Adhesive for superposition
A technology of adhesives and emulsions, applied in the direction of adhesive types, adhesives, polyurea/polyurethane adhesives, etc., which can solve the problems of difficult performance, cold resistance, insufficient heat resistance, and reduced heat resistance.
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[0038] Next, the present invention will be described in more detail based on examples. In addition, this invention is not limited to these Examples.
[0039] In addition, glass transition temperature of ethylene-vinyl acetate copolymer emulsion, benzene elution rate, preparation of samples for adhesive force measurement, normal state adhesive force, water-resistant adhesive force, and low-temperature adhesiveness using the samples And thermal creep resistance was measured according to the following method.
manufacture example 1
[0041]
[0042] Add 800 g of water and 60 g of partially saponified polyvinyl alcohol (saponification degree: 88%) to a 3 L autoclave, pressurize with ethylene, and add 1,000 g of vinyl acetate and diallyl phthalate as an internal crosslinking agent dropwise. 20 g of the ester was used to prepare an ethylene-vinyl acetate copolymer emulsion with a solid content of 55%. During production, the pressure of pressurized ethylene was varied from 2 to 6 MPa to produce four types of ethylene-vinyl acetate copolymer emulsions having different glass transition temperatures. (EVA-1: glass transition temperature 10°C), (EVA-2: glass transition temperature -8°C), (EVA-3: glass transition temperature 25°C), (EVA-4: glass transition temperature - 20℃)
manufacture example 2
[0044]
[0045] Add 800 g of water and 60 g of partially saponified polyvinyl alcohol (the degree of saponification is 88%) in a 3L autoclave, pressurize with ethylene, add 1020 g of vinyl acetate dropwise, and trial-produce a polyvinyl alcohol with a solid content of 55% and a glass transition temperature of Two types of ethylene-vinyl acetate copolymer emulsions at 10°C and -8°C. (EVA-5: glass transition temperature 10°C), (EVA-6: glass transition temperature -8°C)
[0046] Table 1 shows the characteristic values of the produced (A) component ethylene-vinyl acetate copolymer emulsion.
[0047]
[0048] Adhesives were prepared according to the compounding recipes shown in Table 2 and Table 3. While mixing the three components (A), (B) and (C), in order to promote the film-forming properties of the emulsion, 6 parts by mass of butyl carboxylate was added to 100 parts by mass of the ethylene-vinyl acetate copolymer emulsion. Must alcohol acetate, made into adhesive.
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