A method for catalytically preparing cyanophyll
A technology for catalytic preparation of chlorophyll, applied in the field of catalysis, can solve the problems of low conversion rate, inability to recycle the catalyst, poor selectivity of chlorophyll, etc., and achieve the effect of high conversion rate, good contact and easy recycling
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[0028] (1) Magnetic core ZnFe 2 o 4 preparation of
[0029] 3.0 mmol FeCl 3 ·6H 2 O and 1.5mmol Zn(Ac) 2 2H 2 O was dissolved in 40.0 mL of ethylene glycol solution, then 20.0 mmol of sodium acetate and 6.0 mmol of CTAB were added, and ultrasonic treatment was performed for 30 min at a power of 200 W to fully disperse it to obtain a mixture; then the mixture was placed in a water bath at 220 ° C Under the conditions, react for 24 hours to obtain a suspension, which is naturally cooled to room temperature, centrifuged, washed, and dried to obtain ZnFe 2 o 4 magnetic nanocrystals;
[0030] (2) ZnFe 2 o 4 Surface TiO 2 clad
[0031] 0.1g of ZnFe obtained in step 1) 2 o 4 The magnetic nanocrystals were dispersed in the dispersed phase mixed with 20mL ethylene glycol and 5mL deionized water, then 1.0mL ammonia water was added, and the power was 200W for 30min, and then tetra-titanate was added dropwise under the condition of vigorous stirring. Butyl ester, continue to...
Embodiment 1
[0037] The mixed solution obtained by mixing benzyl alcohol, acetal and water according to the molar ratio of 1:10:30 was stirred at room temperature at a stirring rate of 800r / min for 5min, and then adding 12% of the total mass of the mixed solution was magnetic For the ionic liquid catalyst, continue to stir and react for 60 minutes. After the reaction is completed, let it stand for 30 minutes. The magnetic ionic liquid catalyst in the lower layer is directly recycled without any treatment after being separated by a magnetic field. Complete raw materials; wherein, the ionic liquid Y and ZnFe in the magnetic ionic liquid 2 o 4 @TiO 2 The mass ratio of the carrier is 15wt%.
[0038] After analysis, the conversion rate of benzyl alcohol was 99.7%, and the yield of cyanin was 98.6%.
Embodiment 2
[0040] The mixed solution obtained by mixing benzyl alcohol, acetal and water according to the molar ratio of 1:5:10 was stirred at room temperature at a stirring rate of 500r / min for 8min, and then added magnetic For the ionic liquid catalyst, continue to stir and react for 30 minutes. After the reaction is completed, let it stand for 30 minutes. The magnetic ionic liquid catalyst in the lower layer is directly recycled without any treatment after being separated by a magnetic field. Complete raw materials; wherein, the ionic liquid Y and ZnFe in the magnetic ionic liquid 2 o 4 @TiO 2 The mass ratio of the carrier is 30wt%.
[0041] After analysis, the conversion rate of benzyl alcohol was 97.8%, and the yield of cyanin was 96.5%.
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