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Method for preparing nickel-iron oxide by using Ni-Fe alloy melt

A technology of oxides and alloys, applied in chemical instruments and methods, nickel compounds, inorganic chemistry, etc., can solve the problems of high energy consumption and cost, long production process, etc., and achieve short process, low raw material cost, and reduced energy consumption Effect

Active Publication Date: 2020-05-19
JIANGXI UNIV OF SCI & TECH
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

[0003] The main purpose of the present invention is to provide a method for preparing ferronickel oxide by using Ni-Fe alloy melt, aiming to solve the technical problems of long production process, high energy consumption and high cost in the existing preparation method of ferronickel oxide

Method used

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Examples

Experimental program
Comparison scheme
Effect test

Embodiment 1

[0025] The temperature of the Ni-Fe alloy melt is controlled at 650°C, the Ni content is 51wt%, stirred by a mechanical paddle, and spray granulated to obtain Ni-Fe particles with a particle size of about 460 μm;

[0026] Through 10h zirconia ball milling (dry milling) and sieving to obtain Ni-Fe powder with a particle size of ≤25 μm, the yield is 60%, and the coarse particles are added to the next ball mill;

[0027] The Ni-Fe powder is fluidized and roasted at 450°C in oxygen-enriched air with an oxygen concentration of 45% for 8 hours, and the particle size of the obtained nickel-iron oxide is about 30 μm, with good particle size uniformity.

[0028] After the nickel-iron oxide is prepared as an oxygen evolution electrode, in 1M KOH solution, the current density is 10mA / cm -2 , the oxygen evolution overpotential is about 405mV.

Embodiment 2

[0030] The temperature of the Ni-Fe alloy melt is controlled at 630°C, the Ni content is 42wt%, the mechanical paddle is stirred, and the Ni-Fe particles with a particle size of about 520 μm are obtained by spray granulation;

[0031] Through 12h zirconia ball milling (dry milling) and sieving to obtain Ni-Fe powder with a particle size of ≤25 μm, the yield is 55%;

[0032] The Ni-Fe powder is fluidized and roasted at 430°C in oxygen-enriched air with an oxygen concentration of 45% for 8 hours, and the particle size of the obtained nickel-iron oxide is about 32 μm, with good particle size uniformity.

[0033] After the nickel-iron oxide is prepared as an oxygen evolution electrode, in 1M KOH solution, the current density reaches 10mA / cm -2 , the oxygen evolution overpotential is about 423mV.

Embodiment 3

[0035] The temperature of the Ni-Fe alloy melt is controlled at 650°C, the Ni content is 49wt%, the mechanical paddle is stirred, and the Ni-Fe particles with a particle size of about 430 μm are obtained by spray granulation;

[0036] Obtain Ni-Fe powder with a particle size of ≤25 μm by 8h zirconia ball milling (dry milling) and sieving, with a yield of 65%;

[0037] The Ni-Fe powder is fluidized and roasted at 350°C in oxygen-enriched air with an oxygen concentration of 50% for 8 hours, and the particle size of the obtained nickel-iron oxide is about 28 μm, with good particle size uniformity.

[0038] After the nickel-iron oxide is prepared as an oxygen evolution electrode, in 1M KOH solution, the current density reaches 10mA / cm -2 , the oxygen evolution overpotential is about 398mV.

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Abstract

The invention discloses a method of using Ni-Fe alloy melt to prepare iron-nickel oxide, comprising: subjecting nickel oxide ore to reduction smelting by an electric furnace, performing refining desulfurizing, performing converter blowing and cleaning to obtain Ni-Fe alloy melt, and subjecting the Ni-Fe alloy melt to spray granulating to obtain Ni-Fe alloy particles; subjecting the Ni-Fe alloy particles to further ball milling, and screening to obtain Ni-Fe alloy powder having particle size of not more than25 mu m; subjecting the Ni-Fe melt powder to fluidized oxidizing roasting to prepare iron-nickel oxide. The method herein directly utilizing intermediates of a nickel oxide ore smelting process has the advantages of short process, low energy consumption, low material price, and good environmental friendliness.

Description

technical field [0001] The invention relates to the technical field of non-ferrous metal metallurgy, in particular to a method for preparing ferronickel oxide by using a Ni-Fe alloy melt. Background technique [0002] Nickel-iron oxide is widely used in water splitting, molten salt electrolysis and other fields, and is a noble metal-free, highly active catalyst / electrode material. At present, the preparation method of nickel-iron oxide is mainly to use oxalic acid / alkali to precipitate the aqueous solution of nickel and iron, and then calcinate the mixed precipitation of nickel oxalate and iron oxalate (nickel hydroxide and iron hydroxide), so as to prepare nickel-iron oxide. This preparation method needs to obtain the aqueous solution of nickel and iron first, the production process is long, and the energy consumption and cost are high. Contents of the invention [0003] The main purpose of the present invention is to provide a method for preparing ferronickel oxide by u...

Claims

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Application Information

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Patent Type & Authority Patents(China)
IPC IPC(8): C01G53/00C25B11/06
CPCC01G53/00C01P2004/61C01P2006/40C25B11/077
Inventor 钟晓聪徐志峰王瑞祥刘志楼陈芳会
Owner JIANGXI UNIV OF SCI & TECH