Photovoltaic components
A technology of photovoltaic elements and photoelectric conversion layers, applied in photovoltaic power generation, electrical components, electric solid-state devices, etc., can solve the problems of low photoelectric conversion efficiency and durability of organic solar cells, and achieve high photoelectric conversion efficiency and excellent durability Effect
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[0100] Hereinafter, based on an Example, this invention is demonstrated more concretely. It should be noted that the present invention is not limited to the following examples. In addition, among the compounds used in Examples and the like, the abbreviations for use are shown below.
[0101] Isc: short circuit current density
[0102]Voc: open circuit voltage
[0103] η: Photoelectric conversion efficiency
[0105] A-1: A compound represented by the following formula
[0106] A-2: A compound represented by the following formula
[0107] [chemical 7]
[0108]
[0109]
[0110] [70] PCBM: methyl phenyl C71 butyrate.
[0111] The photoelectric conversion efficiency in each example and comparative example was calculated|required by the following formula.
[0112] η(%)=Isc(mA / cm 2 )×Voc(V)×FF / irradiation light intensity (mW / cm 2 )×100
[0113] FF=JVmax / (Isc(mA / cm 2 )×Voc(V))
[0114] JVmax (mW / cm 2 ) is the product value of the cur...
Synthetic example 1
[0118] Compound A-1 was synthesized by the method shown in the following formula.
[0119] [chemical 8]
[0120] .
[0121] 4.3 g of compound (1-a) (manufactured by Tokyo Chemical Industry Co., Ltd.) and 10 g of bromine (manufactured by Wako Pure Chemical Industries, Ltd.) were added to 48% hydrobromic acid (manufactured by Wako Pure Chemical Industries, Ltd.) 150ml, stirred at 120°C for 3 hours. After cooling to room temperature, the precipitated solid was filtered through a glass filter, and washed with 1000 ml of water and 100 ml of acetone. The obtained solid was vacuum-dried at 60° C. to obtain 6.72 g of compound (1-b).
[0122] Add 5.56 g of compound (1-b) to 180 ml of ethanol (manufactured by Wako Pure Chemical Industries, Ltd.), and add NaBH at 5°C under a nitrogen atmosphere 4 (manufactured by Wako Pure Chemical Industries, Ltd.) 13.2 g, and stirred at room temperature for 2 days. After distilling off the solvent, 500 ml of water was added, and the solid was co...
Synthetic example 2
[0129] Compound A-2 was synthesized by the method shown in the following formula. It should be noted that the compound (2-i) described in Synthesis Example 2 was synthesized with reference to the method described in Jana Luobza American Chemical Society (Journal of the American Chemical Society), 2009, Volume 131, pages 7792-7799, and compound (2 -p) Synthesized by referring to the method described in Angebante Chemiinternasionaru Edison (Angewandte Chemie International Edition), 2011, Vol. 50, pp. 9697-9702.
[0130] [chemical 9]
[0131] .
[0132] 38 g (0.27 mol) of methyl 2-thiophenecarboxylate (manufactured by Tokyo Chemical Industry Co., Ltd.) and 108 g (1.34 mol) of chloromethyl methyl ether (manufactured by Tokyo Chemical Industry Co., Ltd.) were stirred at 0° C. After adding 125 g (0.48 mol) of tin tetrachloride (manufactured by Wako Pure Chemical Industries, Ltd.) over 1 hour, it stirred at room temperature for 8 hours. After the stirring was completed, 100 ml o...
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