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Method for modifying positive aluminum foil current collector by utilizing phosphoric acid-fluorine-dichromate

A dichromate and current collector technology, applied in the direction of electrode carrier/current collector, battery electrode, hybrid capacitor current collector, etc., can solve the problems of high cost, complicated preparation process and limited effect

Inactive Publication Date: 2014-06-18
FUJIAN NORMAL UNIV
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

However, the above methods of pre-coating graphene and carbon powder on the aluminum foil current collector have limited effects on improving the performance of the positive aluminum foil current collector, and the preparation process is complicated and the cost is high. Therefore, the present invention uses a simple surface treatment method to improve lithium The surface properties of the positive electrode aluminum foil current collector of the ion battery can reduce the impedance between the positive electrode aluminum foil current collector and the positive electrode material of the lithium ion battery, and reduce the powder dropping phenomenon of the positive electrode

Method used

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Examples

Experimental program
Comparison scheme
Effect test

Embodiment 1

[0011] The aluminum foil was treated with a treatment solution at 51° C. for 5 minutes, rinsed with water, and finally dried naturally to obtain a modified positive electrode aluminum foil current collector.

[0012] The composition of the treatment solution is as follows: sodium dihydrogen phosphate 15 g / L, sodium fluoride 6 g / L, potassium dichromate 5 g / L, 36 w.t.% hydrochloric acid 4 g / L.

[0013] The positive electrode aluminum foil current collector modified with phosphoric acid-fluorine-dichromate is folded in half 180° and returned to the original state, which is recorded as 180°, and then folded 180° is recorded as 360°, and so on. Tests have shown that the prepared modified positive electrode aluminum foil can be folded continuously at 6300° without breaking. Dissolve 3 g of polyvinylidene fluoride resin in 29 ml of dimethylacetamide to prepare viscose. The adhesive is coated on the aluminum foil current collector, and the peel strength reaches 0.0671 N / mm after heat...

Embodiment 2

[0016] The aluminum foil was treated with a treatment solution at 78 °C for 30 min, rinsed with water, and finally dried with hot air at 180 °C to obtain a modified positive electrode aluminum foil current collector.

[0017] The composition of the treatment liquid is as follows: sodium dihydrogen phosphate 19g / L, sodium fluoride 10g / L, potassium dichromate 6g / L, 37 w.t.% concentrated hydrochloric acid 6g / L.

[0018] When the prepared modified positive electrode aluminum foil current collector is used as the positive electrode current collector of the lithium ion battery, it has the advantages of good folding resistance, strong adhesion with the positive electrode material, small impedance, and excellent charge and discharge performance.

Embodiment 3

[0020] The aluminum foil was treated with a treatment solution at 35°C for 1 min, rinsed with water, and finally dried with hot air at 70°C to obtain a modified positive electrode aluminum foil current collector.

[0021] The composition of the treatment solution is as follows: sodium dihydrogen phosphate 10 g / L, sodium fluoride 2 g / L, potassium dichromate 3 g / L, 37 w.t.% concentrated hydrochloric acid 2 g / L.

[0022] When the prepared modified positive electrode aluminum foil current collector is used as the positive electrode current collector of the lithium ion battery, it has the advantages of good folding resistance, strong adhesion with the positive electrode material, small impedance, and excellent charge and discharge performance.

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Abstract

The invention relates to a method for modifying a positive aluminum foil current collector by utilizing phosphoric acid-fluorine-dichromate. The method is characterized by comprising the following steps of processing an aluminum foil for 1min to 30min by utilizing processing liquid at the temperature of 35 to 78 DEG C, washing the aluminum foil by utilizing the water, and finally naturally drying the aluminum foil or drying the aluminum foil by utilizing hot air at the temperature of 70 to 180 DEG C to obtain the modified positive aluminum foil current collector. When the prepared modified positive aluminum foil current collector is applied to a battery or a supercapacitor, the aluminum foil current collector has the advantages of good bending resistance, strong cohesive force with a positive material, small impedance, excellent charging-discharging performance and the like.

Description

technical field [0001] The invention belongs to the technical field of battery electrode preparation, and specifically relates to a positive electrode aluminum foil current collector modified with phosphoric acid-fluorine-dichromate, which can be used in lithium batteries, lithium ion batteries, polymer batteries and supercapacitors. technical background [0002] Lithium-ion batteries have the advantages of high battery voltage, high energy density, no memory effect, long cycle life, and low self-discharge. The performance of positive electrode materials plays a decisive role in the performance of lithium-ion batteries. At present, lithium-ion batteries are mainly composed of organic electrolyte (polymer electrolyte), separator, positive electrode, negative electrode, current collector and other components. Due to the weak conductivity of the liquid organic electrolyte (or polymer electrolyte) used in lithium-ion batteries, in order to achieve the high-current charge and dis...

Claims

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Application Information

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IPC IPC(8): H01M4/66H01G11/66
CPCH01G11/68H01M4/661H01M4/667H01M10/0525Y02E60/10Y02E60/13
Inventor 童庆松潘国涛练冲任媛媛吕超吴钦缘李秀华
Owner FUJIAN NORMAL UNIV