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A kind of preparation method of alkyl glycoside

A technology for alkyl glycosides and glucose, applied in the field of preparation of alkyl glycosides, can solve the problems of complex process, difficult separation of neutralized salts, long process flow, etc., and achieves the effects of expanding application area, low production cost and reducing difficulty

Active Publication Date: 2015-11-18
ZANYU TECH GRP CO LTD +1
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

Therefore, in order to obtain APG products with better color and luster, many patents are developed around the above problems: (1) Using new catalysts, such as immobilized heteropolyacid catalysts (CN101239999A), ionic liquid catalysts (CN101787058A), sulfonic acid resins (EP0378710), heteropolyacid (US4874852), etc., but many catalysts are expensive; (2) improve dealcoholization technology, such as adopting new dealcoholization system (CN201587917U), extraction treatment before dealcoholization (CN1048253C), extraction dealcoholization ( CN200410026350.1, US5512666), adding diluent to dealcoholize (CN1045261C), etc., but the process is complicated, the process is long, and it will cause a certain loss of active substances; (3) Improve neutralization or bleaching technology, such as using alkali metal oxide powder Neutralization (CN1213054C), magnesium hydroxide neutralization (JP92120090), magnesium oxide assisted decolorization (US5554740), etc., but the catalyst cannot be reused, the neutralization salt is not easy to separate, and the use of APG products is limited by the residual alkali metal
Therefore, although the above methods have certain effects, they have certain limitations.

Method used

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Examples

Experimental program
Comparison scheme
Effect test

Embodiment 1

[0018] In a 2000mL high-shear stirring stainless steel reactor with a reflux device, add 750Kg of fatty alcohol and 300Kg of glucose, maintain a vacuum of -95KPa and raise the temperature to 110°C for half an hour, then add NaHSO 4 1.5kg, the stirring speed is 150r / min, and the temperature is raised to 115°C, the mixer is turned on, and the vacuum reaction is maintained for 2 hours. At 130°C and 120 Pa absolute pressure, fatty alcohol is removed; 450Kg of water is added to dilute the product to a 50% solution; NaOH solution is added to adjust the pH value to 10, and the product is discharged to obtain an alkyl glycoside product. The measured absorbance of the product at a wavelength of 420nm is 0.012 (the absorbance of corrected distilled water is 0), the residual sugar is 0.07%, and the residual alcohol is 0.45%.

Embodiment 2

[0020] In a 20-ton reaction kettle, add 3 tons of anhydrous glucose and 12 tons of higher alcohols, start stirring, and raise the temperature to 105°C under a vacuum of -98KPa to vacuumize for 1 hour. Add 15Kg of anhydrous potassium bisulfate, heat up to 115°C, maintain absolute pressure at -98KPa, stir and react in vacuum for 2 hours, then filter, and the filtrate is adsorbed by resin to remove residual H + , and then the above-mentioned filtrate is sent to a thin-film evaporator, and the temperature in the kettle is controlled at 120° C. to dealcoholize under the condition of an absolute pressure of 100 Pa and a vacuum degree. After dealcoholization, the temperature was lowered to 80°C, and 4 tons of distilled water was added to adjust the solid content to 60% to obtain a light yellow aqueous solution of alkyl glycosides. Put the above alkyl glucoside solution into the bleaching kettle, add 50 kg of 30% hydrogen peroxide, stir and heat at a constant temperature of 50°C-70°C ...

Embodiment 3

[0022] In a 10-ton reactor, add 1.3 tons of anhydrous glucose, recover 200Kg of glucose, and 6 tons of higher alcohols, start stirring and raise the temperature to 110°C under a vacuum of -95KPa to vacuumize for 1 hour. Add 7.5Kg of anhydrous sodium hypophosphite, raise the temperature to 115°C, maintain absolute pressure -95KPa vacuum stirring reaction for 2h, then filter, and the filtrate is adsorbed by resin to remove residual H + , and then the above-mentioned filtrate is sent to a molecular distillation tower, and the temperature in the kettle is controlled at 120° C. to dealcoholize under the condition of an absolute pressure of 80 Pa and a vacuum degree. After dealcoholization, the temperature was lowered to 80°C, and 2.5 tons of distilled water was added to adjust the solid content to 50% to obtain a light yellow aqueous solution of alkyl glycosides. Put the above alkyl glucoside solution into the bleaching tank, add 15 kg of 30% hydrogen peroxide, stir and heat at a c...

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Abstract

The invention relates to an alkyl glucoside preparation method. The invention aims at solving a technical problem of providing a preparation method with simple preparation process and wide product application range. The invention adopts a technical scheme that the alkyl glucoside preparation method comprises the steps that: (1) glucose and fatty alcohol are added into a reaction kettle; a temperature is increased to 100-120 DEG C, and the reaction kettle is vacuumed to a pressure of -5Kpa to -98Kpa; a catalyst is added, and a gycosylation reaction is carried out for 2-4h; (2) after the reaction, filtering is carried out when the product is still hot; non-reacted glucose and most of the catalyst are removed; and residual trace acid in a reaction liquid is absorbed by using resin; (3) free fatty alcohol in the mixture is removed by distillation; (4) water is added, and a water solution with a water content of 30-75% is prepared; and a decolorization agent is added such that decolorization is carried out; and (5) a solution pH is regulated to 8-11, such that an alkyl glucoside product is obtained.

Description

technical field [0001] The invention relates to the technical field of fine chemicals, in particular to a method for preparing alkyl glycosides. technical background [0002] Alkylpolyglycoside (APG for short) is a new type of surfactant developed in the late 1980s and early 1990s. It uses renewable resource carbohydrates and long-chain natural fatty alcohols as raw materials, and dehydrates them with acids as catalysts. produced by condensation. APG has many advantages of both non-ionic and anionic surfactants, such as high activity, strong detergency, rich, delicate and stable foam, good compatibility with other surfactants, good biodegradation, non-toxic, non-polluting, etc. Known as a "world-class" surfactant, it is widely used in detergents, industrial emulsifiers, cosmetics, food and pharmaceutical industries. [0003] At present, the synthesis method for the production of alkyl glycosides mainly adopts a one-step method, that is, under a certain temperature, pressur...

Claims

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Application Information

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Patent Type & Authority Patents(China)
IPC IPC(8): C07H15/04C07H1/00
Inventor 郭霞吴维高史立文葛赞黄亚茹方银军华文高
Owner ZANYU TECH GRP CO LTD