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Preparation method of super-hydrophobic full-biomass-based oil-water separation material

A technology for separating materials and biomass, which is applied in the field of preparation of superhydrophobic all-biomass-based oil-water separation materials, which can solve the problem of high oil absorption, achieve the effects of enhanced adsorption performance, simplified production process, and enhanced mechanical strength

Pending Publication Date: 2021-06-04
SICHUAN UNIV
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

This method has simple preparation process, high oil absorption and will not cause secondary pollution to the environment

Method used

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Examples

Experimental program
Comparison scheme
Effect test

Embodiment 1

[0026] Take 5 g sodium carboxymethylcellulose and 5 g sodium periodate respectively, and make 150 ml solution respectively, 50 o Put it in a water bath and stir it at a constant speed until it is completely dissolved, then mix it and adjust the pH to 3, 50 o The reaction was carried out at C for 4 h, and the reaction solution was poured into absolute ethanol for precipitation. The obtained white precipitate was washed 5 times with absolute ethanol, and then the precipitate was configured into a solution and put into a dialysis bag for dialysis for 5 days. After dialysis, the solution was freeze-dried to obtain bisaldehyde carboxymethylcellulose. Mix the dialdehyde carboxymethyl cellulose solution with a mass fraction of 0.1% and the collagen solution with a mass fraction of 0.8%, wherein the dry weight ratio of dialdehyde carboxymethyl cellulose to collagen is 1:8, pour the mixed solution into the mold at –20 o C for 3 days, and then freeze-dried in a freeze dryer for 2 days...

Embodiment 2

[0029] Take by weighing 5 g of sodium carboxymethylcellulose, join in the reactor that stirring device, thermometer are housed, then add 300ml distilled water, the sodium periodate of 7.625 g, the pH value is adjusted to 2, at 45 oStir and react in a water bath at about C for about 4 h. After the reaction, add acetone 2 times the volume of the reaction solution to precipitate dialdehyde carboxymethyl cellulose, and filter after the precipitation is complete. After filtration, washing, drying and crushing, dialdehyde carboxymethyl cellulose is obtained. Weigh 1 g collagen dry product and add 100 ml of water, 5 o Stir continuously at about C for about 8 h to obtain a collagen solution with a concentration of about 1%. At the same time, weigh 0.05 g of dialdehyde carboxymethyl cellulose and add it to 100 ml of water, 75 o Heating in a water bath at about C and stirring continuously for about 0.5 h to obtain a carboxymethyl cellulose solution with a concentration of about 0.05% ...

Embodiment 3

[0032] Take by weighing 5 g of sodium carboxymethyl cellulose, join in the reactor that stirring device, thermometer are housed, then add 300ml distilled water, the sodium periodate of 6.25 g, the pH value is adjusted to 1.5, at 45 o Stir and react in a water bath at about C for about 5 h. After the reaction, add 2 times the volume of absolute ethanol to precipitate dialdehyde carboxymethyl cellulose, and filter after the precipitation is complete. After filtration, washing, drying and crushing, dialdehyde carboxymethyl cellulose is obtained. Weigh 1 g collagen dry product and add 100 ml of water, 5 o Stir continuously at about C for about 8 h to obtain a collagen solution with a concentration of about 1%. At the same time, weigh 0.01 g of dialdehyde carboxymethyl cellulose and add it to 100 ml of water, 75 o Heat in a water bath at about C and keep stirring for about 0.5 h to obtain a dialdehyde carboxymethyl cellulose solution with a concentration of about 0.01%. At room ...

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Abstract

The invention provides a preparation method of a super-hydrophobic full-biomass-based oil-water separation material. The method mainly comprises the following two preparation processes: (1) preparing a dialdehyde carboxymethyl cellulose cross-linking agent, uniformly mixing the dialdehyde carboxymethyl cellulose cross-linking agent with a collagen solution, freezing for 1-10 days under the low-temperature condition of -50 to 0 DEG C, and freeze-drying for 1-2 days to prepare dialdehyde carboxymethyl cellulose-collagen aerogel; (2) dissolving carnauba wax and beewax in ethyl acetate according to a certain proportion to prepare a mixed wax solution, then soaking the aerogel prepared in the step (1) in the wax solution for 110 minutes, taking out aerogel and airing aerogel, and repeating the operation for 35 times to obtain the super-hydrophobic full-biomass-based oil-water separation material. The raw material collagen, the cross-linking agent dialdehyde carboxymethyl cellulose and the hydrophobic modifier natural grease used in the method are all environment-friendly biomass materials, so secondary pollution is avoided; the prepared oil-water separation material has good mechanical properties and oil-water separation capability, can be applied to the field of treatment of oily wastewater, and has good market application prospects.

Description

technical field [0001] The invention belongs to the field of environmental protection where all biomass materials are used for oily wastewater treatment, and specifically relates to a preparation method of a superhydrophobic all biomass-based oil-water separation material. Background technique [0002] With the rapid development of modern industry, a large amount of organic pollution and oily wastewater are produced, and their unreasonable discharge not only has an irreversible impact on the environment, but also threatens human health and food safety. Therefore, how to continuously supply pure water has become one of the main challenges facing mankind. Aiming at the environmental problems caused by organic pollution and industrial oily wastewater, the traditional measures to separate oil and water are mainly physical methods (including gravity centrifugation, electrocoagulation, etc.) and chemical methods (in-situ combustion, chemical solidification, etc.). In the case of ...

Claims

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Application Information

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IPC IPC(8): C08J9/42C08J9/28C08L89/00C08L1/28C08L91/06B01D17/022
CPCC08J9/42C08J9/0061C08J9/28B01D17/0202C08J2389/00C08J2401/28C08J2491/06C08J2201/0484C08J2205/026
Inventor 林炜张丰腾王春华何雨静
Owner SICHUAN UNIV