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Preparation method of lithium battery cathode material cobalt hydroxide

A technology of cobalt hydroxide and positive electrode materials, which is applied in the direction of cobalt oxide/cobalt hydroxide, battery electrodes, lithium batteries, etc., can solve the problems of harsh drying conditions, long production process, wide particle size distribution of cobalt hydroxide, etc., and achieve particle size distribution Narrow, good sphericity, low cost effect

Active Publication Date: 2017-03-08
CNGR ADVANCED MATERIAL CO LTD
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

This method has a long production process and harsh drying conditions, which is not conducive to industrialized production
Therefore, the problems in the prior art have: 1. the particle size distribution of cobalt hydroxide is too wide; 2. the sphericity of cobalt hydroxide is not good

Method used

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Examples

Experimental program
Comparison scheme
Effect test

Embodiment 1

[0024] The preparation method of lithium battery cathode material cobalt hydroxide is characterized in that it comprises the following steps:

[0025] 1) Prepare crystal nucleus by hydrolysis precipitation, add cobalt isopropoxide into pure water, then add dispersant, start stirring at the same time, stirring speed is 700r / min, react at 80°C for 5 hours, and obtain cobalt hydroxide precipitate as crystal nucleus;

[0026] 2) Homogeneous precipitation, the obtained cobalt hydroxide crystal nucleus is added into pure water according to 8 times its mass to make a slurry, then the pure cobalt solution and urea are added, and the temperature is raised to 99°C at a rate of 3.5°C / h, and constant temperature reaction 6 hours, stirring speed 700r / min;

[0027] 3) Alkali washing, filter the material obtained by homogeneous precipitation, add the filtered material to 0.9mol / l sodium hydroxide solution and soak for 3 hours, the soaking temperature is 75°C, and then filter the soaked slurr...

Embodiment 2

[0036] The preparation method of lithium battery cathode material cobalt hydroxide is characterized in that it comprises the following steps:

[0037] 1) Prepare crystal nucleus by hydrolysis precipitation, add cobalt isopropoxide into pure water, then add dispersant, start stirring at the same time, stirring speed is 1100r / min, react at 85°C for 6 hours, and obtain cobalt hydroxide precipitate as crystal nucleus;

[0038] 2) Homogeneous precipitation, the obtained cobalt hydroxide crystal nucleus is added into pure water according to 5 times its mass to make a slurry, then the pure cobalt solution and urea are added, the temperature is raised to 97°C at a rate of 4°C / h, and constant temperature reaction 5 hours, stirring speed 500r / min;

[0039] 3) Alkali washing, filter the material obtained by homogeneous precipitation, add the filtered material to 2.5mol / l sodium hydroxide solution and soak for 3 hours, the soaking temperature is 78°C, and then filter the soaked slurry;

...

Embodiment 3

[0048] The preparation method of lithium battery cathode material cobalt hydroxide is characterized in that it comprises the following steps:

[0049] 1) Prepare crystal nuclei by hydrolysis and precipitation, add cobalt isopropoxide into pure water, then add dispersant, and start stirring at the same time at a stirring speed of 900r / min, and react at 65°C for 7 hours to obtain cobalt hydroxide precipitates as crystal nuclei;

[0050] 2) Homogeneous precipitation, the obtained cobalt hydroxide crystal nucleus is added into pure water according to 6 times its mass to make a slurry, then the pure cobalt solution and urea are added, and the temperature is raised to 98°C at a rate of 4°C / h, and constant temperature reaction 7 hours, stirring speed 750r / min;

[0051] 3) Alkali washing, filter the material obtained by homogeneous precipitation, add the filter material to 2mol / l sodium hydroxide solution and soak for 3.5 hours, the soaking temperature is 80°C, and then filter the soa...

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PUM

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Abstract

The invention discloses a method for preparing a lithium battery anode material cobaltous hydroxide. The method comprises the following steps: 1) performing hydrolytic precipitation to prepare a crystal nucleus; 2) performing homogeneous precipitation; 3) performing alkali washing; and 4) performing after-treatment. A cobaltous hydroxide crystal nucleus which is uniform in particle size distribution can be prepared through hydrolytic precipitation, and the cobaltous hydroxide crystal nucleus can be further added into a reaction kettle to prepare large-particle cobaltous hydroxide through homogeneous precipitation. By adopting the method for preparing the lithium battery anode material cobaltous hydroxide, the prepared cobaltous hydroxide is narrow in particle size distribution and good in degree of sphericity.

Description

technical field [0001] The invention relates to the field of preparation of new energy materials, in particular to a preparation method of cobalt hydroxide, a cathode material of a lithium battery. Background technique [0002] Cobalt hydroxide is an important precursor of lithium battery cathode materials, which is used to produce lithium cobalt oxide cathode lithium battery materials. With the rapid development of my country's economy and society, green energy is favored by people, the battery industry continues to develop at a high speed, and the application fields of cobalt hydroxide continue to expand, and the market demand is also increasing. [0003] The existing methods for preparing cobalt hydroxide include alkali solution precipitation method, precipitation transformation method and the like. For example, H.C. Stark's invention patent CN1190947 discloses the preparation of large particle size cobalt hydroxide by precipitation conversion method. First, cobalt salt ...

Claims

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Application Information

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Patent Type & Authority Patents(China)
IPC IPC(8): H01M4/52C01G51/04H01M10/052
CPCY02E60/10
Inventor 訚硕刘兴国
Owner CNGR ADVANCED MATERIAL CO LTD