A chemically modified Mannich base and its preparation method and application
A Mannich base and chemical modification technology, which is applied in the field of cleaning and utilization of light fuel oil engines, can solve problems such as oxidation and corrosion of metal surfaces, and achieve the effects of good compatibility, good thermal stability, and good polymerization selectivity
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Embodiment 1
[0056] Embodiment 1: the chemical modification of Mannich base
[0057] The specific modification method is as follows:
[0058] (1) Preparation of solvent: 2.5 parts by weight of paraformaldehyde are added to 10 parts by weight of methanol, heated to 60°C, and triethylamine with 3% of the total weight of methanol and paraformaldehyde is used as a catalyst, at a temperature of 80°C Reflux reaction for 3 hours, cooling; then add methanol and paraformaldehyde total weight 50% methylal, then add methanol, paraformaldehyde, methylal total weight 3% naphthalenesulfonic acid solid catalyst, heat up to 90°C, Continue to stir and reflux for 3 hours, stop stirring and cooling, filter and remove the solid catalyst to obtain a low polymerization degree methoxyl ether solvent;
[0059] (2) Mannich base and diethylenetriamine are weighed and mixed in a mass ratio of 2.5:1, and the low polymerization degree methoxy ether solvent prepared in step (1) is added, and the addition amount of the...
Embodiment 2
[0060] Embodiment 2: the chemical modification of Mannich base
[0061] The specific modification method is as follows:
[0062] (1) Preparation of solvent: with embodiment 1.
[0063] (2) Mannich base and p-hydroxydianiline are weighed and mixed in a mass ratio of 2.5:1, and the solvent prepared in step (1) is added, and the addition of solvent is Mannich base and p-hydroxydianiline total weight 20%, stirring in the reaction kettle, adding 2% naphthalenesulfonic acid solid catalyst of the total weight of p-hydroxydiphenylamine and Mannich base, controlling the temperature at 80-120 ° C and pressurizing under the protection of nitrogen with 1-2 kg of pressure, stirring and reacting After 3 hours, nitrogen gas was released, the unreacted solvent was removed by distillation, and the solid catalyst was removed by filtration to obtain chemically modified Mannich base B.
Embodiment 3
[0064] Embodiment 3: the chemical modification of Mannich base
[0065] The specific modification method is as follows:
[0066] (1) Preparation of solvent: with embodiment 1.
[0067] (2) Mannich base and dodecylphenol sulfonate isopropanol ammonium salt are weighed and mixed in a mass ratio of 3:1, and the solvent prepared in step (1) is added, and the amount of solvent added is Mannich base and 20% of the total weight of dodecylphenolsulfonic acid isopropanol ammonium salt, stir in the reactor, add Mannich base and dodecylphenolsulfonic acid isopropanol ammonium salt total weight 2.5% tetrachloride Tin catalyst, controlled temperature 80-120 ℃, pressurized 1-2 kg of nitrogen, stirred and reacted for 3 hours, released nitrogen, distilled off the unreacted solvent, filtered to remove the solid catalyst, and obtained chemically modified Mannich base c.
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