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A kind of fluorine-free fabric water repellent with branched structure and preparation method thereof

A branched structure and water-repellent technology, applied in the direction of repelling fibers to liquids, etc., can solve the problems of poor durability of non-fluorine water-repellent agents, overcome the environmental hazards, overcome the toxicity of bioaccumulation, and solve the problem of poor durability. Effect

Active Publication Date: 2018-06-01
BEIJING INSTITUTE OF TECHNOLOGYGY
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

[0004] Aiming at the problem of poor durability of fluorine-free water-repellent agents in the prior art, the object of the present invention is to provide a fluorine-free fabric water-repellent agent with a branched structure and its preparation method. The water-repellent agent described in the present invention has good durability, Significantly improved the water repellent effect, and the preparation method is simple

Method used

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Examples

Experimental program
Comparison scheme
Effect test

Embodiment 1

[0031] 23.1 parts of diisocyanate, 11.3 parts of long-chain alkane chain extender, 43.7 parts of organosiloxane, 5.8 parts of hydrophilic chain extender, 0.1 part of catalyst, 3.6 parts of neutralizing agent, 10.6 parts of end-capping agent, small molecule polyol 1.1 parts, 494 parts of water, 50 parts of acetone;

[0032] Step 1. Add 30.1g of aminopropyl-terminated polydimethylsiloxane and 0.75g of trihydroxypropane into the flask, and vacuumize at 100°C for 1 hour to remove moisture;

[0033] Step 2. When the temperature of the mixed solution in the flask drops to 40°C, add 15.9g IPDI and 0.068g T 12 , and then heated up to 75°C, stirred for 6h to obtain reaction system A;

[0034] Step 3. When the temperature of reaction system A drops to 50°C, add 7.8g of glyceryl monostearate, then raise the temperature to 75°C, and stir for 5 hours to obtain reaction system B;

[0035] Step 4. When the temperature of reaction system B drops to 35°C, add 4g diethanolamine and 34.4g acet...

Embodiment 2

[0039] 31.7 parts of diisocyanate, 19.5 parts of long-chain alkane chain extender, 23.7 parts of organosiloxane, 6.3 parts of hydrophilic chain extender, 0.1 part of catalyst, 9.2 parts of neutralizing agent, 8.2 parts of end-capping agent, small molecule polyol 1.2 parts, 120 parts of water, 30 parts of acetone;

[0040] Step 1. Add 16.8g of hydroxypropyl-terminated polydimethylsiloxane and 0.88g of trihydroxypropane into the flask, and vacuumize at 110°C for 1.5h to remove water;

[0041] Step 2. When the temperature of the mixed solution in the flask drops to 40°C, add 22.5g TDI and 0.07g TDI 12 , and then heated up to 90°C, stirred for 3h to obtain reaction system A;

[0042] Step 3. When the temperature of reaction system A drops to 45°C, add 13.8g of glyceryl monostearate, then raise the temperature to 85°C, and stir for 3 hours to obtain reaction system B;

[0043] Step 4. When the temperature of reaction system B drops to 40°C, add 4.5g of N-MDEA and 21.3g of acetone...

Embodiment 3

[0047] 28.1 parts of diisocyanate, 15.4 parts of long-chain alkane chain extender, 31.8 parts of organosiloxane, 8.1 parts of hydrophilic chain extender, 0.09 part of catalyst, 3 parts of neutralizing agent, 11.4 parts of end-capping agent, small molecule polyol 2.2 parts, 300 parts of water, 45 parts of acetone;

[0048] Step 1. Add 22.25g of silanol polydimethylsiloxane and 1.55g of pentaerythritol into the flask, and vacuumize at 90°C for 2 hours to remove moisture;

[0049] Step 2. When the temperature of the mixed solution in the flask drops to 50°C, add 19.7g HDI and 0.06g T 9 , and then heated to 98 ° C, stirred for 2 hours to obtain reaction system A;

[0050] Step 3. When the temperature of reaction system A drops to 50°C, add 10.8g of glyceryl distearate, then raise the temperature to 85°C, and stir for 3 hours to obtain reaction system B;

[0051] Step 4. When the temperature of reaction system B drops to 35°C, add 5.7g of triethanolamine and 31.5g of acetone, then ...

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PUM

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Abstract

The invention relates to a fluorine-free fabric water repellent with a branched structure and a preparation method of the fluorine-free fabric water repellent, and belongs to the technical field of textile printing and dyeing chemical industry. The water repellent has good durability and water repellent effect and comprises the following preparation steps: firstly drying and dewatering a mixed solution of organic siloxane and small-molecular polyalcohol under vacuum, adding diisocyanate and a catalyst after the mixed solution is cooled, then raising the temperature and enabling reaction to obtain a reaction system A; after the reaction system A is cooled, adding a long chain alkane chain extender, then raising the temperature and enabling reaction to obtain a reaction system B; after the reaction system B is cooled, firstly adding a hydrophilic chain extender and acetone for reaction, then adding an end-capping agent and continuously enabling reaction to obtain a reaction system C; after the reaction system C is cooled, firstly adding a neutralizing agent for neutralization, then adding water for emulsification and removing the acetone to obtain the fluorine-free fabric water repellent with the branched structure.

Description

technical field [0001] The invention relates to a fluorine-free fabric water-repellent agent with a branched structure and a preparation method thereof, in particular to an organosilicon-modified water-based polyurethane emulsion with a branched structure and a preparation method thereof, belonging to the technical field of textile printing and dyeing chemicals. Background technique [0002] The water-repellent finishing of fabrics can endow fabrics with excellent waterproof and breathable properties, so they are favored by the market. Fluorine-containing water repellents have better water repellency, but they will produce certain carcinogenic and bioaccumulative fluorocarbons during processing and use, especially the perfluorooctanoic acid and perfluorooctane sulfonate produced are potential carcinogens. Therefore, fluorine-free water repellent has become a current research hotspot. [0003] However, the long-chain alkane-based fluorine-free water-repellent agents and sil...

Claims

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Application Information

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Patent Type & Authority Patents(China)
IPC IPC(8): D06M15/653C08G18/65C08G18/61C08G18/32C08G18/12
CPCC08G18/12C08G18/3206C08G18/61C08G18/6517D06M15/564D06M15/653D06M2200/12C08G18/3275C08G18/3278
Inventor 葛震罗运军柴春鹏梁柱徐香玉
Owner BEIJING INSTITUTE OF TECHNOLOGYGY