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Catalytic thermal cracking catalyst and preparation method thereof

A catalytic thermal cracking and catalytic cracking technology, which is applied in the field of catalytic thermal cracking catalyst and its preparation, can solve the problem of insufficient ethylene yield, achieve good thermal and hydrothermal stability, improve sphericity, and high crystallinity.

Active Publication Date: 2013-01-09
CHINA PETROLEUM & CHEM CORP
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

[0005] However, the above catalysts are used for catalytic pyrolysis, and the ethylene yield is not high enough

Method used

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Examples

Experimental program
Comparison scheme
Effect test

preparation example Construction

[0024] In the preparation method of the catalyst provided by the present invention, the preparation of the aluminum binder slurry described in step (2) is prepared according to the preparation method of the aluminum binder slurry in the existing cracking catalyst preparation process, including mixing the aluminum binder with water The steps of mixing, beating, and adding acid for acidification, the preferred amount of acid is one or more of the commonly used acids in cracking catalyst preparation such as hydrochloric acid, nitric acid and phosphoric acid so that the pH value of the slurry is 2-4. The aluminum binder is selected from pseudoboehmite, hydrated alumina with a gibbsite structure, hydrated alumina with a gibbsite structure, hydrated alumina with a Bayerite structure, γ-alumina, η- One or more of alumina, θ-alumina, χ-alumina, and aluminum sol. Based on the weight of the catalyst, the amount of alumina introduced into the aluminum binder slurry is 5-75% by weight, pr...

Embodiment 1

[0033] (1) 4Kg of ZrOCl 2 (wherein zirconia 36% by weight, industrial grade, Zibo Huantuo Chemical Co., Ltd.) is mixed with decationized water to make an aqueous solution with a concentration of 1.0mol / L, and ammonia (Beijing Chemical Plant, 25% by weight) is added to the pH value under stirring. 9, then aged at 25°C for 26 hours with stirring, and filtered to obtain ZrO(OH) 2 Gel, washed with deionized water until no Cl was detected in the washing solution after washing - , drying at 120°C for 24 hours, and calcining at 550°C for 2 hours to obtain zirconia powder;

[0034] (2) 20Kg decationized water is mixed with 10Kg pseudo-boehmite (industrial product of Shandong Aluminum Factory, solid content 63m%), beating, and its pH value is 3 with hydrochloric acid adjustment;

[0035] (3) Add 19Kg halloysite (industrial product of Suzhou China Clay Company, solid content 72.3% by weight) into the slurry obtained in step (2), beating for 5 minutes, then add 0.61Kg of zirconia powde...

Embodiment 2

[0039] (1) 20Kg decationized water is mixed with 10Kg pseudo-boehmite (industrial product of Shandong Aluminum Factory, solid content 63m%), beating, and its pH value is 2.5 with hydrochloric acid adjustment;

[0040] (2) 14Kg ZrOCl 2 (36% by weight, industrial grade, Zibo Huantuo Chemical Co., Ltd.) mixes with decationized water to obtain an aqueous solution with a concentration of 1.5mol / L, and then adds ammoniacal liquor (Beijing Chemical Plant, 25% by weight) to it under stirring. The pH value is 9, aged for 16 hours under stirring at 30°C, and filtered to obtain ZrO(OH) 2 Gel, washed with deionized water until Cl-free in the washed water - Detected, dried at 115°C for 26 hours, and calcined at 600°C for 5 hours to obtain zirconia powder;

[0041] (3) 18Kg halloysite (industrial product of Suzhou China Clay Company, solid content 72.3% by weight) is added in the slurry obtained in step (1) and mixed, beating for 5 minutes, then adding 3.21Kg of zirconia powder prepared i...

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Abstract

The invention relates to a catalytic thermal cracking catalyst and a preparation method thereof. The catalyst comprises the following components by weight percent: 5-75% of aluminum bonding agent, 0.5-70% of zeolite with MFI structure and 3-25% of zirconium oxide substrate, wherein the weight of aluminum bonding agent is calculated according to aluminium oxide; the silicon-aluminium ratio of the zeolite with MFI structure is 15-300, and the diameter of the primary particles is 5-55mu m. The preparation method of the catalyst comprises the following steps: mixing zeolite with MFI structure, aluminium oxide bonding agent and zirconium oxide substrate, beating and drying, wherein in the beating process, zirconium oxide substrate is introduced in two steps. The catalyst of the invention is used for the catalytic thermal cracking of heavy oil, the conversion rate of the raw material is high, the low-carbon olefin selectivity is good; and by using the preparation method of the invention, the wear resistance of the catalyst can be improved and the thermal stability and hydrothermal stability of the catalyst can be increased.

Description

technical field [0001] The invention relates to a catalytic thermal cracking catalyst and a preparation method thereof. Background technique [0002] Catalytic pyrolysis is a method of producing ethylene and propylene from heavy oil in the presence of a catalyst. It has the characteristics of low energy consumption, low raw material requirements, and flexible adjustment of product distribution. The reaction temperature of the catalytic pyrolysis (CPP) process is relatively high, up to 600°C. Therefore, the catalyst used is required to have good thermal and hydrothermal stability, especially as the cracking raw material becomes heavier and worse, and its operating severity increases. Catalytic pyrolysis catalysts put forward higher requirements. [0003] CN1048428C discloses a catalyst for producing low-carbon olefins by converting petroleum hydrocarbons. The catalyst is composed of 0-70% by weight of clay, 5-90% by weight of inorganic oxides and 10-35% by weight of zeolite,...

Claims

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Application Information

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Patent Type & Authority Patents(China)
IPC IPC(8): B01J29/40B01J37/00C10G11/05C07C11/04C07C11/06
CPCY02P20/52
Inventor 许昀赵留周刘宇键朱玉霞田辉平
Owner CHINA PETROLEUM & CHEM CORP