Method for preparing urethane chain rod-type high durable end-group polyene-bond photocuring prepolymer
A light-curing prepolymer, high weather resistance technology, applied in the field of ultraviolet light-curing resin, can solve the problems of complex preparation method, low toughness of hyperbranched ultraviolet light-curing resin, difficult control of reaction process, etc., and achieves high reactivity and high hardness. , the effect of good flexibility
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Embodiment 1
[0018] 20 g of pyromellitic acid monohydroxypropyl ester was added in 5 batches. Add 50g of glycidyl methacrylate, 0.2g of 4-methoxyphenol, 0.36g of triethylamine, and reaction temperature of 80°C into the flask. Add pyromellitic acid monohydroxypropyl once every 30 minutes. Then increase the temperature to 90°C, and test the acid value of the system. If it reaches 3mgKOH / g, stop the reaction and record it as intermediate product B.
[0019] 50 g of hexamethylene diisocyanate was put into a four-necked flask, 50 g of water-removed polyether diol (molecular weight 400) and 0.25 g of dibutyltin dilaurate were added to the dropping funnel, and mixed. The dropping time is controlled at 90 minutes, and the reaction temperature is controlled at 60-70°C. When the molar amount of isocyanate groups in the system is 50% of the added molar amount of hexamethylene diisocyanate, the reaction is stopped.
[0020] The above-mentioned reaction intermediate product B containing three double bonds ...
Embodiment 2
[0022] 20 g of pyromellitic acid monohydroxypropyl ester was added in 5 batches. Add 50g of glycidyl methacrylate, 0.2g of 4-methoxyphenol, 0.36g of triethylamine, and reaction temperature of 80℃ in the flask. Add 4g of pyromellitic acid monohydroxypropyl at intervals, and add all of them. Then raise the temperature to 90°C, and test the acid value of the system. If it reaches 3mgKOH / g, stop the reaction.
[0023] Add 16.8g of hexamethylene diisocyanate into another four-necked flask, mix the above-mentioned reaction intermediate product containing three double bonds and one hydroxyl group after water removal treatment with 0.5g of dibutyltin dilaurate, and mix it by dropping The method is added to the flask, the dropping time is 60-90min, the reaction temperature is controlled between 60-70°C, and when the content of the isocyanate group in the system is less than 2%, the reaction ends and a white viscous liquid is obtained.
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