLO1 shown in SEQ ID NO.1, connect the gene between the pET21b (+) carrier NdeI and XhoI, induce expression in Escherichia coli, screen positive clones, and inoculate into In the LB medium containing 50 μg / mL, cultivate at 37°C and 200r / min for 12h, transfer to the LB medium containing ampicillin with 1% inoculum size, and cultivate at 37°C and 200r / min until the logarithmic growth phase ( OD 600 value reached 0.6), and induced with a final concentration of 0.2mmol / L IPTG at 37°C and 200r / min for 8h, the target protein was present in the cell in t...

Embodiment 2

[0034] Example 2 Preparation of Affinity Adsorbent Using Yeast Flocculin (N-Lg-Flo1p) as Ligand

[0035] Get the N-Lg-Flo1p refolding liquid 8mL that prepares in Example 1 (contain N-Lg-Flo1p protein 16.5mg), purify through Ni-NTA Sepharose 6FF affinity column, use the equilibrium of 5 times column volume Wash the column with buffer solution, collect the washing solution until no protein flows out, measure the content of miscellaneous protein and unbound N-Lg-Flo1p with Q5000 ultra-micro nucleic acid protein analyzer, and calculate the concentration of N-Lg-Flo1p in Ni-NTA agarose. The adsorption amount on gel 6FF was 12.1 mg / mL. Thus, an affinity adsorbent with N-Lg-Flo1p as a ligand is obtained.

Embodiment 3

[0036] Example 3 Adsorption of mannan oligosaccharides with N-Lg-Flo1p-Ni-NTA Sepharose 6FF affinity adsorbent

[0037] Take 1 mL of N-Lg-Flo1p-Ni-NTA Sepharose 6FF affinity adsorbent, add to 10 mL of adsorption buffer (20 mmol / L Tris-HCl buffer, pH7.5, containing 0.2mol / L NaCl, 2mmol / L CaCl 2 ), shake for 1 h on a shaker with a rotational speed of 100 r / min. The affinity adsorbent was loaded into a column, and 5 column volumes were eluted with 20 mM Tris-HCl buffer solution containing 0.2M NaCl, pH 4.5, to collect mannooligosaccharides. The content of mannooligosaccharides in the eluent was determined by anthrone colorimetry, and the calculated adsorption capacity was 10.14 mg / (mL adsorbent).

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Abstract

The invention discloses an affinity adsorbent with yeast flocculin as ligand and its application, belonging to the field of biochemical industry. The present invention obtains the inclusion body N-Lg-Flo1p with His-tag through exogenous expression of Escherichia coli recombinant plasmid, through denaturation, dissolution and renaturation, and after purification by Ni-NTA agarose gel 6FF, a combination of The new affinity adsorbent of N‑Lg‑Flo1p has been tested to have an adsorption capacity of 10.14 mg / mL of mannan oligosaccharides, which lays the foundation for the industrial production of mannan oligosaccharide-specific adsorbents.

Description

technical field [0001] The invention relates to an affinity adsorbent with yeast flocculin as ligand and its application, which belongs to the field of biochemical industry. Background technique [0002] Yeast flocculin (Lg-Flo1p) is encoded by a typical gene containing intragenic repeat sequences in the yeast genome (collectively referred to as the FLO gene family), and is a cell wall protein composed of three domains: N-terminal, C-terminal and intermediate repeat sequences , the C-termini of these proteins are covalently linked to the cell wall, and the exposed N-termini can specifically bind to mannose residues on the adjacent yeast cell wall to cause flocculation. [0003] Manno-oligosaccharides are not digested by the human gastrointestinal tract, can promote the specific proliferation of intestinal probiotics represented by bifidobacteria in organisms, inhibit the growth of harmful bacteria, reduce the generation of toxic metabolites, and improve the human intestinal ...

Claims

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Application Information

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Patent Type & Authority Patents(China)
IPC IPC(8): B01J20/24B01J20/30C12N15/31C12P21/00B01D15/38
CPCB01D15/3809B01J20/24B01J2220/4856C07K14/39
Inventor 蔡国林谢莹陆健李晓敏吴殿辉
Owner JIANGNAN UNIV