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A kind of preparation method of anionic waterborne polyurethane nano-silver composite coating

A water-based polyurethane and composite coating technology, which can be used in antifouling/underwater coatings, paints containing biocides, etc., and can solve problems such as wide particle size distribution of nano-silver

Inactive Publication Date: 2016-03-30
TONGJI UNIV
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

[0006] The purpose of the present invention is to provide a preparation method of anionic water-based polyurethane nano-silver composite coating to solve the problem of wide particle size distribution of nano-silver when existing polyurethane and nano-silver are combined

Method used

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Examples

Experimental program
Comparison scheme
Effect test

Embodiment 1

[0021] Vacuum dehydrate 100 parts of sulfonated water-soluble polyester polyol BY3301 and 33.3 parts of aliphatic isocyanate IPDI, stir evenly, heat up to 90°C for 2 hours, add 100 parts of acetone to cool down, then add 7.2 parts of diethyl ethylene glycol (DEG) , 2 drops of catalyst stannous octoate (T-9), 2 drops of dibutyltin dilaurate (T-12), maintain the temperature at 80°C for 4 hours, add 6.9 parts of sodium sulfamate (A95) after cooling down, and maintain the reaction at 40°C After half an hour, cool and discharge the material, use a high-speed mixer to add ice water to emulsify, and finally remove acetone. The solid content of sulfonate-type water-based polyurethane is 48-52%.

[0022] Take 10ml of sulfonate aqueous polyurethane emulsion, add 20ml of deionized water, add 5ml of silver nitrate solution (concentration 3mg / ml) and stir well. Add sodium borohydride NaBH while stirring 4 , wherein the molar ratio of silver nitrate to sodium borohydride is 1:3, the color ...

Embodiment 2

[0024] 100 parts of sulfonated water-soluble polyester polyol BY3301 and 33.3 parts of aliphatic isocyanate IPDI are vacuum dehydrated, stirred evenly, heated to 90°C for 2 hours, added 80 parts of acetone to cool down, then added 7.2 parts of diethyl ethylene glycol (DEG) , 2 drops of catalyst stannous octoate (T-9), 2 drops of dibutyltin dilaurate (T-12), maintain the temperature at 80°C for 4 hours, add 6.9 parts of sodium sulfamate (A95) after cooling down, and maintain the reaction at 40°C After half an hour, cool and discharge the material, use a high-speed mixer to add ice water to emulsify, and finally remove acetone. The solid content of sulfonate-type water-based polyurethane is 48-52%.

[0025] Take 10ml of sulfonate aqueous polyurethane emulsion, add 10ml of deionized water, add 5ml of silver nitrate solution (concentration 3mg / ml) and stir well. Add sodium borohydride NaBH while stirring 4 , wherein the molar ratio of silver nitrate to sodium borohydride is 1:3, ...

Embodiment 3

[0027] Vacuum dehydrate 100 parts of sulfonated water-soluble polyester polyol BY3301 and 33.3 parts of aliphatic isocyanate IPDI, stir evenly, heat up to 90°C for 2 hours, add 100 parts of acetone to cool down, then add 7.2 parts of diethyl ethylene glycol (DEG) , 2 drops of catalyst stannous octoate (T-9), 2 drops of dibutyltin dilaurate (T-12), maintain the temperature at 80°C for 4 hours, add 6.9 parts of sodium sulfamate (A95) after cooling down, and maintain the reaction at 40°C After half an hour, cool and discharge the material, use a high-speed mixer to add ice water to emulsify, and finally remove acetone. The solid content of sulfonate-type water-based polyurethane is 48-52%.

[0028] Take 10ml of sulfonate aqueous polyurethane emulsion, add 5ml of deionized water, add 5ml of silver nitrate solution (concentration 3mg / ml) and stir well. Add sodium borohydride NaBH while stirring 4 , wherein the molar ratio of silver nitrate to sodium borohydride is 1:3, the color o...

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PUM

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Abstract

The invention relates to a preparation method of an anionic waterborne polyurethane nano-silver composite coating. The composite coating first synthesizes an anionic waterborne polyurethane with high solid content, and then in-situ reduces in an anionic waterborne polyurethane system to generate nano-silver, and then dialyzes the composite solution until the pH is neutral, and finally spray the composite emulsion on the surface of the corresponding substrate to obtain an anionic waterborne polyurethane nano-silver composite coating. This composite system uses the anionic sulfonate group on the molecular chain of the The reducing agent is reduced in situ to generate nano-silver. This preparation process can effectively control the distribution and particle size of nano-silver in the water-based polyurethane composite system, and the particle size of nano-silver is controlled within 20 nanometers.

Description

technical field [0001] The invention belongs to the field of water-based polyurethane / nano precious metal organic-inorganic composite, and in particular relates to a preparation method of an anionic water-based polyurethane nano-silver composite coating. Background technique [0002] As an emerging functional material, nano silver has very stable physical and chemical properties, and has excellent performance in electronics, optics, antibacterial and catalysis, and can be widely used in catalyst materials, battery electrode materials, optical materials, antibacterial materials, coatings, etc. Silver ion is one of the metal ions with the strongest bactericidal and antibacterial activity. It can destroy the respiratory function of bacteria and viruses and cause cell division. Nano-silver has become one of the most promising antibacterial materials through the slow-release process of Ag+ by surface atoms. [0003] Water-based polyurethane (WPU) is relative to solvent-based po...

Claims

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Application Information

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Patent Type & Authority Patents(China)
IPC IPC(8): C09D175/06C09D5/14C08G18/75C08G18/66C08G18/46B22F9/24
Inventor 钟震彭金涛李远耀李健任天斌
Owner TONGJI UNIV