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Preparation method of polyimide intercalation grafted magnesium hydroxide flame retardant

A technology of polyimide and magnesium hydroxide is applied in the field of preparation of polyimide intercalation grafted magnesium hydroxide flame retardant, which can solve the problems of hydrogen chloride generation and large amount of smoke, and achieves low cost, three wastes and the like. Less and more productive effects

Pending Publication Date: 2021-01-22
SHENZHEN AIMSEA IND
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

Halogen-containing polymers are widely used in traditional flame retardants. Once burned, the amount of smoke will be greater, and halogen gases such as hydrogen chloride will be produced.

Method used

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Examples

Experimental program
Comparison scheme
Effect test

Embodiment 1

[0025] First prepare the polyimide prepolymer: at room temperature, first dissolve 1 part by weight of 3,3'4,4'-benzophenone tetracarboxylic dianhydride in 7 parts by weight of dimethyl sulfoxide to prepare into solution A, then 10 parts by weight of triphenylmethane triisocyanate and 5 parts by weight of m-phenylenediamine are dissolved in 25 parts by weight of dimethyl sulfoxide to prepare solution B, and solution A and B is mixed, and then under the condition of nitrogen protection, the reaction vessel is added to the oil bath for reaction, magnetically stirred and the reaction temperature is 70°C, the reaction time is 30min, the rotation speed is 1500r / min, and then the temperature is raised to 140°C, The reaction time is 30min. After the reaction is over, stop heating, and leave the reaction solution for 3h to cool to room temperature to obtain a polyimide prepolymer;

[0026] Then prepare modified nano-magnesium hydroxide: first prepare a silane coupling agent solution w...

Embodiment 2

[0030] First prepare the polyimide prepolymer: at room temperature, first dissolve 1 part by weight of 3,3'4,4'-benzophenone tetracarboxylic dianhydride in 7 parts by weight of dimethyl sulfoxide to prepare into solution A, then 10 parts by weight of diphenylmethane diisocyanate MDI, 5 parts by weight of m-phenylenediamine are dissolved in 25 parts by weight of dimethyl sulfoxide to prepare solution B, and solution A and B is mixed, and then under the condition of nitrogen protection, the reaction vessel is added to the oil bath for reaction, magnetically stirred and the reaction temperature is 70°C, the reaction time is 30min, the rotation speed is 1500r / min, and then the temperature is raised to 140°C, The reaction time is 30min. After the reaction is over, stop heating, and leave the reaction solution for 3h to cool to room temperature to obtain a polyimide prepolymer;

[0031] Then prepare modified nano-magnesium hydroxide: first prepare a silane coupling agent solution wi...

Embodiment 3

[0035] First prepare the polyimide prepolymer: at room temperature, first dissolve 1 part by weight of 3,3'4,4'-benzophenone tetracarboxylic dianhydride in 7 parts by weight of dimethyl sulfoxide to prepare into solution A, then 10 parts by weight of diphenylmethane diisocyanate MDI and 5 parts by weight of p-phenylenediamine are dissolved in 25 parts by weight of dimethyl sulfoxide to prepare solution B, and solution A and B is mixed, and then under the condition of nitrogen protection, the reaction vessel is added to the oil bath for reaction, magnetically stirred and the reaction temperature is 70°C, the reaction time is 30min, the rotation speed is 1500r / min, and then the temperature is raised to 140°C, The reaction time is 30min. After the reaction is over, stop heating, and leave the reaction solution for 3h to cool to room temperature to obtain a polyimide prepolymer;

[0036] Then prepare modified nano-magnesium hydroxide: first prepare a silane coupling agent solution...

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Abstract

The invention discloses a preparation method of a polyimide intercalation grafted magnesium hydroxide flame retardant. The preparation method comprises the following steps: mixing a polyimide prepolymer with modified nano magnesium hydroxide in a solvent, heating and refluxing under the action of a catalyst, cooling and drying; and performing superfine grinding to obtain the uniform flame retardant. The flame retardant integrates the advantages of flame retardance of magnesium hydroxide and polyimide, has a synergistic flame retardant effect and a remarkable flame retardant effect, and has a good application prospect.

Description

technical field [0001] The invention relates to a preparation method of a polyimide intercalation grafted magnesium hydroxide flame retardant, belonging to the technical field of flame retardant preparation. Background technique [0002] Flame retardants are divided into two categories: additive flame retardants and reactive flame retardants, most of which contain halogen and phosphorus. Halogen-containing polymers are widely used in traditional flame retardants. Once burned, the amount of smoke will be greater, and halogen gases such as hydrogen chloride will be produced. Contents of the invention [0003] Due to the low toxicity of inorganic flame retardants, it is fully in line with the current general trend of flame retardants to be environmentally friendly. However, since inorganic flame retardants (such as aluminum hydroxide, magnesium hydroxide, zinc borate, etc.) are fillers, they are added in a large amount in the resin, which often affects the processing perform...

Claims

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Application Information

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Patent Type & Authority Applications(China)
IPC IPC(8): C08K9/06C08K3/22C08L79/08C08L27/06
CPCC08K3/22C08K9/06C08K2003/2224C08K2201/011C08L27/06C08L79/08C08L2201/02
Inventor 严晴严一丰
Owner SHENZHEN AIMSEA IND