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Magnetic nano base metal fluoride load type solid base catalyst and preparation method thereof

A technology of alkali metal fluoride and solid alkali catalyst, applied in the direction of physical/chemical process catalysts, chemical instruments and methods, chemical/physical processes, etc., to achieve strong magnetism, uniform distribution, and good dispersion

Inactive Publication Date: 2011-11-02
BEIJING UNIV OF CHEM TECH
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

So far, there has been no magnetic nano-Fe coated with magnesium-aluminum composite oxide. 3 o 4 As a carrier, a report on the preparation of alkali metal fluoride-supported magnetic nanometer solid base catalyst by rapid rotary evaporation impregnation method

Method used

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Examples

Experimental program
Comparison scheme
Effect test

Embodiment 1

[0022] (1) Preparation and surface modification of magnetic substances

[0023] Weigh 2.7g (0.01mol) FeCl 3 ·6H 2O and 7.2g (0.045mol) of sodium acetate were dissolved in 80ml of ethylene glycol and stirred at room temperature until dissolved to form a uniformly dispersed solution. The resulting solution was transferred to a 100 ml autoclave, and then crystallized at 200° C. for 8 hours. The autoclave was taken out and naturally cooled to room temperature, and the obtained Fe 3 o 4 The suspension was washed three times successively with ethanol and deionized water (100 ml of ethanol each time, and 200 ml of deionized water each time). Use NdFeB permanent magnet to separate Fe during washing 3 o 4 solid. After washing, the obtained Fe 3 o 4 The solid was dispersed in ethanol for storage. The Fe obtained by the above steps 3 o 4 The particle size is 150nm, and the specific saturation magnetization σ s 87.9A·m 2 / kg.

[0024] Weigh 0.1g of the above Fe 3 o 4 Add ...

Embodiment 2

[0031] (1) Preparation and surface modification of magnetic substances

[0032] Weigh 2.7g (0.01mol) FeCl 3 ·6H 2 O and 7.2g (0.045mol) of sodium acetate were dissolved in 80ml of ethylene glycol and stirred at room temperature until dissolved to form a uniformly dispersed solution. The obtained solution was transferred to a 100 ml autoclave, and crystallized at 200° C. for 8 hours. The autoclave was taken out and naturally cooled to room temperature, and the obtained Fe 3 o 4 The suspension was washed three times successively with ethanol and deionized water (100 ml of ethanol each time, and 200 ml of deionized water each time). Use NdFeB permanent magnet to separate Fe during washing 3 o 4 solid. After washing, the obtained Fe 3 0 4 The solid was dispersed in ethanol for storage. The Fe obtained by the above steps 3 o 4 The particle size is 150nm, and the specific saturation magnetization σ s 80.5A·m 2 / kg.

[0033] Weigh 0.1g of the above Fe 3 o 4 Add the s...

Embodiment 3

[0040] (1) Preparation and surface modification of magnetic substances

[0041] Weigh 5.44g (0.02mol) FeCl 3 ·6H 2 O and 14.4g (0.09mol) of sodium acetate were dissolved in 160ml of ethylene glycol and stirred at room temperature until dissolved to form a uniformly dispersed solution. The resulting solution was transferred to a 200ml autoclave, and crystallized at 200°C for 8 hours. The autoclave was taken out and naturally cooled to room temperature, and the obtained Fe 3 o 4 The suspension was washed three times successively with ethanol and deionized water (100 ml of ethanol each time, and 200 ml of deionized water each time). Use NdFeB permanent magnet to separate Fe during washing 3 o 4 solid. After washing, the obtained Fe 3 o 4 The solid was dispersed in ethanol for storage. The Fe obtained by the above steps 3 o 4 The particle size is 140nm, and the specific saturation magnetization σ s 85.2A·m 2 / kg.

[0042] Weigh 0.1g of the above Fe 3 o 4 Add the s...

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Abstract

The present invention relates to a magnetic nano base metal fluoride load type solid base catalyst and a preparation method thereof, belonging to the technical field of a nano catalyst. The solid base catalyst comprises nuclear shell type magnalium composite oxide-coated magnetic nano Fe3O4 carriers and a base metal fluoride load MF, wherein M is any one of L1, Na, K and Cs; the composition comprises the following components by mass percentage: 50%-70% of magnetic nano Fe3O4, 20%-40% of magnalium composite oxides and 5%-15% of base metal fluoride load MF; the particle size of the magnetic nano load type solid base catalyst is 170-190 nm; and the saturation magnetization strength sigma s is 9.3-13.1 A.m<2> / kg. The composition of the solid base catalyst comprises the magnalium metal composite oxide-coated magnetic nano Fe3O4 as the magnetic carriers of the catalyst and the base metal fluoride load MF as a load. The solid base catalyst has the characteristics of controllable particle diameter, uniform distribution, stronger magnetism, good dispersion and the like, is suitable for some organic reactions needing base catalysis, such as Knoevengel condensation, Michael addition and ester exchange and the like.

Description

technical field [0001] The invention belongs to the technical field of nano-catalysts, in particular to a magnetic nano-alkali metal fluoride-supported solid base catalyst and a preparation method thereof, a core-shell magnesium-aluminum composite oxide-coated magnetic nano-Fe 3 0 4 The invention discloses a preparation method of a solid alkali catalyst loaded with alkali metal fluoride. Background technique [0002] In the field of catalysis research, homogeneous catalysis has gradually transitioned to heterogeneous catalysis, and the use of solid base instead of liquid base for catalysis has the following advantages: (1) recyclable, environmentally friendly, non-corrosive, avoiding the use of polar solvents or phases Transfer agent; (2) high selectivity, high catalytic activity, mild reaction conditions, and easy separation of products; (3) can make the reaction process continuous and improve the production capacity of the equipment; (4) can react at high temperature or e...

Claims

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Application Information

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Patent Type & Authority Patents(China)
IPC IPC(8): B01J27/128B01J35/10
Inventor 张慧郤玉生盘登科谭冰峰
Owner BEIJING UNIV OF CHEM TECH