Organic electroluminescent compound, use thereof and organic electroluminescent device
A compound and electroluminescence technology, applied in the fields of organic chemistry, electro-solid devices, electrical components, etc., can solve the problems of low luminous efficiency and high device operating voltage, and achieve the effect of improving luminous efficiency and reducing operating voltage
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[0042] Preparation of organic electroluminescent compounds:
[0043] Synthesis Example 1. Synthesis of Intermediate M1:
[0044]
[0045] Add 1,2-bis(bromomethyl)benzene (26.4g, 0.1mol) and 500ml of anhydrous tetrahydrofuran (THF) into a 1-liter three-necked flask, and add activated zinc powder (13g, 0.2mol), reacted for 2 hours to make a double zinc reagent. CuI (2 g, 10 mmol) and phthaloyl chloride (20 g, 0.1 mol) were added, and reacted at room temperature for 1 hour, and then reacted under reflux for 10 hours. After completion of the reaction, slowly add saturated ammonium chloride aqueous solution to quench the reaction, then extract three times with 100ml ethyl acetate, combine the organic phases obtained, anhydrous MgSO 4 After drying and removing the organic solvent under reduced pressure, the residue was subjected to column separation to obtain intermediate compound M (18.5 g, yield 78.4%).
[0046] Add phenylhydrazine hydrochloride (63.6 g, 0.44 mol), intermedi...
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