Process for synthesizing CePO4 nano-material with monocline structure
A nanomaterial and synthesis method technology, applied in the field of rare earth phosphate nanomaterials, can solve the problems of unfavorable large-scale production and application, raw materials cannot be reused, and high raw material prices, and achieves low raw material prices, easy industrial production, and simple preparation methods. Effect
Inactive Publication Date: 2008-12-10
UNIV OF SCI & TECH BEIJING
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Problems solved by technology
These methods mainly have shortcomings such as high synthesis temperature or non-recyclable raw materials, high raw material prices, and low conversion rates, which are not conducive to large-scale production and application.
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Embodiment 1
[0012] Take 0.0434g Ce(NO 3 ) 3 ·6H 2 O was dissolved in 10mL of distilled water, and 10mL of 6mol / L H 3 PO 4 , stirred for 20mim, and transferred to the reaction kettle. React at 100°C for 6 hours, wash with distilled water and absolute ethanol three times, and dry at 60°C to obtain light green powder.
Embodiment 2
[0014] Take 0.0868g Ce(NO 3 ) 3 ·6H 2 O was dissolved in 10mL of distilled water, and 10mL of 6mol / L H 3 PO 4 , stirred for 20mim, and transferred to the reaction kettle. React at 160°C for 6 hours, wash with distilled water and absolute ethanol three times, and dry at 60°C to obtain light green powder.
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The invention belongs to the field of rare earth phosphate nanometer material, and relates to a method for synthesizing a monoclinic structured CePO4 nanometer material, in particular to a method for synthesizing a monoclinic structured CePO4 nanometer material by adopting low temperature, non-template and recyclable raw material H3PO4; Ce(NO3)3.6H2O is taken as a cerium source and dissolved in water, added with H3PO4 to lead the molar ratio of PO4<3->Ce<3+> in the reactant to be 800-300, stirred for 20-30min to cause thorough mixing, then the mixture is transferred into a hydrothermal reaction kettle, and allowed to react for 6-8h at 100-160 DEG C to obtain monoclinic structured CePO4 nanometer powder. The preparation method of the invention is simple, the equipment is simple, the synthesis temperature is low, the raw material H3PO4 is recyclable and cheap, and no expensive surfactant is needed as the template; the method is characterized by no use of organic solvent, no environmental pollution, energy saving, high conversion ratio, and being easy for industrialized production and the like, and has the advantages of effective reduction of the synthesis temperature and good repeatability, and the method is an ideal pollution-free process.
Description
Technical field: [0001] The invention belongs to the field of rare earth phosphate nanomaterials and relates to a monoclinic structure CePO 4 The synthesis method of nanomaterials, especially the use of low temperature, non-template agent and raw material H 3 PO 4 Reusable Synthetic Monoclinic CePO 4 methods for nanomaterials. Background technique: [0002] CePO 4 It has broad application prospects in ion exchange, fluorescent materials, conductor materials, catalyst materials, etc. Due to its good chemical stability and thermal stability, it has been widely used in various lighting and display instruments. Especially monoclinic structure CePO 4 It has good thermal stability, and its melting temperature is close to 2000°C. It is a good heat-resistant and ceramic material; it has recently been used as a proton-conducting membrane in hydrogen fuel cells; it has attracted much attention as a nuclear waste storage material. Simultaneously nanostructured CePO 4 With a hig...
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IPC IPC(8): C01B25/26C01G17/00C30B29/14C30B7/10
Inventor 于然波宝金荣杨晓丹张家芸陈俊邢献然
Owner UNIV OF SCI & TECH BEIJING
