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A kind of preparation method and application of high-efficiency adsorption modified starch microspheres

A technology of modified starch and starch microspheres, which is applied in chemical instruments and methods, adsorption water/sewage treatment, textile industry wastewater treatment, etc. It can solve the problems of single adsorption reaction active point and limited pollutant adsorption amount, and improve the reaction rate. efficiency, increasing adsorption active sites, and improving chemical stability

Inactive Publication Date: 2016-01-20
GUANGDONG UNIV OF TECH
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

However, in the application of wastewater treatment, starch microspheres have two technical problems: (1) starch microspheres mainly rely on pore volume and specific surface area to perform physical adsorption, the adsorption reaction activity point is single, and the adsorption capacity of pollutants is limited.

Method used

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Examples

Experimental program
Comparison scheme
Effect test

Embodiment 1

[0023] (1) Add 100 g of starch to 140 ml of water, stir evenly, add 1.2 g of sodium chloride and 9.6 mL of epichlorohydrin, adjust the pH to 11.0 with NaOH solution, stir for 16 hours, and then use acetic acid to adjust the pH to 6.0, stand for precipitation, the precipitate is washed twice with water first, then washed with 70% alcohol for 4 times, and finally suction filtered, and the solid is dried in an oven at 60 °C to obtain starch microspheres.

[0024] (2) Fully mix 20 grams of urea, 2 mL of 85% phosphoric acid, and 2 grams of sodium citrate, add 7 mL of ethanol, stir until the urea and sodium citrate are completely dissolved, then add 26 grams of starch microspheres, stir evenly, and place in a 650w microwave oven Heating for 5 minutes (5 seconds for every 10 seconds of heating), the product was washed 3 times with water, then 4 times with 70% alcohol, and finally filtered with suction, and the solid was dried in an oven at 70 °C to obtain modified starch microspheres....

Embodiment 2

[0027] (1) Add 100g of starch to 150ml of water, stir evenly, add 1.5g of sodium chloride and 10mL of epichlorohydrin, adjust the pH to 12.0 with NaOH solution, stir for 15 hours, and then adjust the pH to 6.0 with acetic acid , stand for precipitation, the precipitate is first washed with water 4 times, then washed with 70% alcohol twice, and finally suction filtered, and the solid is dried in an oven at 70 °C to obtain starch microspheres.

[0028] (2) Fully mix 20 grams of urea, 3 mL of 85% phosphoric acid, and 4 grams of sodium citrate, add 8 mL of ethanol, stir until the urea and sodium citrate are completely dissolved, then add 35 grams of starch microspheres, stir evenly, and place in a 650w microwave oven Heating for 2 minutes (5 seconds for every 10 seconds of heating), the product was washed twice with water and 4 times with 70% alcohol, and finally filtered with suction, and the solid was dried in an oven at 60 °C to obtain modified starch microspheres.

[0029] (3)...

Embodiment 3

[0031] (1) Add 100 g of starch to 160 ml of water, stir evenly, add 1.8 g of sodium chloride and 13 mL of epichlorohydrin, adjust the pH to 11.0 with NaOH solution, stir for 20 hours, and then adjust the pH to 6.0 with acetic acid , stand for precipitation, the precipitate is washed three times with water, then three times with 70% alcohol, and finally suction filtered, and the solid is dried in an oven at 60 °C to obtain starch microspheres.

[0032] (2) Fully mix 25 grams of urea, 3 mL of 85% phosphoric acid, and 1 gram of sodium citrate, add 12 mL of ethanol, stir until the urea and sodium citrate are completely dissolved, then add 44 grams of starch microspheres, stir evenly, and place in a 750w microwave oven Heating for 4 minutes (5 seconds for every 10 seconds of heating), the product was washed 3 times with water, then 4 times with 70% alcohol, and finally filtered with suction, and the solid was dried in an oven at 65 °C to obtain modified starch microspheres.

[0033...

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Abstract

The invention discloses a preparation method of high-efficiency adsorptive modified starch microspheres, the obtained adsorptive modified starch microspheres and a use method thereof. In the present invention, starch, urea and phosphoric acid are synthesized under certain reaction conditions to obtain phosphoric acid-carbamic acid starch ester, which greatly improves the adsorption capacity, and also introduces carbamate groups to improve the water solubility of phosphoric acid-carbamic acid starch ester. Thereby affecting its separation from the aqueous solution. The invention firstly prepares starch microspheres, and then uses starch microspheres, urea, phosphoric acid and sodium citrate as raw materials to prepare phosphoric acid-carbamic acid starch microspheres by a one-step method. The microsphere molecule of the present invention greatly improves the adsorption capacity. The modified starch microspheres prepared by the invention are especially suitable for the adsorption treatment of printing and dyeing wastewater.

Description

technical field [0001] The invention relates to a preparation method and application of high-efficiency adsorptive modified starch microspheres, belonging to the technical field of preparation of water treatment agents. The modified starch microspheres prepared by the invention are especially suitable for the adsorption treatment of printing and dyeing wastewater. Background technique [0002] While printing and dyeing has become an important industry for exporting and earning foreign exchange in my country, it has also become one of the industries with high energy consumption and high pollution. On average, it needs to consume 0.2-0.5m 3 The printing and dyeing wastewater contains dyes, pastes, additives, acids, alkalis, fiber impurities and inorganic salts, etc., which are extremely chromatic and difficult to handle. Especially in recent years, the stability of the dye structure has been greatly improved, further increasing the difficulty of decolorization. The methods o...

Claims

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Application Information

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Patent Type & Authority Patents(China)
IPC IPC(8): B01J20/24B01J20/28B01J20/30C02F1/28C02F103/30
Inventor 林亲铁潘建新赵健鄂
Owner GUANGDONG UNIV OF TECH