A kind of silicon carbon composite material, its preparation method and application
A silicon-carbon composite material and nano-silicon technology, which is applied to active material electrodes, structural parts, electrical components, etc., can solve the problem of high cost of negative electrode silicon-carbon materials, and achieve the effects of high consistency, low cost and simple preparation process.
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Embodiment 1
[0057] A method for preparing a silicon-carbon composite material comprises the steps of:
[0058] (1) Preparation of porous nano-silicon:
[0059] Use a disc chipper to eliminate scrapped solar silicon panels to a particle size of 800 μm, then sand-grind and classify by a mechanical mill to obtain nano-silicon with a particle size of 100 nm, and then use ethanol and deionized water (volume ratio 1 : 1) carry out ultrasonic cleaning, filter, then transfer to 0.1mol / L hydrofluoric acid and soak for 12h, and use deionized water to clean, dry to obtain porous nano-silicon;
[0060] (2) Preparation of silicon-carbon composite materials:
[0061] Add 1g of vinyltriethoxysilane to 20mL of carbon tetrachloride organic solvent to form a solution, then add 3g of porous nano-silicon, 1g of polyethylene glycol and 1g of silicon chloride, mix well, ultrasonically disperse for 6h, and then filter Solid product and transfer to tube furnace;
[0062] Calcination: In an inert atmosphere, h...
Embodiment 2
[0065] A method for preparing a silicon-carbon composite material comprises the steps of:
[0066] (1) Preparation of porous nano-silicon:
[0067] Use a disc chipper to eliminate scrapped solar silicon panels to a particle size of 500 μm, then sand-grind and classify by a mechanical mill to obtain nano-silicon with a particle size of 50 nm, and then use ethanol and deionized water (volume ratio 1:1) Ultrasonic cleaning, filtering, then transferring to 0.5mol / L hydrofluoric acid for immersion for 1h, and cleaning with deionized water, drying to obtain porous nano-silicon;
[0068] (2) Preparation of silicon-carbon composite materials:
[0069] Add 0.5g of vinyltrimethoxysilane to 50mL of N-methylpyrrolidone organic solvent to form a solution, then add 1g of porous nano-silicon, 0.5g of polyvinyl alcohol and 0.5g of silicon tetrabromide and mix well, then ultrasonically disperse for 1h , after which the solid product was filtered and transferred to a tube furnace;
[0070] C...
Embodiment 3
[0072] A method for preparing a silicon-carbon composite material comprises the steps of:
[0073] (1) Preparation of porous nano-silicon:
[0074] Use a disc chipper to eliminate scrapped solar silicon panels to a particle size of 1000 μm, then sand-grind and classify through a mechanical mill to obtain nano-silicon with a particle size of 200 nm, and then use ethanol and deionized water (volume ratio) successively 1:1) ultrasonically cleaned, filtered, then transferred to 0.1mol / L hydrofluoric acid and soaked for 24 hours, washed with deionized water, and dried to obtain porous nano-silicon;
[0075] (2) Preparation of silicon-carbon composite materials:
[0076] Add 2g of vinyl tris(β-methoxyethoxy)silane to 200mL N,N-dimethylformamide organic solvent to form a solution, then add 5g of porous nano-silicon, 2g of polyvinyl alcohol and 2g of chloride After the silicon is evenly mixed, ultrasonically disperse for 12 hours, then filter and transfer to a tube furnace;
[0077...
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