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Method for recovering vanadium in acidic vanadium precipitation waste liquid of oxygen-enriched roasting

A technology of oxygen-enriched roasting and vanadium precipitation, which is applied in the direction of improving process efficiency, can solve the problems of high cost of extraction methods, slow treatment, large environmental pollution, etc., so as to reduce water consumption and environmental pollution, realize no waste water discharge, The effect of easy industrialization promotion

Active Publication Date: 2019-04-16
CHENGDU ADVANCED METAL MATERIALS IND TECH RES INST CO LTD
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

[0003] The extraction method is expensive and pollutes the environment, while the ion exchange resin or membrane method is expensive and slow to process
The amount of vanadium precipitation waste liquid in the acidic vanadium precipitation process is large, there are many kinds of metal impurities, and the valence state is not uniform. A method with relatively low cost and relatively large treatment capacity for the treatment of the vanadium-containing waste liquid and the recovery of vanadium

Method used

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Examples

Experimental program
Comparison scheme
Effect test

Embodiment 1

[0017] Select 100g of coconut shell activated carbon whose particle size is mostly 0.6 mm, put it into distilled water, clean it with ultrasonic waves for 15 minutes, take it out and put it into an acidic potassium permanganate solution containing potassium permanganate with a mass percent concentration of 5% for 24 hours. After 1 hour, rinse with distilled water twice, put it in an oven and dry it at 350°C for 3 hours. After cooling, add 10g styrene, 100g distilled water, 0.5g sodium dodecylsulfonate and stir evenly, then add 10g aminotrimethylene Base phosphonic acid, after heating up to 80°C and adding 0.1g of ammonium persulfate. Raise the temperature to 90°C and react for 5 hours, take it out and soak it in ethanol for 24 hours, after drying, put it into the waste liquid according to the volume ratio of activated carbon: vanadium precipitation waste liquid is 1:100, stir and react for 9 hours, filter, the metal in the obtained filtrate The impurity content is less than 0....

Embodiment 2

[0019] Select 100g of coconut shell activated carbon whose particle size is mostly 1.4 mm, put it into distilled water, clean it with ultrasonic waves for 20 minutes, take it out and put it into an acidic potassium permanganate solution containing potassium permanganate with a mass percent concentration of 7% for 30 minutes. After 1 hour, wash with distilled water twice, put it in an oven and bake at 400°C for 3 hours, then add 10g styrene, 100g distilled water, 0.8g sodium dodecylsulfonate and stir well, then add 20g aminotrimethylene Base phosphonic acid, after heating up to 80°C and adding 1g of ammonium persulfate. Raise the temperature to 90°C and react for 5 hours, take it out and soak it in ethanol for 30 hours, after drying, put it into the waste liquid according to the volume ratio of activated carbon: vanadium precipitation waste liquid: 2:100, stir and react for 10 hours, filter, and the metal in the obtained filtrate The impurity content is less than 0.019g / L, meet...

Embodiment 3

[0021] Select 100g of coconut shell activated carbon whose particle size is mostly 2.2 mm, put it into distilled water, clean it with ultrasonic waves for 25 minutes, take it out and put it into an acidic potassium permanganate solution containing potassium permanganate with a mass percent concentration of 8% for 36 hours. After 1 hour, rinse with distilled water for 3 times, put it in an oven and dry it at 450°C for 2 hours. After cooling, add 10g of styrene, 100g of distilled water, 1g of sodium dodecylsulfonate and stir evenly, then add 30g of aminotrimethylene Phosphonic acid, after heating up to 85°C and adding 1g of ammonium persulfate. Raise the temperature to 95°C and react for 4 hours, take it out and soak it in ethanol for 36 hours, after drying, put it into the waste liquid according to the volume ratio of activated carbon: vanadium precipitation waste liquid is 3:100, stir and react for 11 hours, then filter, the metal in the obtained filtrate The impurity content ...

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Abstract

The invention relates to the field of a recovery method for vanadium in vanadium precipitation waste liquid, in particular to the recovery method for vanadium in oxygen-enriched air roasting acid vanadium precipitation waste liquid. The method is low in cost and capable of recycling vanadium in the vanadium precipitation waste liquid effectively. The method comprises the following step of (1) pretreatment of activated carbon compound; (2) modification graft of activated carbon; (3) remove of metal impurities and concentration of vanadium; (4) sequestration desorption; and (5) vanadium precipitation. The method has the following obvious advantages of (1) being low in cost; (2) being capable of recycling vanadium completely and effectively; and (3) being easy to industrialized popularization. The method can be combined with a prior vanadium precipitation industrialized production line, so that the process of vanadium precipitation-waste liquid treatment-waste liquid recovery can be realized, the emission without waste water can be basically realized and the water consumption and the environmental pollution can be reduced. The method is particularly applicable to the recovery technology for vanadium in the oxygen-enriched air roasting acid vanadium precipitation waste liquid.

Description

technical field [0001] The invention relates to the field of methods for recovering vanadium in vanadium precipitation waste liquid, in particular to a method for recovering vanadium in oxygen-enriched roasting acidic vanadium precipitation waste liquid. Background technique [0002] Vanadium is an important strategic material. With the development of science and technology, the application fields of vanadium continue to expand, and the requirements for the purity of vanadium products are also getting higher and higher. The new processes for extracting vanadium are different, but the general process steps basically include five operating steps: oxygen-enriched roasting, leaching, separation and purification, precipitation, and calcination. Among the current common vanadium precipitation processes, the acidic ammonium salt vanadium precipitation process has become the main process for vanadium precipitation due to the high purity of the prepared product and good vanadium yiel...

Claims

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Application Information

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Patent Type & Authority Patents(China)
IPC IPC(8): C22B7/00C22B34/22C22B3/24
CPCC22B3/24C22B7/006C22B34/22Y02P10/20
Inventor 李道玉彭穗刘波陈勇
Owner CHENGDU ADVANCED METAL MATERIALS IND TECH RES INST CO LTD