Core-shell structure negative electrode material, preparation method thereof and lithium ion battery
A lithium-ion battery, core-shell structure technology, applied in negative electrodes, battery electrodes, secondary batteries, etc., can solve the problems of product performance to be further improved, high cost, etc., and achieve low price, good stability, and simple preparation. Effect
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Embodiment 1
[0059] This embodiment provides a method for preparing a negative electrode material with a core-shell structure, the specific steps of which are:
[0060] (1) Prepare ZnO powder. Dissolve 0.08g of zinc acetate in 50mL of diethylene glycol solution, stir for 12h, then pour it into a polytetrafluoroethylene autoclave, and keep it warm at 120°C for 10h. After cooling to room temperature, centrifuge 3 times with alcohol and deionized water respectively at 8000 rpm. Then the obtained precipitate was vacuum-dried at 80°C for 12h;
[0061] (2) Preparation of ZIF-8. Weigh 1.4g zinc nitrate hexahydrate Zn(NO 3 ) 2 .6H 2 O was dissolved in 100 mL methanol. Weigh 3.087g of 2-methylimidazole and dissolve it in 100mL of methanol. Add the methanol solution of 2-methylimidazole to the methanol solution of zinc nitrate dropwise and keep stirring, and the time for adding the methanol solution of 2-methylimidazole is 0.9h;
[0062] (3) then slowly pour the ZnO powder (0.05g) in the ste...
Embodiment 2
[0069] This embodiment provides a method for preparing a negative electrode material with a core-shell structure, the specific steps of which are:
[0070] (1) Prepare ZnO powder. Dissolve 0.08g of zinc acetate in 50mL of diethylene glycol solution, stir for 12h, then pour it into a polytetrafluoroethylene autoclave, and keep it warm at 120°C for 10h. After cooling to room temperature, centrifuge 3 times with alcohol and deionized water respectively at 8000 rpm. Then the obtained precipitate was vacuum-dried at 80°C for 12h;
[0071] (2) Preparation of ZIF-8. Weigh 1.4g zinc nitrate hexahydrate Zn(NO 3 ) 2 .6H 2 O was dissolved in 100 mL methanol. Weigh 3.087g of 2-methylimidazole and dissolve it in 100mL of methanol. Add the methanol solution of 2-methylimidazole to the methanol solution of zinc nitrate dropwise and keep stirring, and the time for adding the methanol solution of 2-methylimidazole is 0.9h;
[0072] (3) then slowly pour the ZnO powder (0.05g) in the ste...
Embodiment 3
[0079] This embodiment provides a method for preparing a negative electrode material with a core-shell structure, the specific steps of which are:
[0080](1) Prepare ZnO powder. Dissolve 0.08g of zinc acetate in 50mL of diethylene glycol solution, stir for 12h, then pour it into a polytetrafluoroethylene autoclave, and keep it warm at 120°C for 10h. After cooling to room temperature, centrifuge 3 times with alcohol and deionized water respectively at 8000 rpm. Then the obtained precipitate was vacuum-dried at 80°C for 12h;
[0081] (2) Preparation of ZIF-8. Weigh 1.4g zinc nitrate hexahydrate Zn(NO 3 ) 2 .6H 2 O was dissolved in 100 mL methanol. Weigh 3.087g of 2-methylimidazole and dissolve it in 100mL of methanol. Add the methanol solution of 2-methylimidazole to the methanol solution of zinc nitrate dropwise and keep stirring, and the time for adding the methanol solution of 2-methylimidazole is 0.9h;
[0082] (3) then slowly pour the ZnO powder (0.05g) in the step...
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