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Preparation method for crosslinking modification membrane with non-woven fabrics as matrix

A technology of cross-linking modification and non-woven fabrics, which is applied in the direction of chemical instruments and methods, membranes, membrane technology, etc. It can solve the problems of cumbersome modification steps and difficult long-lasting modification effects, so as to achieve the goal of not being prone to secondary pollution and modification The effect of long-lasting and stable effect and good flux recovery performance

Active Publication Date: 2016-07-13
ZHEJIANG UNIV OF TECH
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

However, the above method has the disadvantages that the modification effect is difficult to last or the modification steps are cumbersome.

Method used

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Examples

Experimental program
Comparison scheme
Effect test

Embodiment 1

[0020] 1) Weigh 13g of hydroxyethyl methacrylate and 0.126g of allyl methacrylate respectively, dissolve them in 52.5g of methanol, then add 16.4mg of initiator azobisisobutyronitrile, seal under nitrogen protection, and store at 60°C After reacting in a water bath for 6 hours, precipitate in ether, and dry in a vacuum oven at 60°C for 12 hours to obtain a prepolymer;

[0021] 2) Weigh 2g of prepolymer and dissolve it in 4.7g of methanol, and add 15.3mg of cross-linking agent 3,6-dioxa-1,8-octanedithiol and 21.4mg of photoinitiator benzoin dimethyl ether to form a scraper The film solution was scraped and coated on the non-woven fabric with a 200μm scraper, and immediately put in 2μW / cm 2 It was irradiated under ultraviolet light for 300s, and dried and stored at room temperature.

Embodiment 2

[0023] 1) Weigh 13g of hydroxyethyl methacrylate and 0.21g of allyl methacrylate respectively, dissolve them in 52.8g of methanol, then add 16.4mg of initiator azobisisobutyronitrile, seal under nitrogen protection, and store at 60°C After reacting in a water bath for 8 hours, precipitate in ether, and dry in a vacuum oven at 60°C for 12 hours to obtain a prepolymer;

[0024] 2) Weigh 2g of prepolymer and dissolve it in 4.7g of methanol, and add 25.2mg of cross-linking agent 3,6-dioxa-1,8-octanedithiol and 35.5mg of photoinitiator benzoin dimethyl ether to form a scraper The film solution was scraped and coated on the non-woven fabric with a 200μm scraper, and immediately put in 2μW / cm 2 It was irradiated under ultraviolet light for 300s, and dried and stored at room temperature.

Embodiment 3

[0026] 1) Weigh 13g of hydroxyethyl methacrylate and 0.63g of allyl methacrylate respectively, dissolve them in 54.5g of methanol, then add 16.4mg of initiator azobisisobutyronitrile, seal under nitrogen protection, and store at 60°C After reacting in a water bath for 10 hours, precipitate in ether, and dry in a vacuum oven at 60°C for 12 hours to obtain a prepolymer;

[0027] 2) Weigh 2g of prepolymer and dissolve it in 4.7g of methanol, and add 73.5mg of cross-linking agent 3,6-dioxa-1,8-octanedithiol and 0.1g of photoinitiator benzoin dimethyl ether to form a scraper The film solution was scraped and coated on the non-woven fabric with a 200μm scraper, and immediately put in 2μW / cm 2 It was irradiated under ultraviolet light for 300s, and dried and stored at room temperature.

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PUM

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Abstract

The invention discloses a preparation method for a crosslinking modification membrane with non-woven fabrics as a matrix. The method comprises the following steps of weighing a certain amount of hydrophilic monomer and a certain amount of allyl methacrylate to be dissolved in a methyl alcohol solution, then, adding an initiator, sealing and using nitrogen for protection, performing a stirring reaction in a water bath kettle, then, performing precipitation separation in a diethyl ether solution to obtain a prepolymer, using methyl alcohol and diethyl ether for repeated washing, and performing drying in a vacuum drying oven to obtain the prepolymer; dissolving the synthetized prepolymer into the methyl alcohol, adding a crosslinking agent and a photoinitiator to form a film scraping solution, using a scraper for blade coating of the non-woven fabrics with the film scraping solution, putting the non-woven fabrics under ultraviolet light immediately for irradiation crosslinking, and performing drying storage at normal temperature for use. The method is easy to implement, mild in reaction condition and low in energy consumption, the obtained compound modification non-woven fabrics have the excellent hydrophilia and protein pollution resistance, secondary pollution is not likely to be caused, and the modification effect is lasting.

Description

technical field [0001] The invention relates to a preparation method of a cross-linked modified film with a non-woven fabric as a matrix. Background technique [0002] Non-woven fabric is a new type of filter medium emerging in the world since the 21st century, and its application in membrane separation technology is becoming more and more mature. In particular, polypropylene non-woven fabric has the characteristics of high porosity, economical price, high specific surface area and excellent spatial structure, making it a hot choice for separation materials. However, the single physical and chemical properties and strong hydrophobicity of the surface of polypropylene non-woven fabrics lead to poor wettability, large water contact angle and low water flux during filtration; secondly, due to the lack of necessary functional adsorption sites on the surface, The limited ability to adsorb pollutants in water, especially proteins, will eventually lead to protein deposition on the...

Claims

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Application Information

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IPC IPC(8): B01D67/00B01D69/02B01D71/44
CPCB01D67/0011B01D69/02B01D71/44B01D2325/36
Inventor 费正东朱雅芝王涛范萍陈枫钟明强
Owner ZHEJIANG UNIV OF TECH