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Method for producing alkylate by low-temperature hydro-alkylation of C4 olefins

A carbon tetraolefin and alkylated gasoline technology, which is applied in the production of liquid hydrocarbon mixtures, petroleum industry, organic chemistry, etc., can solve the problems of reducing the comprehensive utilization value of carbon tetraolefin, and achieve the effect of short service life in one pass

Active Publication Date: 2012-10-17
PETROCHINA CO LTD
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

[0009] In short, since the above patents are carried out at a relatively high reaction temperature, a large amount of methane and ethane will inevitably be produced, which reduces the comprehensive utilization value of carbon tetraolefins

Method used

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Examples

Experimental program
Comparison scheme
Effect test

Embodiment 1

[0027] Refinery heavy carbon four is the reaction raw material, and its olefin content is as high as 79% (w). Catalyst A is used as the catalyst for the alkylation reaction, and strip-shaped aluminum oxide is used as the inert material. The volume ratio of the catalyst and the inert material is 1:1 into a fixed bed reactor. At a reaction temperature of 250°C, a reaction pressure of 2.0Mpa, and a liquid volume space velocity of 0.8h -1 1. Under the reaction condition of hydrogen oil ratio of 120:1, the alkylation reaction is carried out in a fixed bed reactor, and the yield of liquid above C5 can be as high as 75% to 80% in the process of running for 1260 hours. The sum of linear alkanes and branched alkanes in alkylated oil is higher than 63%, naphthenics is 11.97%, benzene is as low as 0.35%, total aromatics is 10.14%, and olefins are less than 1.5%. In the gas phase products generated, the dry gas content is as low as 0.004% to 0.005%. The octane number of the liquid-phase...

Embodiment 2

[0029] The reaction raw materials and the catalyst are the same as in Example 1, and the strip ceramics are used as the inert material, and the catalyst and the strip ceramics are added to the fixed-bed reactor at a volume ratio of 1.1:1. At a reaction temperature of 280°C, a reaction pressure of 2.5Mpa, and a liquid volume space velocity of 1.0h -1 1. Under the reaction condition of hydrogen oil ratio of 150:1, after the alkylation reaction in the fixed bed reactor, the liquid yield is as high as 75% or more in the process of running for 1240 hours. The sum of linear alkanes and branched alkanes in alkylated oil is higher than 67%, naphthenics is 11.95%, benzene is as low as 0.58%, total aromatics is 11.49%, and olefins are less than 1.5%. In the gas phase products generated, the dry gas content is as low as 0.004% to 0.005%. The liquid phase produced oil had an octane number of 93.8 (RON).

Embodiment 3

[0031] Refinery heavy carbon four is used as reaction raw material, and its olefin content is as high as 82% (w). Catalyst B is used as catalyst for alkylation reaction, and strip-shaped aluminum oxide is used as inert material. Ratio of 0.8:1 into the fixed bed reactor. At a reaction temperature of 230°C, a reaction pressure of 1.8Mpa, and a liquid volume space velocity of 1.1h -1 1. Under the reaction condition of hydrogen oil ratio of 160:1, after the alkylation reaction in the fixed bed reactor, the liquid yield is as high as 75% or more in the process of running for 1300 hours. The sum of linear alkanes and branched alkanes in alkylated oil is higher than 68%, naphthenic content is as high as 13.50%, benzene content is as low as 0.21%, total aromatics content is 11.10%, and olefin content is less than 1.5%. In the gas phase products generated, the dry gas content is as low as 0.002%. The octane number of the liquid-phase forming oil was 94.6 (RON).

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Abstract

The invention provides a method for producing alkylate by low-temperature hydro-alkylation of C4 olefins. The method comprises the following steps that: the mixed C4 is put in a thermal insulation fixed bed reactor filled with zeolite molecular sieve catalyst for alkylated reaction. The method is characterized in that: the catalyst is mixed with inert materials during filling; the zeolite molecular sieve catalyst and the inert materials are mixed according to a volume ratio of between 0.5-2:1 and put in the reactor; and under conditions of temperature of between 150 and 300 DEG C, hydrogen-oil volume ratio of between 100 and 260:1, reaction pressure of between 1 and 2MPa and liquid volume airspeed of between 0.8 and 1.6h<-1>, the mixture is reacted to generate blended components of high octane gasoline, or a high-quality ethylene cracking material. The octane value of the generated alkylate is high, the summation of contents of straight chain paraffin and branched chain paraffin is high (more than 60 percent), the content of cycloparaffinic hydrocarbon is high (more than 10 percent), the content of benzene is quite low (less than 1 percent), the content of total aromatic hydrocarbon is low (less than 15 percent), and the content of olefin is low (less than 2 percent).

Description

technical field [0001] The invention relates to a method for producing alkylated oil by low-temperature hydroalkylation of carbon tetraolefins. It is especially suitable for the production of alkylated oil rich in straight-chain alkanes, branched-chain alkanes and cycloalkanes with low aromatics content through alkylation reaction of C4-olefins at low temperature. Background technique [0002] Mixed liquefied gas is a by-product of catalytic cracking units in refineries and steam cracking units in petrochemical enterprises. The output of liquefied gas is large. At present, most of the liquefied gas is burned as civilian liquefied gas, which is an astonishing waste. C4 liquefied petroleum gas contains a large amount of various butenes, and converting butenes into fuel gasoline is a very meaningful way of resource utilization. In recent years, people have done a lot of research on the aromatization reaction of carbon tetraolefins on zeolite molecular sieve catalysts, and the ...

Claims

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Application Information

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Patent Type & Authority Patents(China)
IPC IPC(8): C10G50/00C07C11/08C07C5/03
Inventor 晁世海李吉春张志喜程亮亮马应海黄彦科
Owner PETROCHINA CO LTD