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A method for enhancing the fluorescence of molybdenum disulfide based on double L-type metasurface structure

A molybdenum disulfide and structure-enhancing technology, applied in the field of nanophotonics, can solve problems such as insufficient photoluminescence intensity, and achieve the effects of less processing process, simple process and enhanced intensity

Active Publication Date: 2022-06-21
SOUTHEAST UNIV
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

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Problems solved by technology

[0005] Aiming at the problem of insufficient photoluminescence intensity of existing molybdenum disulfide materials, the present invention utilizes surface plasmon resonance enhancement, and proposes a method for enhancing the fluorescence of molybdenum disulfide based on a double L-shaped metasurface structure

Method used

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  • A method for enhancing the fluorescence of molybdenum disulfide based on double L-type metasurface structure
  • A method for enhancing the fluorescence of molybdenum disulfide based on double L-type metasurface structure
  • A method for enhancing the fluorescence of molybdenum disulfide based on double L-type metasurface structure

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Embodiment 1

[0028] Example 1: as figure 1 As shown, the metasurface structure is a double-L chiral structure, which is fixed in the metal groove, no filler is arranged in the metal groove, and a single layer of molybdenum disulfide is suspended on the metasurface structure and is only monolithic with the metasurface structure. Surface-to-surface contact, and silicon oxide is used as the substrate at the bottom of the metal groove. The metasurface structure consists of several arrays of double-L chiral structures.

[0029] Among them, the array period is 0.4 μm, the metal thickness of the metasurface structure is 60 nm, and the metal groove material is silver, which has a small intrinsic loss.

[0030] In this embodiment, the single-layer molybdenum disulfide of the light-emitting material is only in contact with one side of the metal groove, thereby ensuring that the excited surface plasmon resonance has a small intrinsic loss. Secondly, the design of the suspended molybdenum disulfide ...

Embodiment 2

[0031] Example 2: as figure 2 , the silver nanoarray is composed of two L-like grooves, the size of which is shown in the figure. The two L-shaped structures have the same size parameters as each other and are centrally symmetric, forming a chiral structure. The distance between the two L-shaped structures is 40 nm, the long side is 140 nm, and the widths are 85 nm and 65 nm.

Embodiment 3

[0032] Example 3: as image 3 is the selected specific preparation flow chart based on the double L-type metasurface structure;

[0033] Step 1: Coating a layer of silver metal film on the silicon oxide substrate;

[0034] Step 2: The metal layer is etched, and a centrosymmetric double L-shaped metasurface chiral structure is constructed by focused ion beam etching;

[0035] Step 3: The monolayer of molybdenum disulfide is wet transferred to the upper surface of the metal tank of the post-treated sample;

[0036] In step 1, the coating method is one of electron beam evaporation method EBE, chemical vapor deposition method CVD, magnetron sputtering method and thermal evaporation method.

[0037] In step 2, the etching method is one of electron beam lithography EBL and focused ion beam etching FIB.

[0038] In step 3, the wet transfer method for transferring molybdenum disulfide to the metasurface structure is as follows: taking the film-formed molybdenum disulfide on a silic...

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Abstract

The invention discloses a method for enhancing the fluorescence of molybdenum disulfide based on a double L-shaped metasurface structure, which enhances the photoluminescence intensity of molybdenum disulfide by exciting double resonances of surface plasmons; The material uses the double L-type metasurface structure to excite the surface plasmon resonance, and the double resonance generated in the excitation band and the emission band enhances the light absorption efficiency of molybdenum disulfide. Based on the metasurface chiral structure, the invention can enhance the photoluminescence of molybdenum disulfide, further explore the physical mechanism of valley spin, and regulate the polarization state of fluorescence. At the same time, the invention can be applied to high-performance low-dimensional material devices, optoelectronic devices, etc.

Description

technical field [0001] The invention relates to the technical field of nanophotonics, in particular to a method for enhancing the fluorescence of molybdenum disulfide based on a double L-type supersurface structure. Background technique [0002] Molybdenum disulfide, as a single atomic layer thin film material, is a new type of two-dimensional material, which has been widely used in various functions due to its high carrier mobility, excellent tuning ability and nonlinear effect. in the design of optoelectronic devices. Generally, the forbidden band widths of different layers of molybdenum disulfide are different. Multilayer molybdenum disulfide is an indirect bandgap semiconductor. As the number of layers decreases, quantum confinement effects and boundary effects will occur, resulting in a wider band gap. Monolayer molybdenum disulfide becomes a direct bandgap semiconductor. Therefore, in contrast to the layered structure, monolayer molybdenum disulfide is a straight-gap...

Claims

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Application Information

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Patent Type & Authority Patents(China)
IPC IPC(8): C09K11/68
CPCC09K11/681
Inventor 胡国华王均耀林霖霞黄磊恽斌峰崔一平
Owner SOUTHEAST UNIV