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A kind of preparation method of attapulgite and its method for treating heavy metal wastewater

A technology of attapulgite and heavy metals, applied in chemical instruments and methods, other chemical processes, etc., can solve the problems of small adsorption capacity, unenvironmental protection, slow sedimentation rate, etc. The effect of promoting diffusion

Active Publication Date: 2018-03-16
NANJING INST OF ENVIRONMENTAL SCI MINIST OF ECOLOGY & ENVIRONMENT OF THE PEOPLES REPUBLIC OF CHINA +1
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

[0005] Aiming at the problems that existing attapulgite modification methods have problems such as unenvironmental protection, small adsorption capacity, slow sedimentation rate, and poor wastewater treatment effect, the present invention provides a new attapulgite preparation method and a method for treating heavy metal wastewater. Attapulgite / Fe 3 o 4 Composite materials are used in combination with high-efficiency coagulants, and the characteristics of the two processes are combined to make the modified attapulgite / Fe with saturated adsorption 3 o 4 The composite material accelerates the sedimentation under the action of the flocculant PAM to realize rapid solid-liquid separation; at the same time, the flocculant can absorb the heavy metal ions remaining in the water during the reaction process, further improving the removal efficiency of heavy metal ions and the decolorization effect of wastewater, and reducing the treatment of wastewater cost, worth promoting

Method used

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Examples

Experimental program
Comparison scheme
Effect test

Embodiment 1

[0038] A preparation method of novel attapulgite and a method for treating heavy metal wastewater, the steps of which are:

[0039] (1) 20g of attapulgite mineral powder and 100mL of deionized water were mixed in a volumetric flask, stirred at a speed of 150r / min for 45min, after standing for 3h, the supernatant liquid and the lower layer of sand were discarded to obtain the attapulgite purified soil Suspension, the attapulgite obtained after centrifugation of the suspension is placed in an oven to dry at 100°C, and set aside;

[0040] (2) Put the attapulgite after the above pretreatment into sulfuric acid with a concentration of 4mol / L, stir, heat at a constant temperature at 80°C for 1h, cool and let it stand to room temperature, rinse the attapulgite with deionized water, until The rinsing water is neutral, dried and ground at 100°C, and passed through a 200-mesh sieve to obtain acid-modified attapulgite;

[0041] (3) ferrous sulfate and ferric sulfate according to the mol...

Embodiment 2

[0046] 1. Prepare novel modified attapulgite / Fe according to the steps of (1)~(5) in Example 1 3 o 4 Composite material, the difference is: the mass ratio of attapulgite powder and deionized water in step (1) is 1:6, stirs 40min with the rotating speed of 200r / min, then leaves standstill 2.5h; In step (2) The concentration of the sulfuric acid solution is 3mol / L, and it is stirred at a constant temperature at 80°C; in step (3), n(Fe 2+ ):n(Fe 3+ )=1:4, strong (stirring speed is 350r / min) stirring 15min under the condition of constant temperature 70 ℃; The mass ratio of acid-modified attapulgite and iron ion solution, ammonia solution in step (4) is 1: 4:7, when dripping ammonia water, adjust the stirring speed to 120r / min, the ammonia water dripping speed is 2 drops / second, keep the pH of the solution at 12 during the dripping of ammonia water, and the aging time is 25min, then use anhydrous After washing with ethanol four times, the product was dried in a drying oven at 50...

Embodiment 3

[0049] 1. Prepare novel modified attapulgite / Fe according to the steps of (1)~(5) in Example 1 3 o 4 Composite material, the difference is: the mass ratio of attapulgite powder and deionized water in step (1) is 1:8, stirs 40min with the rotating speed of 200r / min, then leaves standstill 2.5h; In step (2) The concentration of the sulfuric acid solution is 5mol / L, and it is stirred at a constant temperature at 80°C; in step (3), n(Fe 2+ ):n(Fe 3+ )=1:5, strongly (stirring speed is 330r / min) stirs 13min under the condition of constant temperature 75 ℃; The mass ratio of acid-modified attapulgite and iron ion solution, ammonia solution in step (4) is 1: 5:8, when dripping ammonia water, adjust the stirring speed to 150r / min, the ammonia water dripping speed is 2 drops / second, keep the pH of the solution at 12 during the dripping of ammonia water, and the aging time is 23min, then use anhydrous After washing with ethanol four times, the product was dried in a drying oven at 55°...

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PUM

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Abstract

The invention discloses a preparation method of novel attapulgite and a method for treating heavy metal wastewater, belonging to the field of sewage treatment. In this method, attapulgite is used as raw material, and attapulgite is modified by pretreatment, acid modification, Fe3O4 loading, activation heat treatment and other processes. The modified attapulgite / Fe3O4 composite material has a large specific surface area and high adsorption capacity. It has the advantages of strong colloidal properties; the combination of modified attapulgite / Fe3O4 composite material and flocculation process to treat heavy metal-containing wastewater can effectively absorb heavy metals in water, and also has a good decolorization effect, with fast reaction rate and sedimentation separation With the advantages of fast speed and easy operation, it is a new, efficient and convenient treatment method for heavy metal wastewater.

Description

technical field [0001] The invention belongs to the field of sewage treatment, and more specifically relates to a method for preparing attapulgite and a method for treating heavy metal wastewater. Background technique [0002] In recent years, research on attapulgite as an adsorbent to treat industrial wastewater has been reported. Attapulgite is a hydrous magnesium-rich silicate clay mineral with excellent adsorption properties and certain ion exchange capacity. The activated attapulgite has a good adsorption and purification effect on heavy metal ions, and has the characteristics of high treatment efficiency and low adsorption cost. [0003] At present, for the preparation of modified materials of attapulgite, the interaction process between attapulgite and heavy metal ions, especially for Ni 2+ 、Cu 2+ , Pb 2+ The reaction mechanism of heavy metal ions has been thoroughly studied. Under normal circumstances, attapulgite, as a powder material, is difficult to exist in ...

Claims

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Application Information

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Patent Type & Authority Patents(China)
IPC IPC(8): B01J20/12
Inventor 张后虎路逸居赵克强赵泽华刘高杰蔡邦成
Owner NANJING INST OF ENVIRONMENTAL SCI MINIST OF ECOLOGY & ENVIRONMENT OF THE PEOPLES REPUBLIC OF CHINA