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Purification method of penicillin and cephalosporin

A cephalosporin and purification method technology, applied in the field of chemical engineering, can solve the problems of cumbersome operation and long time required for separation, and achieve the effects of high separation efficiency, improved separation effect and long service life

Inactive Publication Date: 2011-05-04
ZHEJIANG UNIV
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

The disadvantage of ion exchange chromatography is that the separation takes a long time and the operation is cumbersome

Method used

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Examples

Experimental program
Comparison scheme
Effect test

Embodiment 1

[0027] Weigh 3g of penicillin G sodium and dissolve it in water, and load it on the chromatographic column. After the Toyopearl HW-40F filler is fully swelled by the eluent (0.005mol / L, pH7.0 sodium citrate buffer solution), the column is packed by wet method. The column size is φ1.6cm×60cm, and the column volume (BV ) is 120.6 mL. At 5° C., 0.005 mol / L, pH 7.0 sodium citrate buffer was used to flow through the chromatographic column at an elution flow rate of 0.5 BV / hr, and the amount of eluent was 3 BV. Macromolecular impurities are eluted in the front, and penicillin G sodium is eluted in the back, and macromolecular impurities and penicillin G sodium are collected respectively and freeze-dried. The yield of penicillin G sodium was 95.8%.

[0028] The sensitization of macromolecular impurities and purified penicillin G sodium was tested by passive skin allergy test. Rabbit anti-penicillin-binding protein serum (preparation method as described in the Summary of the Invent...

Embodiment 2

[0030] Adjust the pH value of the 250 mg / mL penicillin G sodium solution to 8.0, place it at 25°C for 15 days, and load 2 mL of the sample on the chromatographic column. After the Toyopearl HW-40S filler is fully swelled by the eluent (0.1mol / L, pH7.0 sodium citrate buffer), the column is packed by wet method, the column size is φ1.6cm×33cm, and the column volume (BV ) is 66.4mL. At 25° C., 0.1 mol / L, pH 7.0 sodium citrate buffer was used to flow through the chromatographic column at an elution flow rate of 0.3 BV / hr, and the amount of eluent was 4 BV. Before the elution position of penicillin G sodium, ultraviolet absorbing substances were eluted and collected and freeze-dried. Passive skin sensitization test As described in Example 1, components eluting prior to penicillin G sodium can elicit an allergic reaction in guinea pigs.

Embodiment 3

[0032] Weigh 1 g of ampicillin, dissolve it in water, and load it on the chromatographic column. After the Toyopearl HW-40S filler is fully swollen by the eluent (0.5% sodium chloride solution), the column is packed by wet method. The column size is φ1.6cm×30cm, and the column volume (BV) is 60.3mL. At 15°C, 0.5% sodium chloride solution was used to flow through the chromatographic column at an elution flow rate of 0.5BV / hr, and the amount of eluent used was 3BV. Macromolecular impurities and ampicillin were collected separately and freeze-dried. The yield of ampicillin was 96.6%. Passive skin allergy test As described in Example 1, the macromolecular impurities in ampicillin cause allergic reactions in guinea pigs, and the purified ampicillin has no sensitization.

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Abstract

The invention discloses a method for purifying penicillin and cephalosporin, which comprises the following steps that: the penicillin or the cephalosporin is dissolved into water, the mixture is loaded to a chromatographic column filled by a Toyopearl HW-40 filler, the water or an electrolyte solution is used to elute an eluent, and the purified penicillin or the cephalosporin is obtained after the separation. The method separates macromolecular impurities in the penicillin and the cephalosporin by a chromatography, and a filler adopted by the method is Toyopearl HW-40; and the filler can produce adsorption effect on the penicillin and the cephalosporin when taking a water solution as a mobile phase, so the separation effect of the macromolecular impurities in the penicillin and the cephalosporin is improved greatly.

Description

technical field [0001] The invention relates to the technical field of chemical engineering, in particular to a method for purifying penicillins and cephalosporins. Background technique [0002] Penicillins and cephalosporins are antibiotics widely used in clinical practice. They have the characteristics of high efficiency, low toxicity, and good dispersibility. However, these drugs can cause allergic reactions in some patients, and anaphylactic shock is extremely harmful. [0003] The necessary condition for a molecule to be an allergen is that it must have an antigenic determinant with a specific structure that can be recognized by antibodies, and at least two antigenic determinants must be present. The β-lactam antibiotics currently used in clinical practice are neither immunogenic nor cause allergic reactions. The compound does not trigger an allergic reaction. [0004] Macromolecular impurities (molecular weight greater than 1000) in antibiotic products can come from ...

Claims

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Application Information

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Patent Type & Authority Patents(China)
IPC IPC(8): C07D499/18C07D501/12A61P31/00B01D15/08
Inventor 苏宝根卢昕博邢华斌杨亦文苏云任其龙
Owner ZHEJIANG UNIV