Method for synthesizing polyester block silicone oil by waste polyester
A technology of polyester block and polyester silicone oil, which is applied in the synthesis of polyester block silicone oil, and in the field of synthesizing polyester block silicone oil with waste polyester, which can solve the problems of using unpolyether polyester copolymer polyols, etc. Achieve the effect of simple process
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Embodiment 1
[0019] Synthesis of polyether polyester polyols from polyester waste: in a four-necked flask with a thermometer, a stirrer, a nitrogen inlet pipe and a fractionation device, 39g of diethylene glycol, 49g of PET polyester bottle fragments, 1000 Molecular weight polyethylene oxide 1000g, n-butyl titanate as catalyst 0.4g. In the case of feeding nitrogen, the temperature is gradually raised to 180°C, the temperature of the fractionation column is lower than 105°C, and the temperature is maintained until no small molecules are distilled; then the temperature is raised to 240°C, and the reaction is kept for 4 hours until the system becomes transparent and uniform; Vacuumize at -0.09MPa for 1h. Cool down to 140°C and discharge.
[0020] Synthesis of block polyester silicone oil: 50g polyether polyester polyol, 60g terminal ethyl acrylate silicone oil (molecular weight: 10000), n-butyl titanate as catalyst 0.1g. Under the condition of feeding nitrogen, gradually raise the temperatu...
Embodiment 2
[0022] Synthetic polyether polyester polyols from waste materials: in a four-necked flask with a thermometer, a stirrer, a nitrogen inlet pipe and a fractionation device, successively drop into ethylene glycol 49g, PET polyester bottle fragments 29g, polyepoxide with a molecular weight of 2000 680 g of ethane, and 0.3 g of n-butyl titanate as a catalyst. In the case of feeding nitrogen, the temperature is gradually raised to 190°C, the temperature of the fractionation column is lower than 105°C, and the temperature is maintained until no small molecules are distilled; then the temperature is raised to 250°C, and the reaction is kept for 4 hours until the system becomes transparent and uniform; Vacuum at -0.098MPa for 1h. Cool down to 140°C and discharge.
[0023] Synthesis of block polyester silicone oil: 70g of polyether polyester polyol, 30g of acrylate-terminated silicone oil (molecular weight: 20,000), and 0.3g of n-butyl titanate as a catalyst. Under the condition of fe...
Embodiment 3
[0025] Synthesis of polyether polyester polyols from waste materials: in a four-necked flask with a thermometer, a stirrer, a nitrogen inlet pipe and a fractionation device, 38 g of neopentyl glycol, 29 g of PET polyester bottle fragments, and polycyclic polycyclic alcohols of 3000 molecular weight are successively dropped into Oxyethane 680g, manganese acetate as catalyst 0.3g. In the case of feeding nitrogen, the temperature is gradually raised to 190°C, the temperature of the fractionation column is lower than 105°C, and the temperature is maintained until no small molecules are distilled; then the temperature is raised to 250°C, and the reaction is kept for 4 hours until the system becomes transparent and uniform; Vacuum at -0.098MPa for 1h. Cool down to 140°C and discharge.
[0026] Synthesis of block polyester silicone oil: 80g polyether polyester polyol, 25g terminal butyl acrylate silicone oil (molecular weight: 10000), 0.3g zinc acetate as catalyst. Under the condit...
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