A kind of fluorine-containing polyimide copper clad laminate and its preparation method
A copper-clad laminate and polyimide technology, applied in the field of fluorine-containing polyimide copper-clad laminate and its preparation, can solve the problem of low heat resistance, inferior to aromatic heterocyclic polymer systems, and inability to meet high temperature requirements Conditional application and other issues to achieve high temperature resistance, excellent electrical and mechanical properties, and low cost
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Embodiment 1
[0034] Put 548 grams (1.0 moles) of 2,2-bis[4-(2,4-diaminoanilino)phenyl]hexafluoropropane and 22,000 grams of N,N-dimethylacetamide into the reaction kettle, at room temperature After stirring and dissolving, cool to below 1°C, add 196 grams (2.0 moles) of maleic anhydride, stir and react at 1°C for 0.5 hours, then add 310 grams (1.0 moles) of 3,3',4,4'-tetracarboxylic di Phenyl ether dianhydride was stirred and reacted for 1 hour to obtain 3254 g of component A, which was designated as A-1.
Embodiment 2
[0036] 548 grams (1.0 moles) of 2,2-bis[4-(2,4-diaminoanilino)phenyl]hexafluoropropane, 2890 grams of N,N-dimethylacetamide and 2000 grams of N-methyl -2-Pyrrolidone was put into the reaction kettle, stirred and dissolved at room temperature, cooled to below 1°C, added 156.8 grams (1.6 moles) of maleic anhydride, stirred and reacted at 5°C for 0.5 hours, then added 310 grams (1.0 moles) of 3, 3',4,4'-Tetracarboxydiphenyl ether dianhydride and 208 g (0.4 moles) of 2,2-bis[4-(3,4-dicarboxyphenoxy)phenyl]propane dianhydride, continued stirring After 2 hours of reaction, 6112.8 g of component A was obtained, which was designated as A-2.
Embodiment 3
[0038] 1093 grams (2.0 moles) of 2,2-bis[4-(2-trifluoromethyl-4-aminophenoxy)phenyl]propane and 2190 grams of N-methyl-2-pyrrolidone were placed in the reactor , after stirring and dissolving at room temperature, cooled to below 1°C, added 589 grams (1.9 moles) of 3,3',4,4'-tetracarboxydiphenyl ether dianhydride, stirred and reacted at 5°C for 2 hours, added 9.8 grams ( 0.1 mole) maleic anhydride, continue to react for 0.5 hour, obtain 3283 gram B components, denoted as B-1.
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