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Synthetic method of renewable polyester polyol

A technology of polyester polyol and synthesis method, which is applied in the field of synthesis of renewable polyester polyol, can solve problems such as less research, and achieve the effects of wide sources, excellent hydrolysis resistance and solvent resistance, and low price

Active Publication Date: 2017-06-23
ZHANGJIAGANG NANGUANG CHEM
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

However, most studies are limited to triglycerides in vegetable oils, and there are fewer studies on oleic acid, a derivative of vegetable oils

Method used

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Examples

Experimental program
Comparison scheme
Effect test

Embodiment 1

[0038] The synthetic method of renewable polyester polyol comprises the following steps:

[0039] 1) The following raw materials in parts by weight:

[0040] 40 parts of industrial grade oleic acid with a purity above 90%; 40 parts of maleic anhydride; 160 parts of diethylene glycol; 0.2-0.3 parts of hindered phenolic antioxidant; 0.6-0.7 parts of hydroquinone; 0.1-0.2 parts of tetramethyl titanate; 0.2 parts of an alkaline alcohol solution composed of methanol and KOH, the mass concentration of the alkaline alcohol solution being 10%;

[0041] 2) Preliminary reaction of oleic acid: in N 2 Under the atmosphere, mix all the technical grade oleic acid, all the maleic anhydride, and 0.3 parts of hydroquinone and 0.1 parts of hindered phenolic antioxidant, and then heat to 210 °C at a heating rate of 20 ° C / h ℃ and keep the temperature for reaction. During the reaction, the mixed solution is constantly stirred until the water output reaches 85% of the theoretical water output,...

Embodiment 2

[0045] The synthetic method of renewable polyester polyol comprises the following steps:

[0046] 1) The following raw materials in parts by weight:

[0047] 60 parts of industrial grade oleic acid with a purity of more than 90%; 50 parts of maleic anhydride; 220 parts of diethylene glycol; 0.3 parts of phosphite antioxidant; 0.7 parts of hydroquinone; 0.2 part of ethyl ester; 0.2 part of alkaline alcohol solution composed of ethanol and NaOH, the mass concentration of the alkaline alcohol solution is 10%;

[0048] 2) Preliminary reaction of oleic acid: in N 2Under the atmosphere, mix all the technical grade oleic acid, all the maleic anhydride, and 0.3 part of hydroquinone and 0.1 part of phosphite antioxidant, and then heat at a heating rate of 20°C / h to 230°C and keep the temperature for reaction. During the reaction process, the mixed solution is constantly stirred until the water output reaches 85% of the theoretical water output. The acid value of the maleic anhydride...

Embodiment 3

[0055] The synthetic method of renewable polyester polyol comprises the following steps:

[0056] 1) The following raw materials in parts by weight:

[0057] 50 parts of industrial-grade oleic acid with a purity of more than 90%; 45 parts of maleic anhydride; 200 parts of diethylene glycol; 0.3 parts of composite antioxidants; 0.6 parts of hydroquinone; tetraisopropyl titanate 0.2 part of ester; 0.2 part of sodium methoxide solution, the mass concentration of the sodium methoxide solution is 20%;

[0058] 2) Preliminary reaction of oleic acid: in N 2 Under the atmosphere, mix all the industrial grade oleic acid, all the maleic anhydride, 0.3 part of hydroquinone and 0.1 part of composite antioxidant, and then heat it to 220°C at a heating rate of 20°C / h And keep the temperature for reaction, constantly stir the mixed solution during the reaction, until the water yield reaches 85% of the theoretical water yield, the reaction is complete, then lower the temperature to 110°C to...

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Abstract

The invention discloses a synthetic method of renewable polyester polyol. The synthetic method adopts industrial grade oleic acid as a main raw material. The synthetic method comprises the following steps: firstly utilizing the industrial grade oleic acid to have ene reaction with maleic anhydride to obtain an oleic acid maleation product, then utilizing the oleic acid maleation product to have polycondensation reaction with diethylene glycol, adding an alkaline alcohol solution, distilling to decrease an acidic value, and obtaining the renewable polyester polyol with a high hydroxyl value and low acidic value. The raw materials used in the synthetic method are easy to get and low in price; the hydroxyl value of the prepared polyester polyol is 230 to 240 mgKOH / g, the acidic value is lower than 0.8mgKOH / g, the viscosity is 2200 to 2400Pa.s, the acidic value is relatively low, so that the subsequent synthesis of polyurethane is facilitated; and the synthesized renewable polyester polyol has the characteristics of high bonding strength, excellent hydrolysis resistance, excellent solvent resistance, and the like.

Description

technical field [0001] The invention relates to a synthetic method of polyester polyol, in particular to a synthetic method of renewable polyester polyol. Background technique [0002] Polyurethane materials, as more and more polymer materials, are widely used in construction, transportation, textiles, printing and packaging, adhesives and many other fields due to their excellent mechanical properties, high wear resistance and resilience, and diversified service conditions. . [0003] Polyester polyols are usually formed by condensation (or transesterification) of organic dicarboxylic acids (anhydrides or esters) and polyols (including diols) or by polymerization of lactones and polyols, and are mainly used as raw materials for the synthesis of polyurethane resins . The preparation process is generally produced by a batch method: that is, the organic dicarboxylic acid (anhydride or ester) and polyol (including diol) are first added to the reactor to melt, and nitrogen is i...

Claims

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Application Information

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Patent Type & Authority Applications(China)
IPC IPC(8): C08G63/676C08G63/78C08G63/85
CPCC08G63/676C08G63/78C08G63/85
Inventor 颜迪冯向华
Owner ZHANGJIAGANG NANGUANG CHEM