Unlock instant, AI-driven research and patent intelligence for your innovation.

Method for preparing lithium phosphate nano-particles

A nanoparticle, lithium phosphate technology, applied in nanotechnology, nanotechnology, chemical instruments and methods, etc., can solve the problems of large particle size of lithium phosphate particles, serious particle growth, unfavorable rapid nucleation and other problems, and achieve good equipment reliability. , small size, easy to operate effect

Active Publication Date: 2014-04-30
TSINGHUA UNIV
View PDF3 Cites 7 Cited by
  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

Due to the low mixing and mass transfer efficiency of conventional reactors, the local supersaturation is low, which is not conducive to rapid nucleation, and because the reaction time is generally 1 to 5 hours, the reaction time is longer, and the particle growth is more serious, resulting in lithium phosphate particles. The particle size is large and uneven, and the average particle size is in the micron range

Method used

the structure of the environmentally friendly knitted fabric provided by the present invention; figure 2 Flow chart of the yarn wrapping machine for environmentally friendly knitted fabrics and storage devices; image 3 Is the parameter map of the yarn covering machine
View more

Examples

Experimental program
Comparison scheme
Effect test

Embodiment 1

[0023] A membrane dispersion microreactor is used, which uses a microporous membrane as the dispersion medium. Prepare 1L of 2.00mol / L lithium hydroxide aqueous solution and put it into the storage container to obtain solution A. At the same time, 1L of 0.50mol / L phosphoric acid aqueous solution was prepared and put into the storage container to obtain solution B. At a reaction temperature of 20°C, solution A was added to the microreactor at a flow rate of 50ml / min from the storage container, solution B was added to the microreactor at a flow rate of 50ml / min from the storage container, and solution A and solution B were in the microreactor. The fast-forward mixing and precipitation reaction occurred in the reactor, and the reaction time was 0.3s. Slurry C is obtained from the outlet of the reactor, the slurry C is filtered to obtain the precipitate, the precipitate is washed and dried at 60° C., and finally milled to obtain lithium phosphate nanoparticles with an average part...

Embodiment 2

[0025] A micro-mesh micro-reactor is used, which uses a micro-mesh plate as the dispersion medium. Prepare 1L of 1.50mol / L lithium carbonate aqueous solution and put it into the storage container to obtain solution A. At the same time, 1L of 1.00mol / L phosphoric acid aqueous solution was prepared and put into the storage container to obtain solution B. At a reaction temperature of 50°C, solution A was added to the microreactor at a flow rate of 70ml / min from the storage container, solution B was added to the microreactor at a flow rate of 70ml / min from the storage container, and solution A and solution B were in the microreactor. The mixing and precipitation reaction occurred in the reactor, and the reaction time was 0.3s. Slurry C is obtained from the reactor outlet, the slurry C is filtered to obtain the precipitate, the precipitate is washed and dried at 80° C., and finally milled to obtain lithium phosphate nanoparticles with an average particle size of 100 nm and a yield ...

Embodiment 3

[0027] A co-current micro-flute micro reactor is used, which has a co-current micro-flute micro structure. Prepare 1L of 3.00mol / L lithium acetate aqueous solution and put it into a storage container to obtain solution A. At the same time, 3L of 0.50mol / L phosphoric acid aqueous solution was prepared and put into the storage container to obtain solution B. At a reaction temperature of 90°C, solution A was added to the microreactor at a flow rate of 10ml / min from the storage container, solution B was added to the microreactor at a flow rate of 30ml / min from the storage container, and solution A and solution B were in the microreactor. The mixing and precipitation reaction occurred in the reactor, and the reaction time was 0.6s. Slurry C is obtained from the reactor outlet, the slurry C is filtered to obtain the precipitate, the precipitate is washed and dried at 70° C., and finally milled to obtain lithium phosphate nanoparticles with an average particle diameter of 120 nm and ...

the structure of the environmentally friendly knitted fabric provided by the present invention; figure 2 Flow chart of the yarn wrapping machine for environmentally friendly knitted fabrics and storage devices; image 3 Is the parameter map of the yarn covering machine
Login to View More

PUM

PropertyMeasurementUnit
particle sizeaaaaaaaaaa
melting pointaaaaaaaaaa
particle diameteraaaaaaaaaa
Login to View More

Abstract

The invention discloses a method for preparing lithium phosphate nano-particles in the technical field of chemistry and chemical engineering. The method comprises the steps of quickly mixing an aqueous solution containing lithium element with an aqueous solution containing phosphorus element in a micro-reactor for reacting at a temperature ranging from 20 to 90 DEG C, obtaining slurry containing lithium phosphate precipitation from the outlet of the reactor, performing solid-liquid separation, washing, drying and grinding on the slurry, and finally obtaining the lithium phosphate particles in nano-particle form and good in monodispersity. The method has the characteristics of mild reaction conditions, good equipment reliability, small volume of desired reactor, continuous and simple process, easy operation and the like. The particle size of the lithium phosphate particles prepared by the method ranges from 50 to 200nm; the lithium phosphate particles are controllable in size and even in distribution, and the yield of product is about 90%.

Description

Technical field [0001] The invention relates to the field of chemistry and chemical engineering, in particular to a method for preparing lithium phosphate nanoparticles by mixing an aqueous solution containing lithium and phosphorus using a microreactor. Background technique [0002] Lithium phosphate is a lithium salt of orthophosphoric acid, a colorless orthorhombic crystal, similar to olivine. Lithium phosphate has a melting point of 837°C, which is a high-temperature resistant material; at the same time, due to the advantages of no radioactivity, short light, long luminous efficiency, and low cost, it can be used as a raw material for the production of color phosphors; in terms of miniature compact power sources, nitrogen-containing phosphoric acid Lithium film is the most widely used electrolyte film in the research of all solid-state thin-film lithium batteries; it is used as a catalyst in the reaction of propylene oxide isomerization to propylene alcohol (230~270℃), and it...

Claims

the structure of the environmentally friendly knitted fabric provided by the present invention; figure 2 Flow chart of the yarn wrapping machine for environmentally friendly knitted fabrics and storage devices; image 3 Is the parameter map of the yarn covering machine
Login to View More

Application Information

Patent Timeline
no application Login to View More
Patent Type & Authority Applications(China)
IPC IPC(8): C01B25/30B82Y30/00
Inventor 骆广生毕佳颖王凯张同宝吕阳成
Owner TSINGHUA UNIV