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A kind of nano silver/epoxy resin high dielectric composite material and preparation method thereof

A technology of epoxy resin and composite materials, which is applied in the field of composite material manufacturing, can solve problems such as difficult to uniformly disperse resin due to agglomeration, large specific surface area of ​​nano-silver, large dielectric loss, etc., and achieve easy mass production, improved stability, and good dispersion Effect

Inactive Publication Date: 2019-11-26
WUHAN UNIV OF TECH +1
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

[0004] However, during the processing of this type of epoxy-based composite material, due to the small size and large specific surface area of ​​the nano-silver particles, it is easy to agglomerate and difficult to disperse evenly in the resin, resulting in a large dielectric loss.

Method used

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Examples

Experimental program
Comparison scheme
Effect test

Embodiment 1

[0022] Prepare a kind of high dielectric composite resin, the steps are as follows:

[0023] 1) Mix 1g N-(2-aminoethyl)-3-aminopropyltriethoxysilane, 5g silver nitrate, 0.5g 2,4,6-tris(dimethylaminomethyl)phenol, 1g o-benzene Diformaldehyde and 8.5g of methylhexahydrophthalic anhydride were added to 10g of E44 epoxy resin in turn, stirred at a high speed and dispersed evenly to obtain a mixed sol;

[0024] 2) Pour the mixed sol obtained in step 1) into an iron mold, place it in a blast drying oven and heat it up in stages to solidify, heat at a constant temperature of 60°C for 6 hours, then raise the temperature to 100°C and heat for 6 hours at a constant temperature, and then raise the temperature to a constant temperature of 150°C After heating for 4 hours, a nano-silver / epoxy resin high dielectric composite material is obtained.

[0025] The composite material prepared in this example has a dielectric constant of 8.2 and a dielectric loss of 0.023 at 1 kHz measured at room...

Embodiment 2

[0032] Prepare a kind of high dielectric composite resin, the steps are as follows:

[0033] 1) Mix 1g N-(2-aminoethyl)-3-aminopropyltrimethoxysilane, 5g silver oxalate, 0.2g tetraethylammonium bromide, 1g isophthalaldehyde, 8.5g methyltetrahydrophthalic anhydride Add in 10g E44 epoxy resin successively, stir at high speed and disperse evenly to obtain mixed sol;

[0034] 2) Pour the mixed sol obtained in step 1) into an iron mold, place it in a blast drying oven and heat it up in stages to solidify, heat at a constant temperature of 60°C for 4 hours, then raise the temperature to 100°C for 4 hours, and then raise the temperature to a constant temperature of 150°C After heating for 3 hours, the nano-silver / epoxy resin high dielectric composite material is obtained.

[0035] The composite material prepared in this example has a dielectric constant of 8.7 and a dielectric loss of 0.025 at 1 kHz measured at room temperature.

Embodiment 3

[0042] Prepare a kind of high dielectric composite resin, the steps are as follows:

[0043] 1) Mix 0.2g N-(2-aminoethyl)-3-aminopropyltrimethoxysilane, 1g silver acetate, 0.3g 2-ethyl-4-methylimidazole, 0.4g terephthalaldehyde, 8.5 1g methyl hexahydrophthalic anhydride is added in the 10g E51 epoxy resin successively, high-speed stirring disperses and obtains mixed sol;

[0044] 2) Pour the mixed sol obtained in step 1) into an iron mold, place it in a blast drying oven and heat it up in stages to solidify, heat at a constant temperature of 60°C for 2 hours, then raise the temperature to 100°C and heat for 2 hours at a constant temperature, and then raise the temperature to a constant temperature of 150°C After heating for 2 hours, a nano-silver / epoxy resin high dielectric composite material is obtained.

[0045] The composite material prepared in this example has a dielectric constant of 5.7 and a dielectric loss of 0.016 at 1 kHz measured at room temperature.

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Abstract

The invention relates to a nanometer silver / epoxy resin high dielectric composite material and a preparation method thereof. The high dielectric composite material is prepared by the following steps: (1) a complexing agent, Ag salt, a promoter, a reducing agent containing two aldehyde groups, and an acid anhydride curing agent are added into epoxy resin in order, uniform stirring is carried out, and mixed sol is obtained; (2) mixed soli obtained in the step (1) is poured into a die, the die is placed in a heating container, constant temperature heating is carried out at 60-90 DEG C for 2-6 hours, the temperature is raised to 100-130 DEG C, constant temperature heating is carried out for 2-6 hours, the temperature is raised to 150-180 DEG C and constant temperature heating is carried out for 2-4 hours, and the nanometer silver / epoxy resin high dielectric composite material is obtained. A silver mirror reaction is carried out for in-situ generation of nanometer silver particles with excellent conductivity, the particles have good dispersibility, in order to solve the problem of low dielectric constant or high dielectric loss existed in a fine conductive particle / epoxy resin system.

Description

technical field [0001] The invention belongs to the technical field of composite material manufacturing, and relates to a nano-silver / epoxy resin high-dielectric composite material and a preparation method thereof. Background technique [0002] After curing, epoxy resin has excellent mechanical properties, adhesive properties, corrosion resistance, and its curing shrinkage rate and linear expansion coefficient are small, dimensional stability and processability are good, and comprehensive performance is good. It is widely used in embedded capacitors. make. However, with the development of power electronic equipment in the direction of large capacity and high voltage, the requirements for the safety and operational reliability of capacitors are more stringent, and the requirements for the dielectric properties of epoxy resin are also getting higher and higher. [0003] Typically, pure epoxy resins have lower dielectric constant values. However, according to the Coulomb bloc...

Claims

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Application Information

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Patent Type & Authority Patents(China)
IPC IPC(8): C08L63/00C08K3/08
CPCC08K3/08C08K2003/0806C08K2201/001C08K2201/011C08L63/00
Inventor 晏石林鲍睿邵世东王若谷
Owner WUHAN UNIV OF TECH