Heat curable resin composition, overcoating agent for flexible circuit board, and surface protective film
A resin composition, thermosetting technology, applied in printed circuit, printed circuit, printed circuit manufacturing, etc., can solve the problem that the wiring pattern has not been studied in detail, and achieve excellent long-term reliability, not easy to warp and deform, and tightness excellent effect
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[0195] The following examples are given to illustrate the present invention, but the present invention is not limited by these examples.
Synthetic example 1
[0197] Synthesis example of carboxyl group-containing polyurethane resin (A-1) using polycarbonate diol
[0198] In a reaction vessel equipped with a stirring device, a thermometer, and a condenser, C-1065N (polycarbonate diol manufactured by Kuraray Co., Ltd.) was added as polycarbonate diol (polyol component (b)), and the raw material diol molar ratio was 1,9-nonanediol: 2-methyl-1,8-octanediol = 65:35, molecular weight 991) 70.7 g, 2,2-dimethylol as a dihydroxy compound (c) having a carboxyl group 13.5 g of butyric acid (manufactured by Nippon Kasei Co., Ltd.) and 128.9 g of diethylene glycol ethyl ether acetate (manufactured by Daicel Chemical Co., Ltd.) as a solvent were all dissolved in the solvent at 90°C.
[0199] The temperature of the reaction liquid was lowered to 70° C., and 42.4 g of Desmogel-W (manufactured by Sumitomo Bayer Uletan Co., Ltd.) was added dropwise through the dropping funnel over 30 minutes as the polyisocyanate (a).
[0200] After completion of ...
Synthetic example 2
[0203] Synthesis example of carboxyl group-containing polyurethane resin (A-2) using polybutadiene diol
[0204] In the reaction container that has stirring device, thermometer, condenser, add the commercial product named G-1000 (Nippon Soda Co., Ltd.) as polybutadiene diol (polyol component (b)) 646.5g, as having 103.8 g of 2,2-dimethylolbutyric acid (manufactured by Nippon Kasei Co., Ltd.) and 989.5 g of diethylene glycol ethyl ether acetate (manufactured by Daicel Chemical Co., Ltd.) as a solvent of the dihydroxy compound (c) of the carboxyl group, All starting materials were dissolved in solvent at 90°C.
[0205] The temperature of the reaction liquid was lowered to 70° C., and 217.3 g of Takenet 600 (manufactured by Mitsui Takeda Chemical Co., Ltd.) was dropped as polyisocyanate (a) over 30 minutes through the dropping funnel.
[0206] After completion of the dropwise addition, the reaction was carried out at 80°C for 1 hour, at 90°C for 1 hour, and at 100°C for 1.5 ho...
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